4,088 research outputs found

    Diffusion-Limited One-Species Reactions in the Bethe Lattice

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    We study the kinetics of diffusion-limited coalescence, A+A-->A, and annihilation, A+A-->0, in the Bethe lattice of coordination number z. Correlations build up over time so that the probability to find a particle next to another varies from \rho^2 (\rho is the particle density), initially, when the particles are uncorrelated, to [(z-2)/z]\rho^2, in the long-time asymptotic limit. As a result, the particle density decays inversely proportional to time, \rho ~ 1/kt, but at a rate k that slowly decreases to an asymptotic constant value.Comment: To be published in JPCM, special issue on Kinetics of Chemical Reaction

    Exact mean first-passage time on the T-graph

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    We consider a simple random walk on the T-fractal and we calculate the exact mean time τg\tau^g to first reach the central node i0i_0. The mean is performed over the set of possible walks from a given origin and over the set of starting points uniformly distributed throughout the sites of the graph, except i0i_0. By means of analytic techniques based on decimation procedures, we find the explicit expression for τg\tau^g as a function of the generation gg and of the volume VV of the underlying fractal. Our results agree with the asymptotic ones already known for diffusion on the T-fractal and, more generally, they are consistent with the standard laws describing diffusion on low-dimensional structures.Comment: 6 page

    Facilitated diffusion of proteins on chromatin

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    We present a theoretical model of facilitated diffusion of proteins in the cell nucleus. This model, which takes into account the successive binding/unbinding events of proteins to DNA, relies on a fractal description of the chromatin which has been recently evidenced experimentally. Facilitated diffusion is shown quantitatively to be favorable for a fast localization of a target locus by a transcription factor, and even to enable the minimization of the search time by tuning the affinity of the transcription factor with DNA. This study shows the robustness of the facilitated diffusion mechanism, invoked so far only for linear conformations of DNA.Comment: 4 pages, 4 figures, accepted versio

    Probing Non-Integer Dimensions

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    We show that two-dimensional convection-diffusion problems with a radial sink or source at the origin may be recast as a pure diffusion problem in a fictitious space in which the spatial dimension is continuously-tunable with the Peclet number. This formulation allows us to probe various diffusion-controlled processes in non-integer dimensions.Comment: 6 pages, 2 column-revtex4 format. Submitted to special issue of Journal of Physics: Condensed Matter, on "Chemical Kinetics Beyond the Textbook: Fluctuations, Many-Particle Effects and Anomalous Dynamics", eds. K. Lindenberg, G. Oshanin, & M. Tachiy

    Quantum phase transitions, frustration, and the Fermi surface in the Kondo lattice model

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    The quantum phase transition from a spin-Peierls phase with a small Fermi surface to a paramagnetic Luttinger-liquid phase with a large Fermi surface is studied in the framework of a one-dimensional Kondo-Heisenberg model that consists of an electron gas away from half filling, coupled to a spin-1/2 chain by Kondo interactions. The Kondo spins are further coupled to each other with isotropic nearest-neighbor and next-nearest-neighbor antiferromagnetic Heisenberg interactions which are tuned to the Majumdar-Ghosh point. Focusing on three-eighths filling and using the density-matrix renormalization-group (DMRG) method, we show that the zero-temperature transition between the phases with small and large Fermi momenta appears continuous, and involves a new intermediate phase where the Fermi surface is not well defined. The intermediate phase is spin gapped and has Kondo-spin correlations that show incommensurate modulations. Our results appear incompatible with the local picture for the quantum phase transition in heavy fermion compounds, which predicts an abrupt change in the size of the Fermi momentum.Comment: 9 pages, 8 figure

    Two-Species Annihilation with Drift: A Model with Continuous Concentration-Decay Exponents

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    We propose a model for diffusion-limited annihilation of two species, A+BAA+B\to A or BB, where the motion of the particles is subject to a drift. For equal initial concentrations of the two species, the density follows a power-law decay for large times. However, the decay exponent varies continuously as a function of the probability of which particle, the hopping one or the target, survives in the reaction. These results suggest that diffusion-limited reactions subject to drift do not fall into a limited number of universality classes.Comment: 10 pages, tex, 3 figures, also available upon reques

    Exact calculations of first-passage quantities on recursive networks

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    We present general methods to exactly calculate mean-first passage quantities on self-similar networks defined recursively. In particular, we calculate the mean first-passage time and the splitting probabilities associated to a source and one or several targets; averaged quantities over a given set of sources (e.g., same-connectivity nodes) are also derived. The exact estimate of such quantities highlights the dependency of first-passage processes with respect to the source-target distance, which has recently revealed to be a key parameter to characterize transport in complex media. We explicitly perform calculations for different classes of recursive networks (finitely ramified fractals, scale-free (trans)fractals, non-fractals, mixtures between fractals and non-fractals, non-decimable hierarchical graphs) of arbitrary size. Our approach unifies and significantly extends the available results in the field.Comment: 16 pages, 10 figure
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