Interparticle interactions:Energy potentials, energy transfer, and nanoscale mechanical motion in response to optical radiation

In the interactions between particles of material with slightly different electronic levels, unusually large shifts in the pair potential can result from photoexcitation, and on subsequent electronic excitation transfer. To elicit these phenomena, it is necessary to understand the fundamental differences between a variety of optical properties deriving from dispersion interactions, and processes such as resonance energy transfer that occur under laser irradiance. This helps dispel some confusion in the recent literature. By developing and interpreting the theory at a deeper level, one can anticipate that in suitable systems, light absorption and energy transfer will be accompanied by significant displacements in interparticle separation, leading to nanoscale mechanical motion

Properties of Non-Abelian Fractional Quantum Hall States at Filling ν=kr\nu=\frac{k}{r}

We compute the physical properties of non-Abelian Fractional Quantum Hall (FQH) states described by Jack polynomials at general filling $\nu=\frac{k}{r}$. For $r=2$, these states are identical to the $Z_k$ Read-Rezayi parafermions, whereas for $r>2$ they represent new FQH states. The $r=k+1$ states, multiplied by a Vandermonde determinant, are a non-Abelian alternative construction of states at fermionic filling $2/5, 3/7, 4/9...$. We obtain the thermal Hall coefficient, the quantum dimensions, the electron scaling exponent, and show that the non-Abelian quasihole has a well-defined propagator falling off with the distance. The clustering properties of the Jack polynomials, provide a strong indication that the states with $r>2$ can be obtained as correlators of fields of \emph{non-unitary} conformal field theories, but the CFT-FQH connection fails when invoked to compute physical properties such as thermal Hall coefficient or, more importantly, the quasihole propagator. The quasihole wavefuntion, when written as a coherent state representation of Jack polynomials, has an identical structure for \emph{all} non-Abelian states at filling $\nu=\frac{k}{r}$.Comment: 2 figure

Sensitive imaging of electromagnetic fields with paramagnetic polar molecules

We propose a method for sensitive parallel detection of low-frequency electromagnetic fields based on the fine structure interactions in paramagnetic polar molecules. Compared to the recently implemented scheme employing ultracold $^{87}$Rb atoms [B{\"o}hi \textit{et al.}, Appl. Phys. Lett. \textbf{97}, 051101 (2010)], the technique based on molecules offers a 100-fold higher sensitivity, the possibility to measure both the electric and magnetic field components, and a probe of a wide range of frequencies from the dc limit to the THz regime

Equation of state for hard sphere fluids with and without Kac tails

In this note, we propose a simple derivation of the one dimensional hard rod equation of state, with and without a Kac tail (appended long range and weak potential). The case of hard spheres in higher dimension is also addressed and it is shown there that our arguments --which avoid any mathematical complication-- allow to recover the virial form of the equation of state in a direct way.Comment: pedagogical pape

Generalized Clustering Conditions of Jack Polynomials at Negative Jack Parameter α\alpha

We present several conjectures on the behavior and clustering properties of Jack polynomials at \emph{negative} parameter $\alpha=-\frac{k+1}{r-1}$, of partitions that violate the $(k,r,N)$ admissibility rule of Feigin \emph{et. al.} [\onlinecite{feigin2002}]. We find that "highest weight" Jack polynomials of specific partitions represent the minimum degree polynomials in $N$ variables that vanish when $s$ distinct clusters of $k+1$ particles are formed, with $s$ and $k$ positive integers. Explicit counting formulas are conjectured. The generalized clustering conditions are useful in a forthcoming description of fractional quantum Hall quasiparticles.Comment: 12 page

Laser-controlled fluorescence in two-level systems

The ability to modify the character of fluorescent emission by a laser-controlled, optically nonlinear process has recently been shown theoretically feasible, and several possible applications have already been identified. In operation, a pulse of off-resonant probe laser beam, of sufficient intensity, is applied to a system exhibiting fluorescence, during the interval of excited- state decay following the initial excitation. The result is a rate of decay that can be controllably modified, the associated changes in fluorescence behavior affording new, chemically specific information. In this paper, a two-level emission model is employed in the further analysis of this all-optical process; the results should prove especially relevant to the analysis and imaging of physical systems employing fluorescent markers, these ranging from quantum dots to green fluorescence protein. Expressions are presented for the laser-controlled fluorescence anisotropy exhibited by samples in which the fluorophores are randomly oriented. It is also shown that, in systems with suitably configured electronic levels and symmetry properties, fluorescence emission can be produced from energy levels that would normally decay nonradiatively. © 2010 American Chemical Society

Steady-state MreB helices inside bacteria: dynamics without motors

Within individual bacteria, we combine force-dependent polymerization dynamics of individual MreB protofilaments with an elastic model of protofilament bundles buckled into helical configurations. We use variational techniques and stochastic simulations to relate the pitch of the MreB helix, the total abundance of MreB, and the number of protofilaments. By comparing our simulations with mean-field calculations, we find that stochastic fluctuations are significant. We examine the quasi-static evolution of the helical pitch with cell growth, as well as timescales of helix turnover and denovo establishment. We find that while the body of a polarized MreB helix treadmills towards its slow-growing end, the fast-growing tips of laterally associated protofilaments move towards the opposite fast-growing end of the MreB helix. This offers a possible mechanism for targeted polar localization without cytoplasmic motor proteins.Comment: 7 figures, 1 tabl

Resonance energy transfer: The unified theory revisited

Resonanceenergy transfer (RET) is the principal mechanism for the intermolecular or intramolecular redistribution of electronic energy following molecular excitation. In terms of fundamental quantum interactions, the process is properly described in terms of a virtual photon transit between the pre-excited donor and a lower energy (usually ground-state) acceptor. The detailed quantum amplitude for RET is calculated by molecular quantum electrodynamical techniques with the observable, the transfer rate, derived via application of the Fermi golden rule. In the treatment reported here, recently devised state-sequence techniques and a novel calculational protocol is applied to RET and shown to circumvent problems associated with the usual method. The second-rank tensor describing virtual photon behavior evolves from a Green’s function solution to the Helmholtz equation, and special functions are employed to realize the coupling tensor. The method is used to derive a new result for energy transfer systems sensitive to both magnetic- and electric-dipole transitions. The ensuing result is compared to that of pure electric-dipole–electric-dipole coupling and is analyzed with regard to acceptable transfer separations. Systems are proposed where the electric-dipole–magnetic-dipole term is the leading contribution to the overall rate