847 research outputs found

    Enhanced electron correlations in FeSb2_2

    Full text link
    FeSb2_2 has been recently identified as a new model system for studying many-body renormalizations in a dd-electron based narrow gap semiconducting system, strongly resembling FeSi. The electron-electron correlations in FeSb2_2 manifest themselves in a wide variety of physical properties including electrical and thermal transport, optical conductivity, magnetic susceptibility, specific heat and so on. We review some of the properties that form a set of experimental evidences revealing the crucial role of correlation effects in FeSb2_2. The metallic state derived from slight Te doping in FeSb2_2, which has large quasiparticle mass, will also be introduced.Comment: 9 pages, 7 figures; submitted to Annalen der Physi

    Unchanged thermopower enhancement at the semiconductor-metal transition in correlated FeSb2x_{2-x}Tex_x

    Full text link
    Substitution of Sb in FeSb2_2 by less than 0.5% of Te induces a transition from a correlated semiconductor to an unconventional metal with large effective charge carrier mass mm^*. Spanning the entire range of the semiconductor-metal crossover, we observed an almost constant enhancement of the measured thermopower compared to that estimated by the classical theory of electron diffusion. Using the latter for a quantitative description one has to employ an enhancement factor of 10-30. Our observations point to the importance of electron-electron correlations in the thermal transport of FeSb2_2, and suggest a route to design thermoelectric materials for cryogenic applications.Comment: 3 pages, 3 figures, accepted for publication in Appl. Phys. Lett. (2011

    Highly Dispersive Electron Relaxation and Colossal Thermoelectricity in the Correlated Semiconductor FeSb2_2

    Full text link
    We show that the colossal thermoelectric power, S(T)S(T), observed in the correlated semiconductor FeSb2_2 below 30\,K is accompanied by a huge Nernst coefficient ν(T)\nu(T) and magnetoresistance MR(T)(T). Markedly, the latter two quantities are enhanced in a strikingly similar manner. While in the same temperature range, S(T)S(T) of the reference compound FeAs2_2, which has a seven-times larger energy gap, amounts to nearly half of that of FeSb2_2, its ν(T)\nu(T) and MR(T)(T) are intrinsically different to FeSb2_2: they are smaller by two orders of magnitude and have no common features. With the charge transport of FeAs2_2 successfully captured by the density functional theory, we emphasize a significantly dispersive electron-relaxation time τ(ϵk)\tau(\epsilon_k) due to electron-electron correlations to be at the heart of the peculiar thermoelectricity and magnetoresistance of FeSb2_2.Comment: 8 pages, 5 figure

    Vortex avalanches in the non-centrosymmetric superconductor Li2Pt3B

    Full text link
    We investigated the vortex dynamics in the non-centrosymmetric superconductor Li_2Pt_3B in the temperature range 0.1 K - 2.8 K. Two different logarithmic creep regimes in the decay of the remanent magnetization from the Bean critical state have been observed. In the first regime, the creep rate is extraordinarily small, indicating the existence of a new, very effective pinning mechanism. At a certain time a vortex avalanche occurs that increases the logarithmic creep rate by a factor of about 5 to 10 depending on the temperature. This may indicate that certain barriers against flux motion are present and they can be opened under increased pressure exerted by the vortices. A possible mechanism based on the barrier effect of twin boundaries is briefly discussed

    A precursor state to unconventional superconductivity in CeIrIn5{_5}

    Full text link
    We present sensitive measurements of the Hall effect and magnetoresistance in CeIrIn5{_5} down to temperatures of 50 mK and magnetic fields up to 15 T. The presence of a low temperature coherent Kondo state is established. Deviations from Kohler's rule and a quadratic temperature dependence of the cotangent of the Hall angle are reminiscent of properties observed in the high temperature superconducting cuprates. The most striking observation pertains to the presence of a \textit{precursor} state--characterized by a change in the Hall mobility--that appears to precede the superconductivity in this material, in similarity to the pseudogap in the cuprate high TcT_c superconductors.Comment: 4 figure

    Polaronic state and nanometer-scale phase separation in colossal magnetoresistive manganites

    Full text link
    High resolution topographic images obtained by scanning tunneling microscope in the insulating state of Pr0.68Pb0.32MnO3 single crystals showed regular stripe-like or zigzag patterns on a width scale of 0.4 - 0.5 nm confirming a high temperature polaronic state. Spectroscopic studies revealed inhomogeneous maps of zero-bias conductance with small patches of metallic clusters on length scale of 2 - 3 nm only within a narrow temperature range close to the metal-insulator transition. The results give a direct observation of polarons in the insulating state, phase separation of nanometer-scale metallic clusters in the paramagnetic metallic state, and a homogeneous ferromagnetic state

    Kondo effect in Ce(x)La(1-x)Cu(2.05)Si(2) intermetallics

    Full text link
    The magnetic susceptibility and susceptibility anisotropy of the quasi-binary alloy system Ce(x)La(1-x)Cu(2.05)Si(2) have been studied for low concentration of Ce ions. The single-ion desc ription is found to be valid for x < 0.1. The experimental results are discussed in terms of t he degenerate Coqblin-Schrieffer model with a crystalline electric field splitting Delta = 330 K. The properties of the model, obtained by combining the lowest-order scaling and the pertur bation theory, provide a satisfactory description of the experimental data down to 30 K. The e xperimental results between 20 K and 2 K are explained by the exact solution of the Kondo mode l for an effective doublet.Comment: 11 pages, 13 Postscript figures, 1 tabl

    Investigation of the Spin-Peierls transition in CuGeO_3 by Raman scattering

    Full text link
    Raman experiments on the spin-Peierls compound CuGeO3_3 and the substituted (Cu1x_{1- x},Znx_x)GeO3_3 and Cu(Ge1x_{1-x},Gax_x)O3_3 compounds were performed in order to investigate the response of specific magnetic excitations of the one-dimensional spin-1/2 chain to spin anisotropies and substitution-induced disorder. In pure CuGeO3_3, in addition to normal phonon scattering which is not affected at all by the spin-Peierls transition, four types of magnetic scattering features were observed. Below TSP_{SP}=14 K a singlet-triplet excitation at 30 cm1^{-1}, two-magnon scattering from 30 to 227 cm1^{-1} and folded phonon modes at 369 and 819 cm1^{-1} were identified. They were assigned by their temperature dependence and lineshape. For temperatures between the spin-Peierls transition TSP_{SP} and approximately 100 K a broad intensity maximum centered at 300 cm1^{-1} is observed.Comment: 7 pages, LaTex2e, including 3 figures (eps) to be published in Physica B (1996
    corecore