Laser radiation pressure slowing of a molecular beam

There is substantial interest in producing samples of ultracold molecules for possible applications in quantum computation, quantum simulation of condensed matter systems, precision measurements, controlled chemistry, and high precision spectroscopy. A crucial step to obtaining large samples of ultracold, trapped molecules is developing a means to bridge the gap between typical molecular source velocities (~150-600 m/s) and velocities for which trap loading or confinement is possible (~5-20 m/s). Here we show deceleration of a beam of neutral strontium monofluoride (SrF) molecules using radiative force. Under certain conditions, the deceleration results in a substantial flux of molecules with velocities <50 m/s. The observed slowing, from ~140 m/s, corresponds to scattering ~10000 photons. We also observe longitudinal velocity compression under different conditions. Combined with molecular laser cooling techniques, this lays the groundwork to create slow and cold molecular beams suitable for trap loading.Comment: 7 pages, 7 figures. Supplementary material updated

Scaling by 5 on a 1/4-Cantor Measure

Each Cantor measure (\mu) with scaling factor 1/(2n) has at least one associated orthonormal basis of exponential functions (ONB) for L^2(\mu). In the particular case where the scaling constant for the Cantor measure is 1/4 and two specific ONBs are selected for L^2(\mu), there is a unitary operator U defined by mapping one ONB to the other. This paper focuses on the case in which one ONB (\Gamma) is the original Jorgensen-Pedersen ONB for the Cantor measure (\mu) and the other ONB is is 5\Gamma. The main theorem of the paper states that the corresponding operator U is ergodic in the sense that only the constant functions are fixed by U.Comment: 34 page

Franck-Condon Factors and Radiative Lifetime of the A^{2}\Pi_{1/2} - X^{2}\Sigma^{+} Transition of Ytterbium Monoflouride, YbF

The fluorescence spectrum resulting from laser excitation of the A^{2}\Pi_{1/2} - X^{2}\Sigma^{+} (0,0) band of ytterbium monofluoride, YbF, has been recorded and analyzed to determine the Franck-Condon factors. The measured values are compared with those predicted from Rydberg-Klein-Rees (RKR) potential energy curves. From the fluorescence decay curve the radiative lifetime of the A^{2}\Pi_{1/2} state is measured to be 28\pm2 ns, and the corresponding transition dipole moment is 4.39\pm0.16 D. The implications for laser cooling YbF are discussed.Comment: 5 pages, 5 figure

Centennial-to-millennial hydrologic trends and variability along the North Atlantic Coast, USA, during the Holocene

Author Posting. © American Geophysical Union, 2014. This article is posted here by permission of American Geophysical Union for personal use, not for redistribution. The definitive version was published in Geophysical Research Letters 41 (2014): 4300–4307, doi:10.1002/2014GL060183.Geophysical and sedimentary records from five lakes in Massachusetts reveal regionally coherent hydrologic variability during the Holocene. All of the lakes have risen since ~9.0 ka, but multicentury droughts after 5.6 ka repeatedly lowered their water levels. Quantified water level histories from the three best-studied lakes share >70% of their reconstructed variance. Four prominent low-water phases at 4.9–4.6, 4.2–3.9, 2.9–2.1, and 1.3–1.2 ka were synchronous across coastal lakes, even after accounting for age uncertainties. The droughts also affected sites up to ~200 km inland, but water level changes at 5.6–4.9 ka appear out of phase between inland and coastal lakes. During the enhanced multicentury variability after ~5.6 ka, droughts coincided with cooling in Greenland and may indicate circulation changes across the North Atlantic region. Overall, the records demonstrate that current water levels are exceptionally high and confirm the sensitivity of water resources in the northeast U.S. to climate change.The National Science Foundation (EAR-0602408, EAR- 1036191, and DEB-0816731 to Shuman; EAR-0602380 to Donnelly) and the Woods Hole Oceanographic Institution, Ocean and Climate Change Institute (Donnelly) funded this research.2014-12-2

Stark deceleration of CaF molecules in strong- and weak-field seeking states

We report the Stark deceleration of CaF molecules in the strong-field seeking ground state and in a weak-field seeking component of a rotationally-excited state. We use two types of decelerator, a conventional Stark decelerator for the weak-field seekers, and an alternating gradient decelerator for the strong-field seekers, and we compare their relative merits. We also consider the application of laser cooling to increase the phase-space density of decelerated molecules.Comment: 10 pages, 8 figure

VUV frequency combs from below-threshold harmonics

Recent demonstrations of high-harmonic generation (HHG) at very high repetition frequencies (~100 MHz) may allow for the revolutionary transfer of frequency combs to the vacuum ultraviolet (VUV). This advance necessitates unifying optical frequency comb technology with strong-field atomic physics. While strong-field studies of HHG have often focused on above-threshold harmonic generation (photon energy above the ionization potential), for VUV frequency combs an understanding of below-threshold harmonic orders and their generation process is crucial. Here we present a new and quantitative study of the harmonics 7-13 generated below and near the ionization threshold in xenon gas. We show multiple generation pathways for these harmonics that are manifested as on-axis interference in the harmonic yield. This discovery provides a new understanding of the strong-field, below-threshold dynamics under the influence of an atomic potential and allows us to quantitatively assess the achievable coherence of a VUV frequency comb generated through below threshold harmonics. We find that under reasonable experimental conditions temporal coherence is maintained. As evidence we present the first explicit VUV frequency comb structure beyond the 3rd harmonic.Comment: 16 pages, 4 figures, 1 tabl

Deceleration and trapping of heavy diatomic molecules using a ring-decelerator

We present an analysis of the deceleration and trapping of heavy diatomic molecules in low-field seeking states by a moving electric potential. This moving potential is created by a 'ring-decelerator', which consists of a series of ring-shaped electrodes to which oscillating high voltages are applied. Particle trajectory simulations have been used to analyze the deceleration and trapping efficiency for a group of molecules that is of special interest for precision measurements of fundamental discrete symmetries. For the typical case of the SrF molecule in the (N,M) = (2, 0) state, the ring-decelerator is shown to outperform traditional and alternate-gradient Stark decelerators by at least an order of magnitude. If further cooled by a stage of laser cooling, the decelerated molecules allow for a sensitivity gain in a parity violation measurement, compared to a cryogenic molecular beam experiment, of almost two orders of magnitude

Large-Area Silicon Detectors for the Advanced Composition Explorer (ACE) Solar Isotope Spectrometer (SIS)

Extensive measurements were made of the thicknesses and dead-layers of the large-area, highpurity silicon detectors used for the Solar Isotope Spectrometer (SIS), an instrument to be launched on the Advanced Composition Explorer (ACE) spacecraft. Tests using accelerated beams of heavy nuclei were also carried out to characterize the completed instrument