Experimental Tomographic State Reconstruction of Itinerant Microwave Photons

A wide range of experiments studying microwave photons localized in superconducting cavities have made important contributions to our understanding of the quantum properties of radiation. Propagating microwave photons, however, have so far been studied much less intensely. Here we present measurements in which we reconstruct the Wigner function of itinerant single photon Fock states and their superposition with the vacuum using linear amplifiers and quadrature amplitude detectors. We have developed efficient methods to separate the detected single photon signal from the noise added by the amplifier by analyzing the moments of the measured amplitude distribution up to 4th order. This work is expected to enable studies of propagating microwaves in the context of linear quantum optics.Comment: 4 pages, 4 figure

Photon State Tomography for Two-Mode Correlated Itinerant Microwave Fields

Continuous variable entanglement between two modes of a radiation field is usually studied at optical frequencies. As an important step towards the observation of entanglement between propagating microwave photons we demonstrate the experimental state reconstruction of two field modes in the microwave domain. In particular, we generate two-mode correlated states with a Josephson parametric amplifier and detect all four quadrature components simultaneously in a two-channel heterodyne setup using amplitude detectors. Analyzing two-dimensional phase space histograms for all possible pairs of quadratures allows us to determine the full covariance matrix and reconstruct the four-dimensional Wigner function. We demonstrate strong correlations between the quadrature amplitude noise in the two modes. Under ideal conditions two-mode squeezing below the standard quantum limit should be observable in future experiments.Comment: 4 pages, 4 figure

Characterizing Quantum Microwave Radiation and its Entanglement with Superconducting Qubits using Linear Detectors

Recent progress in the development of superconducting circuits has enabled the realization of interesting sources of nonclassical radiation at microwave frequencies. Here, we discuss field quadrature detection schemes for the experimental characterization of itinerant microwave photon fields and their entanglement correlations with stationary qubits. In particular, we present joint state tomography methods of a radiation field mode and a two-level system. Including the case of finite quantum detection efficiency, we relate measured photon field statistics to generalized quasi-probability distributions and statistical moments for one-channel and two-channel detection. We also present maximum-likelihood methods to reconstruct density matrices from measured field quadrature histograms. Our theoretical investigations are supported by the presentation of experimental data, for which microwave quantum fields beyond the single-photon and Gaussian level have been prepared and reconstructed.Comment: 14 pages, 5 figure

Optical tomography of Fock state superpositions

We consider optical tomography of photon Fock state superpositions in connection with recent experimental achievements. The emphasis is put on the fact that it suffices to represent the measured tomogram as a main result of the experiment. We suggest a test for checking the correctness of experimental data. Explicit expressions for optical tomograms of Fock state superpositions are given in terms of Hermite polynomials. Particular cases of vacuum and low photon-number state superposition are considered as well as influence of thermal noise on state purity is studied.Comment: 5 pages, 2 figure

Observation of squeezed light from one atom excited with two photons

Single quantum emitters like atoms are well-known as non-classical light sources which can produce photons one by one at given times, with reduced intensity noise. However, the light field emitted by a single atom can exhibit much richer dynamics. A prominent example is the predicted ability for a single atom to produce quadrature-squeezed light, with sub-shot-noise amplitude or phase fluctuations. It has long been foreseen, though, that such squeezing would be "at least an order of magnitude more difficult" to observe than the emission of single photons. Squeezed beams have been generated using macroscopic and mesoscopic media down to a few tens of atoms, but despite experimental efforts, single-atom squeezing has so far escaped observation. Here we generate squeezed light with a single atom in a high-finesse optical resonator. The strong coupling of the atom to the cavity field induces a genuine quantum mechanical nonlinearity, several orders of magnitude larger than for usual macroscopic media. This produces observable quadrature squeezing with an excitation beam containing on average only two photons per system lifetime. In sharp contrast to the emission of single photons, the squeezed light stems from the quantum coherence of photon pairs emitted from the system. The ability of a single atom to induce strong coherent interactions between propagating photons opens up new perspectives for photonic quantum logic with single emittersComment: Main paper (4 pages, 3 figures) + Supplementary information (5 pages, 2 figures). Revised versio

Superradiance and Phase Multistability in Circuit Quantum Electrodynamics

By modeling the coupling of multiple superconducting qubits to a single cavity in the circuit-quantum electrodynamics (QED) framework we find that it should be possible to observe superradiance and phase multistability using currently available technology. Due to the exceptionally large couplings present in circuit-QED we predict that superradiant microwave pulses should be observable with only a very small number of qubits (just three or four), in the presence of energy relaxation and non-uniform qubit-field coupling strengths. This paves the way for circuit-QED implementations of superradiant state readout and decoherence free subspace state encoding in subradiant states. The system considered here also exhibits phase multistability when driven with large field amplitudes, and this effect may have applications for collective qubit readout and for quantum feedback protocols.Comment: Published Versio

High Efficiency Colloidal Quantum Dot Infrared Light Emitting Diodes via Engineering at the Supra-Nanocrystalline Level

Colloidal quantum dot (CQD) light-emitting diodes (LEDs) deliver a compelling performance in the visible, yet infrared CQD LEDs underperform their visible-emitting counterparts, largely due to their low photoluminescence quantum efficiency. Here we employ a ternary blend of CQD thin film that comprises a binary host matrix that serves to electronically passivate as well as to cater for an efficient and balanced carrier supply to the emitting quantum dot species. In doing so, we report infrared PbS CQD LEDs with an external quantum efficiency of ~7.9% and a power conversion efficiency of ~9.3%, thanks to their very low density of trap states, on the order of 1014 cm−3, and very high photoluminescence quantum efficiency in electrically conductive quantum dot solids of more than 60%. When these blend devices operate as solar cells they deliver an open circuit voltage that approaches their radiative limit thanks to the synergistic effect of the reduced trap-state density and the density of state modification in the nanocomposite.Peer ReviewedPostprint (author's final draft

Observation of Resonant Photon Blockade at Microwave Frequencies using Correlation Function Measurements

Creating a train of single photons and monitoring its propagation and interaction is challenging in most physical systems, as photons generally interact very weakly with other systems. However, when confining microwave frequency photons in a transmission line resonator, effective photon-photon interactions can be mediated by qubits embedded in the resonator. Here, we observe the phenomenon of photon blockade through second-order correlation function measurements. The experiments clearly demonstrate antibunching in a continuously pumped source of single microwave photons measured using microwave beam splitters, linear amplifiers, and quadrature amplitude detectors. We also investigate resonance fluorescence and Rayleigh scattering in Mollow-triplet-like spectra