Combined neutron reflectometry and rheology

We have combined neutron reflectometry with rheology in order to investigate the solid boundary of liquids and polymers under shear deformation. Our approach allows one to apply a controlled stress to a material while resolving the structural arrangements on the sub nanometer length scale with neutron reflectivity, off-specular and small angle scattering at the same time. The specularly reflected neutron intensity of a 20 % by weight solution of the Pluronic F127 in deuterated water is evaluated. We find pronounced changes in the near interface structure under applied deformation for surfaces with different surface energies, which are correlated with changes in the storage and loss modulus

Recent developments of MCViNE and its applications at SNS

MCViNE is an open source, object-oriented Monte Carlo neutron ray-tracing simulation software package. Its design allows for flexible, hierarchical representations of sophisticated instrument components such as detector systems, and samples with a variety of shapes and scattering kernels. Recently this flexible design has enabled several applications of MCViNE simulations at the Spallation Neutron Source (SNS) at Oak Ridge National Lab, including assisting design of neutron instruments at the second target station and design of novel sample environments, as well as studying effects of instrument resolution and multiple scattering. Here we provide an overview of the recent developments and new features of MCViNE since its initial introduction (Jiao et al 2016 Nucl. Instrum. Methods Phys. Res., Sect. A 810, 86–99), and some example applications

Correlation between microstructure and magnetotransport in organic semiconductor spin valve structures

We have studied magnetotransport in organic-inorganic hybrid multilayer junctions. In these devices, the organic semiconductor (OSC) Alq$_3$ (tris(8-hydroxyquinoline) aluminum) formed a spacer layer between ferromagnetic (FM) Co and Fe layers. The thickness of the Alq$_3$ layer was in the range of 50-150 nm. Positive magnetoresistance (MR) was observed at 4.2 K in a current perpendicular to plane geometry, and these effects persisted up to room temperature. The devices' microstructure was studied by X-ray reflectometry, Auger electron spectroscopy and polarized neutron reflectometry (PNR). The films show well-defined layers with modest average chemical roughness (3-5 nm) at the interface between the Alq$_3$ and the surrounding FM layers. Reflectometry shows that larger MR effects are associated with smaller FM/Alq$_3$ interface width (both chemical and magnetic) and a magnetically dead layer at the Alq$_3$/Fe interface. The PNR data also show that the Co layer, which was deposited on top of the Alq$_3$, adopts a multi-domain magnetic structure at low field and a perfect anti-parallel state is not obtained. The origins of the observed MR are discussed and attributed to spin coherent transport. A lower bound for the spin diffusion length in Alq$_3$ was estimated as $43 \pm 5$ nm at 80 K. However, the subtle correlations between microstructure and magnetotransport indicate the importance of interfacial effects in these systems.Comment: 21 pages, 11 figures and 2 table

Spin-polarized neutron reflectivity: A probe of vortices in thin-film superconductors

URL:http://link.aps.org/doi/10.1103/PhysRevB.59.14692 DOI:10.1103/PhysRevB.59.14692It is demonstrated that the specular reflectivity of spin-polarized neutrons can be used to study vortices in a thin-film superconductor. Experiments were performed on a 6000 Å thick c-axis film of YBa2Cu3O7-x with the magnetic field applied parallel to the surface. A magnetic hysteresis loop was observed for the spin-polarized reflection and, from these data, the average density of vortices was extracted. A model is presented which relates the specular reflectivity to the one-dimensional spatial distribution of vortices in the direction perpendicular to the surface. Unlike other techniques, neutron reflectivity observes vortices in a geometry where they are parallel to the interface.Support ~P.F.M., S.W.H.! from the Midwest Superconductivity Consortium ~MISCON! under the U.S. DOE Grant No. DE-FG02-90ER45427, the NSF DMR Grant No. 96-23827, and ~L.H.G., E.P.! from the NSF DMR Grant No. 94-21957, and ONR Grant No. N-00014-95-1-0831 is gratefully acknowledged. We thank E. Fullerton for useful discussions and D.H. Lowndes for help in understanding the surface roughness of oxide superconductors

Ferromagnetic Domain Distribution in Thin Films During Magnetization Reversal

We have shown that polarized neutron reflectometry can determine in a model-free way not only the mean magnetization of a ferromagnetic thin film at any point of a hysteresis cycle, but also the mean square dispersion of the magnetization vectors of its lateral domains. This technique is applied to elucidate the mechanism of the magnetization reversal of an exchange-biased Co/CoO bilayer. The reversal process above the blocking temperature is governed by uniaxial domain switching, while below the blocking temperature the reversal of magnetization for the trained sample takes place with substantial domain rotation

Annealing-Dependent Magnetic Depth Profile in Ga[1-x]Mn[x]As

We have studied the depth-dependent magnetic and structural properties of as-grown and optimally annealed Ga[1-x]Mn[x]As films using polarized neutron reflectometry. In addition to increasing total magnetization, the annealing process was observed to produce a significantly more homogeneous distribution of the magnetization. This difference in the films is attributed to the redistribution of Mn at interstitial sites during the annealing process. Also, we have seen evidence of significant magnetization depletion at the surface of both as-grown and annealed films.Comment: 5 pages, 3 figure

Wavelet Inverse Neutron Scattering Study of Layered Metallic NiC-Ti Composites

Composites are prevalent in high technology devices such as aircraft, computers, automobiles and communications systems. They improve brittleness and provide a lower density which enhances mechanical strength. Electron and light manipulating composites will be used more and more in the future. It is necessary to have a capability of inspecting composites, both to assure production quality and as a baseline for later NDE. In this paper, we present a study using wavelet, inverse neutron optics and the grazing angle neutron spectrometer, GANS, at the Missouri University Research Reactor, MURR

An EDSL approach to high performance Haskell programming

This paper argues for a new methodology for writing high per-formance Haskell programs by using Embedded Domain Specific Languages. We exemplify the methodology by describing a complete li-brary, meta-repa, which is a reimplementation of parts of the repa library. The paper describes the implementation of meta-repa and contrasts it with the standard approach to writing high performance libraries. We conclude that even though the embedded language approach has an initial cost of defining the language and some syntactic overhead it gives a more tailored programming model, stronger performance guarantees, better control over optimizations, simpler implementation of fusion and inlining and allows for mov-ing type level programming down to value level programming in some cases. We also provide benchmarks showing that meta-repa is as fast, or faster, than repa. Furthermore, meta-repa also includes push arrays and we demonstrate their usefulness for writing certain high performance kernels such as FFT

Dynamic Masking Rate Schedules for MLM Pretraining

Most works on transformers trained with the Masked Language Modeling (MLM) objective use the original BERT model's fixed masking rate of 15%. Our work instead dynamically schedules the masking ratio throughout training. We found that linearly decreasing the masking rate from 30% to 15% over the course of pretraining improves average GLUE accuracy by 0.46% in BERT-base, compared to a standard 15% fixed rate. Further analyses demonstrate that the gains from scheduling come from being exposed to both high and low masking rate regimes. Our results demonstrate that masking rate scheduling is a simple way to improve the quality of masked language models and achieve up to a 1.89x speedup in pretraining