Systematics of the odd-even effect in the resonance ionization of Os and Ti

Measurements of the odd-even effect in the mass spectrometric analysis of Ti and Os isotopes by resonance ionization mass spectrometry have been performed for ΔJ = + 1, 0 and -1 transitions. Under saturating conditions of the ionization and for ΔJ = + 1 transitions odd-even effects are reduced below the 0.5% level. Depending on the polarization state of the laser large odd isotope enrichments are observed for ΔJ = 0 and -1 transitions which can be reduced below the 0.5% level by depolarization of the laser field

Design and commissioning of a timestamp-based data acquisition system for the DRAGON recoil mass separator

The DRAGON recoil mass separator at TRIUMF exists to study radiative proton and alpha capture reactions, which are important in a variety of astrophysical scenarios. DRAGON experiments require a data acquisition system that can be triggered on either reaction product ($\gamma$ ray or heavy ion), with the additional requirement of being able to promptly recognize coincidence events in an online environment. To this end, we have designed and implemented a new data acquisition system for DRAGON which consists of two independently triggered readouts. Events from both systems are recorded with timestamps from a $20$ MHz clock that are used to tag coincidences in the earliest possible stage of the data analysis. Here we report on the design, implementation, and commissioning of the new DRAGON data acquisition system, including the hardware, trigger logic, coincidence reconstruction algorithm, and live time considerations. We also discuss the results of an experiment commissioning the new system, which measured the strength of the $E_{\text{c}.\text{m}.} = 1113$ keV resonance in the $^{20}$Ne$\left(p, \gamma \right)^{21}$Na radiative proton capture reaction.Comment: 11 pages, 7 figures, accepted for publication in EPJ A "tools for experiment and theory

Systematics of isotope ratio measurements with resonant laser photoionization sources

Sources of laser-induced even-even and odd-even isotopic selectivity in the resonance ionization mass spectroscopy of Os and Ti have been investigated experimentally for various types of transitions. A set of conditions with regard to laser bandwidth and frequency tuning, polarization state and intensity was obtained for which isotopic selectivity is either absent or reduced below the 2 % level

Laser-induced isotopic effects in titanium resonance ionization

Titanium isotope ratios have been measured by resonance ionization mass spectrometry (RIMS) with special emphasis on the nature of laser-induced isotopic selectivity. A pronounced wavelength dependence of even mass isotope ratios is caused by large nuclear volume effects near the magic neutron number 28 in ^(50)Ti . Optical isotope shifts, ranging from 0.07 to 0.21 cm^(-l), between ^(50)Ti and ^(46)Ti were measured for several transitions. The ^(50)Ti/^(46)Ti and ^(48)Ti/^(46)Ti ratios, nevertheless, exhibited only mass-dependent fractionation, in which the lighter Ti isotopes were enriched by ~2.5%/amu, when the laser operating parameters were properly controlled. Odd-even mass isotopic selectivity in the resonant ionization process was also examined for several transitions as a function of the laser polarization state and intensity. Under saturating conditions for a ΔJ= +1 transition and a high degree of laser depolarization for a ΔJ = 0 transition, the odd-even isotopic enhancement was reduced below the 2% level. The Ti isotope data agree with our previous results for Os and indicate that, by a careful choice of resonance transitions and laser operating parameters, isotope ratios can be measured accurately and reliably with RIMS

Fremdlinge in Leoville and Allende CAI – Clues to Post-Formation Cooling and Alteration

Fremdlinge are perhaps the most exotic and least understood objects in CAI and their very existence places severe constraints regarding formation and cooling histories of the host CAI. Following the discovery and description of Willy, which appears to be an "Ur-Fremdling" or prototype for smaller Fremdlinge in CAI, we have begun a systematic study of CAI of different petrographic types to see if the Fremdlinge are consistent with a common mode of formation and differing degrees of reprocessing. Fifteen type B I, B2, and compact A CAI from Allende and Leoville were selected. The relative abundance of Fremdlinge varies dramatically among CAI, however some CAI of each type and from each meteorite contain abundant Fremdlinge. The range of phase assemblages and mineral chemistries of Fremdlinge from Allende and Leoville is very similar suggesting that the parent sources for Fremdlinge were quite similar. Chemically and texturally, Fremdlinge grade continuously from complex, heterogeneous Willy-like objects to altered, homogeneous metal nuggets. Some complex Fremdlinge like Willy were found in B1 CAI; none were observed in B2 CAI

