Antinormally Ordered Photodetection of Continuous-mode Field

When the electromagnetic field is detected by stimulated emission, rather than by absorption, antinormally ordered photodetection can be realized. One of the distinct features of this photodetection scheme is its sensitivity to zero-point fluctuation due to the existence of the spontaneous emission. We have recently succeeded in experimentally demonstrating the antinormally ordered photodetection by exploiting nondegenerate stimulated parametric down-conversion process. To properly account for the experiment, the detection process needs to be treated with time-dependent and continuous-mode operators because of the broadband nature of the parametric down-conversion process and the wide spectrum of the pump that we used. Here, we theoretically analyze the antinormally ordered intensity correlation of the continuous-mode fields by pursuing the detection process in the Heisenberg picture. It is shown that the excess positive correlation due to zero-point fluctuation reduces because of the frequency-distinguishability of the two emitted photon pairs.Comment: 11 pages, 1 figures, to appear in the special issue of Int. J. Quant. Info. for the NQSI workshop in Kyot

On the relationship between pump chirp and single-photon chirp in spontaneous parametric downconversion

We study the chronocyclic character, i.e. the joint temporal and spectral properties, of the single-photon constituents of photon pairs generated by spontaneous parametric down conversion. In particular we study how single photon properties, including purity and single-photon chirp, depend on photon pair properties, including the type of signal-idler spectral and correlations and the level of pump chirp.Comment: 13 pages, 6 figure

Subnanosecond spectral diffusion of a single quantum dot in a nanowire

We have studied spectral diffusion of the photoluminescence of a single CdSe quantum dot inserted in a ZnSe nanowire. We have measured the characteristic diffusion time as a function of pumping power and temperature using a recently developed technique [G. Sallen et al, Nature Photon. \textbf{4}, 696 (2010)] that offers subnanosecond resolution. These data are consistent with a model where only a \emph{single} carrier wanders around in traps located in the vicinity of the quantum dot

Subnanosecond spectral diffusion measurement using photon correlation

Spectral diffusion is a result of random spectral jumps of a narrow line as a result of a fluctuating environment. It is an important issue in spectroscopy, because the observed spectral broadening prevents access to the intrinsic line properties. However, its characteristic parameters provide local information on the environment of a light emitter embedded in a solid matrix, or moving within a fluid, leading to numerous applications in physics and biology. We present a new experimental technique for measuring spectral diffusion based on photon correlations within a spectral line. Autocorrelation on half of the line and cross-correlation between the two halves give a quantitative value of the spectral diffusion time, with a resolution only limited by the correlation set-up. We have measured spectral diffusion of the photoluminescence of a single light emitter with a time resolution of 90 ps, exceeding by four orders of magnitude the best resolution reported to date

Shaping the waveform of entangled photons

We demonstrate experimentally the tunable control of the joint spectrum, i.e. waveform and degree of frequency correlations, of paired photons generated in spontaneous parametric downconversion. This control is mediated by the spatial shape of the pump beam in a type-I noncollinear configuration. We discuss the applicability of this technique to other sources of frequency entangled photons, such as electromagnetically induced Raman transitions.Comment: 5 Pages, 4 Figure

Optimal focusing for maximal collection of entangled narrow-band photon pairs into single-mode fibers

We present a theoretical and experimental investigation of the emission characteristics and the flux of photon pairs generated by spontaneous parametric downconversion in quasi-phase matched bulk crystals for the use in quantum communication sources. We show that, by careful design, one can attain well defined modes close to the fundamental mode of optical fibers and obtain high coupling efficiencies also for bulk crystals, these being more easily aligned than crystal waveguides. We distinguish between singles coupling, conditional coincidence, and pair coupling, and show how each of these parameters can be maximized by varying the focusing of the pump mode and the fiber-matched modes using standard optical elements. Specifically we analyze a periodically poled KTP-crystal pumped by a 532 nm laser creating photon pairs at 810 nm and 1550 nm. Numerical calculations lead to coupling efficiencies above 94% at optimal focusing, which is found by the geometrical relation L/z_R to be ~ 1 to 2 for the pump mode and ~ 2 to 3 for the fiber-modes, where L is the crystal length and z_R is the Rayleigh-range of the mode-profile. These results are independent on L. By showing that the single-mode bandwidth decreases as 1/L, we can therefore design the source to produce and couple narrow bandwidth photon pairs well into the fibers. Smaller bandwidth means both less chromatic dispersion for long propagation distances in fibers, and that telecom Bragg gratings can be utilized to compensate for broadened photon packets--a vital problem for time-multiplexed qubits. Longer crystals also yield an increase in fiber photon flux proportional to sqrt{L}, and so, assuming correct focusing, we can only see advantages using long crystals.Comment: 19 pages, 15 figures, ReVTeX4, minor revisio

Mode-coupling theory for structural and conformational dynamics of polymer melts

A mode-coupling theory for dense polymeric systems is developed which unifyingly incorporates the segmental cage effect relevant for structural slowing down and polymer chain conformational degrees of freedom. An ideal glass transition of polymer melts is predicted which becomes molecular-weight independent for large molecules. The theory provides a microscopic justification for the use of the Rouse theory in polymer melts, and the results for Rouse-mode correlators and mean-squared displacements are in good agreement with computer simulation results.Comment: 4 pages, 3 figures, Phys. Rev. Lett. in pres

Single-qubit optical quantum fingerprinting

We analyze and demonstrate the feasibility and superiority of linear optical single-qubit fingerprinting over its classical counterpart. For one-qubit fingerprinting of two-bit messages, we prepare `tetrahedral' qubit states experimentally and show that they meet the requirements for quantum fingerprinting to exceed the classical capability. We prove that shared entanglement permits 100% reliable quantum fingerprinting, which will outperform classical fingerprinting even with arbitrary amounts of shared randomness.Comment: 4 pages, one figur

Efficient single-photon emission from electrically driven InP quantum dots epitaxially grown on Si(001)

The heteroepitaxy of III-V semiconductors on silicon is a promising approach for making silicon a photonic platform for on-chip optical interconnects and quantum optical applications. Monolithic integration of both material systems is a long-time challenge, since different material properties lead to high defect densities in the epitaxial layers. In recent years, nanostructures however have shown to be suitable for successfully realising light emitters on silicon, taking advantage of their geometry. Facet edges and sidewalls can minimise or eliminate the formation of dislocations, and due to the reduced contact area, nanostructures are little affected by dislocation networks. Here we demonstrate the potential of indium phosphide quantum dots as efficient light emitters on CMOS-compatible silicon substrates, with luminescence characteristics comparable to mature devices realised on III-V substrates. For the first time, electrically driven single-photon emission on silicon is presented, meeting the wavelength range of silicon avalanche photo diodes' highest detection efficiency