On the dispersion management of fluorite whispering-gallery mode resonators for Kerr optical frequency comb generation in the telecom and mid-infrared range

Optical whispering gallery mode (WGM) resonators have been very attracting platforms for versatile Kerr frequency comb generations. We report a systematic study on the material dispersion of various optical materials that are capable of supporting quality factors above $10^9$. Using an analytical approximation of WGM resonant frequencies in disk resonators, we investigate the effect of the geometry and transverse mode order on the total group-velocity dispersion ($GVD$). We demonstrate that the major radii and the radial mode indices play an important role in tailoring the $GVD$ of WGM resonators. In particular, our study shows that in WGM disk-resonators, the polar families of modes have very similar $GVD$, while the radial families of modes feature dispersion values that can differ by up to several orders of magnitude. The effect of these giant dispersion shifts are experimentally evidenced in Kerr comb generation with magnesium fluoride. From a more general perspective, this critical feature enables to push the zero-dispersion wavelength of fluorite crystals towards the mid-infrared (mid-IR) range, thereby allowing for efficient Kerr comb generation in that spectral range. We show that barium fluoride is the most interesting crystal in this regard, due to its zero dispersion wavelength ($ZDW$) at $1.93 \rm{\mu m}$ and an optimal dispersion profile in the mid-IR regime. We expect our results to facilitate the design of different platforms for Kerr frequency comb generations in both telecommunication and mid-IR spectral ranges

Routes to spatiotemporal chaos in Kerr optical frequency combs

We investigate the various routes to spatiotemporal chaos in Kerr optical frequency combs obtained through pumping an ultra-high quality whispering-gallery mode resonator with a continuous-wave laser. The Lugiato-Lefever model is used to build bifurcation diagrams with regards to the parameters that are externally controllable, namely, the frequency and the power of the pumping laser. We show that the spatiotemporal chaos emerging from Turing patterns and solitons display distinctive dynamical features. Experimental spectra of chaotic Kerr combs are also presented for both cases, in excellent agreement with theoretical spectra

Quantum Dynamics of Kerr Optical Frequency Combs below and above Threshold: Spontaneous Four-Wave-Mixing, Entanglement and Squeezed States of Light

In this article, we use quantum Langevin equations to provide a theoretical understanding of the non-classical behavior of Kerr optical frequency combs when pumped below and above threshold. In the configuration where the system is under threshold, the pump field is the unique oscillating mode inside the resonator, and triggers the phenomenon of spontaneous four-wave mixing, where two photons from the pump are symmetrically up- and down-converted in the Fourier domain. This phenomenon can only be understood and analyzed from a fully quantum perspective as a consequence of the coupling between the field of the central (pumped) mode and the vacuum fluctuations of the various sidemodes. We analytically calculate the power spectra of the spontaneous emission noise, and we show that these spectra can be either single- or double peaked depending on the parameters of the system. We also calculate as well the overall spontaneous noise power per sidemode, and propose simplified analytical expressions for some particular cases. In the configuration where the system is pumped above threshold, we investigate the phenomena of quantum correlations and multimode squeezed states of light that can occur in the Kerr frequency combs originating from stimulated four-wave mixing. We show that for all stationary spatio-temporal patterns, the side-modes that are symmetrical relatively to the pumped mode in the frequency domain display quantum correlations that can lead to squeezed states of light. We also explicitly determine the phase quadratures leading to photon entanglement, and analytically calculate their quantum noise spectra. We finally discuss the relevance of Kerr combs for quantum information systems at optical telecommunication wavelengths, below and above threshold.Comment: 27 pages, 11 figure

Spatiotemporal Model for Kerr Comb Generation in Whispering Gallery Mode Resonators

We establish an exact partial differential equation to model Kerr comb generation in whispering-gallery mode resonators. This equation is a variant of the Lugiato-Lefever equation that includes higher-order dispersion and nonlinearity. This spatio-temporal model, whose main variable is the total intracavity field, is significantly more suitable than the modal expansion approach for the theoretical understanding and the numerical simulation of wide-span combs. It allows us to explore pulse formation in which a large number of modes interact cooperatively. This versatile approach can be straightforwardly extended to include higher-order dispersion, as well as other phenomena like Raman, Brillouin and Rayleigh scattering. We demonstrate for the first time that when the dispersion is anomalous, Kerr comb generation can arise as the spectral signature of dissipative cavity solitons, leading to wide-span combs with low pumping.Comment: 5 pages, 2 figure

Stability Analysis of the Lugiato-Lefever Model for Kerr Optical Frequency Combs. Part I: Case of Normal Dispersion

We propose a detailed stability analysis of the Lugiato-Lefever model for Kerr optical frequency combs in whispering gallery mode resonators pumped in the normal dispersion regime. We analyze the spatial bifurcation structure of the stationary states depending on two parameters that are experimentally tunable, namely the pump power and the cavity detuning. Our study demonstrates that the non-trivial equilibria play an important role in this bifurcation map, as their associated eigenvalues undergo critical bifurcations that are foreshadowing the existence of localized spatial structures. In particular, we show that in the normal dispersion regime, dark cavity solitons can emerge in the system, and thereby generate a Kerr comb. We also show how these solitons can coexist in the resonator as long as they do not interact with each other. The Kerr combs created by these (sets of) dark solitons are also analyzed, and their stability is discussed as well.Comment: 11 pages, 9 figures, 1 tabl

Barium fluoride whispering-gallery-mode disk-resonator with one billion quality-factor

We demonstrate a monolithic optical whispering gallery mode resonator fabricated with barium fluoride (BaF$_2$) with an ultra-high quality ($Q$) factor above $10^9$ at $1550$ nm, and measured with both the linewidth and cavity-ring-down methods. Vertical scanning optical profilometry shows that the root mean square surface roughness of $2$ nm is achieved for our mm-size disk. To the best of our knowledge, we show for the first time that one billion $Q$-factor is achievable by precision polishing in relatively soft crystals with mohs hardness of ~$3$. We show that complex thermo-optical dynamics can take place in these resonators. Beside usual applications in nonlinear optics and microwave photonics, high energy particle scintillation detection utilizing monolithic BaF$_2$ resonators potentially becomes feasible

Observation of Spatiotemporal Chaos Induced by a Cavity Soliton in a Fiber Ring Resonator

We report on the experimental observation of temporal cavity soliton destabilization via spatiotemporal chaos in a coherently-driven optical fiber ring resonator. Numerical simulations and theoretical analyses are in good agreement with experimental observations.Comment: Submitted to CLEO US on 27/01/201