Effect of allopurinol on phosphocreatine recovery and muscle function in older people with impaired physical function:a randomised controlled trial

Background: Allopurinol has vascular antioxidant effects and participates in purinergic signalling within muscle. We tested whether allopurinol could improve skeletal muscle energetics and physical function in older people with impaired physical performance. Methods: We conducted a randomised, double blind, parallel group, placebo-controlled trial, comparing 20 weeks of allopurinol 600 mg once daily versus placebo. We recruited community-dwelling participants aged 65 and over with baseline 6-min walk distance of &lt;400 m and no contraindications to magnetic resonance imaging scanning. Outcomes were measured at baseline and 20 weeks. The primary outcome was post-exercise phosphocreatine (PCr) recovery rate measured using 31P magnetic resonance spectroscopy of the calf. Secondary outcomes included 6-min walk distance, short physical performance battery (SPPB), lean body mass measured by bioimpedance, endothelial function and quality of life. Results: In total, 124 participants were randomised, mean age 80 (SD 6) years. A total of 59 (48%) were female, baseline 6-min walk distance was 293 m (SD 80 m) and baseline SPPB was 8.5 (SD 2.0). Allopurinol did not significantly improve PCr recovery rate (treatment effect 0.10 units [95% CI, −0.07 to 0.27], P = 0.25). No significant changes were seen in endothelial function, quality of life, lean body mass or SPPB. Allopurinol improved 6-min walk distance (treatment effect 25 m [95% 4–46, P = 0.02]). This was more pronounced in those with high baseline oxidative stress and urate. Conclusion: Allopurinol improved 6-min walk distance but not PCr recovery rate in older people with impaired physical function. Antioxidant strategies to improve muscle function for older people may need to be targeted at subgroups with high baseline oxidative stress. </p

Correlated Isotope Fractionation and Formation of Purple FUN Inclusions

Allende coarse-grained inclusions characterized by a distinct purple color and high spinel contents (≤ 50 vol.%) exhibit a higher frequency of FUN isotopic anomalies (≈20%) than the general CAI population (≤6%). We used the ion microprobe to measure Mg, Si, Cr and Fe isotopic compositions of three Purple Spinel-rich Inclusions (PSI = ψ) which are petrographically similar to Type B CAl to investigate: 1) variations in isotopic fractionation within inclusions, including secondary phases; 2) correlated isotopic fractionation; and 3) excess ^(26)Mg

The Cr Isotopic Composition of Phosphates in IIIB Iron Meteorites: A Search for ^(53)Mn

The metal phases of iron meteorites contain excess ^(107) Ag most plausibly derived from the in situ decay of ^(107)Pd (T_(1/2) = 6.5 x 10^6y) (Kaiser and Wasserburg, 1983; Chen and Wasserburg, 1983). The Ag isotopic data suggest that diverse types of iron meteorites, including the Type IIIABs, usually associated with fractional crystallization and core formation in planetesimals, formed and cooled to - 600°C within - 10^7y of ^(107)Pd production

Probing Correlated Ground States with Microscopic Optical Model for Nucleon Scattering off Doubly-Closed-Shell Nuclei

The RPA long range correlations are known to play a significant role in understanding the depletion of single particle-hole states observed in (e, e') and (e, e'p) measurements. Here the Random Phase Approximation (RPA) theory, implemented using the D1S force is considered for the specific purpose of building correlated ground states and related one-body density matrix elements. These may be implemented and tested in a fully microscopic optical model for NA scattering off doubly-closed-shell nuclei. A method is presented to correct for the correlations overcounting inherent to the RPA formalism. One-body density matrix elements in the uncorrelated (i.e. Hartree-Fock) and correlated (i.e. RPA) ground states are then challenged in proton scattering studies based on the Melbourne microscopic optical model to highlight the role played by the RPA correlations. Effects of such correlations which deplete the nuclear matter at small radial distance (r $<$ 2 fm) and enhance its surface region, are getting more and more sizeable as the incident energy increases. Illustrations are given for proton scattering observables measured up to 201 MeV for the $^{16}$O, $^{40}$Ca, $^{48}$Ca and $^{208}$Pb target nuclei. Handling the RPA correlations systematically improves the agreement between scattering predictions and data for energies higher than 150 MeV.Comment: 20 pages, 7 figure