22,836 research outputs found

    The Ionization Fraction in the DM Tau Protoplanetary Disk

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    We present millimeter-wave observations of several molecular ions in the disk around the pre-main-sequence star DM Tau and use these to investigate the ionization fraction in different regions of the disk. New Submillimeter Array (SMA) observations of H2D+ J=1_10 - 1_11, N2H+ J=4-3 and CO J=3-2 are presented. H2D+ and N2H+ are not detected and using the CO 3-2 disk size the observations result in an upper limit of <0.47 K km s-1 for both lines, a factor of 2.5 below previous single-dish H2D+ observations. Assuming LTE, a disk midplane temperature of 10-20 K and estimates of the H2D+ o/p ratio, the observed limit corresponds to NH2D+ < 4 - 21 \times 1012 cm-2. We adopt a parametric model for the disk structure from the literature and use new IRAM 30 meter telescope observations of the H13CO+ J=3-2 line and previously published SMA observations of the N2H+ J=3-2, HCO+ J=3-2 and DCO+ J=3-2 lines to constrain the ionization fraction, xi, in three temperature regions in the disk where theoretical considerations suggest different ions should dominate: (1) a warm, upper layer with T>20 K where CO is in the gas-phase and HCO+ is most abundant, where we estimate xi \simeq 4 \times 10-10, (2) a cooler molecular layer with T = 16-20 K where N2H+ and DCO+ abundances are predicted to peak, with xi \simeq 3\times10-11, and (3) the cold, dense midplane with T<16 K where H3+ and its deuterated isotopologues are the main carriers of positive charge, with xi < 3\times10-10. While there are considerable uncertainties, these estimates are consistent with a decreasing ionization fraction into the deeper, colder, and denser disk layers. Stronger constraints on the ionization fraction in the disk midplane will require not only substantially more sensitive observations of the H2D+ 1_10 - 1_11 line, but also robust determinations of the o/p ratio, observations of D2H+ and stronger constraints on where N2 is present in the gas phase.Comment: Accepted for publication in ApJ. 20 pages, including 5 figure

    Optically nonlinear energy transfer in light-harvesting dendrimers

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    Dendrimeric polymers are the subject of intense research activity geared towards their implementation in nanodevice applications such as energy harvesting systems,organic light-emitting diodes, photosensitizers, low-threshold lasers, and quantum logic elements, etc. A recent development in this area has been the construction of dendrimers specifically designed to exhibit novel forms of optical nonlinearity, exploiting the unique properties of these materials at high levels of photon flux. Starting from a thorough treatment of the underlying theory based on the principles of molecular quantum electrodynamics, it is possible to identify and characterize several optically nonlinear mechanisms for directed energy transfer and energy pooling in multichromophore dendrimers. Such mechanisms fall into two classes: first, those where two-photon absorption by individual donors is followed by transfer of the net energy to an acceptor; second, those where the excitation of two electronically distinct but neighboring donor groups is followed by a collective migration of their energy to a suitable acceptor. Each transfer process is subject to minor dissipative losses. In this paper we describe in detail the balance of factors and the constraints that determines the favored mechanism, which include the excitation statistics, structure of the energy levels, laser coherence factors, chromophore selection rules and architecture, possibilities for the formation of delocalized excitons, spectral overlap, and the overall distribution of donors and acceptors. Furthermore, it transpires that quantum interference between different mechanisms can play an important role. Thus, as the relative importance of each mechanism determines the relevant nanophotonic characteristics, the results reported here afford the means for optimizing highly efficient light-harvesting dendrimer devices

    Interparticle interactions:Energy potentials, energy transfer, and nanoscale mechanical motion in response to optical radiation

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    In the interactions between particles of material with slightly different electronic levels, unusually large shifts in the pair potential can result from photoexcitation, and on subsequent electronic excitation transfer. To elicit these phenomena, it is necessary to understand the fundamental differences between a variety of optical properties deriving from dispersion interactions, and processes such as resonance energy transfer that occur under laser irradiance. This helps dispel some confusion in the recent literature. By developing and interpreting the theory at a deeper level, one can anticipate that in suitable systems, light absorption and energy transfer will be accompanied by significant displacements in interparticle separation, leading to nanoscale mechanical motion

    Photon Distribution Function for Long-Distance Propagation of Partially Coherent Beams through the Turbulent Atmosphere

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    The photon density operator function is used to calculate light beam propagation through turbulent atmosphere. A kinetic equation for the photon distribution function is derived and solved using the method of characteristics. Optical wave correlations are described in terms of photon trajectories that depend on fluctuations of the refractive index. It is shown that both linear and quadratic disturbances produce sizable effects for long-distance propagation. The quadratic terms are shown to suppress the correlation of waves with different wave vectors. We examine the intensity fluctuations of partially coherent beams (beams whose initial spatial coherence is partially destroyed). Our calculations show that it is possible to significantly reduce the intensity fluctuations by using a partially coherent beam. The physical mechanism responsible for this pronounced reduction is similar to that of the Hanbury-Braun, Twiss effect.Comment: 28 pages, 4 figure

    A decade of ejecta dust formation in the Type IIn SN 2005ip

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    In order to understand the contribution of core-collapse supernovae to the dust budget of the early universe, it is important to understand not only the mass of dust that can form in core-collapse supernovae but also the location and rate of dust formation. SN 2005ip is of particular interest since dust has been inferred to have formed in both the ejecta and the post-shock region behind the radiative reverse shock. We have collated eight optical archival spectra that span the lifetime of SN 2005ip and we additionally present a new X-shooter optical-near-IR spectrum of SN 2005ip at 4075d post-discovery. Using the Monte Carlo line transfer code DAMOCLES, we have modelled the blueshifted broad and intermediate width Hα\alpha, Hβ\beta and He I lines from 48d to 4075d post-discovery using an ejecta dust model. We find that dust in the ejecta can account for the asymmetries observed in the broad and intermediate width Hα\alpha, Hβ\beta and He I line profiles at all epochs and that it is not necessary to invoke post-shock dust formation to explain the blueshifting observed in the intermediate width post-shock lines. Using a Bayesian approach, we have determined the evolution of the ejecta dust mass in SN 2005ip over 10 years presuming an ejecta dust model, with an increasing dust mass from ~108^{-8} M_{\odot} at 48d to a current dust mass of \sim0.1 M_{\odot}.Comment: Accepted by MNRAS, 17 pages, 11 figures. Author accepted manuscript. Accepted on 04/03/19. Deposited on 07/03/1
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