288 research outputs found

    A model for liquid-striped liquid phase separation in liquids of anisotropic polarons

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    The phase separation between a striped polaron liquid at the particular density and a high density polaron liquid is described by a modified Van der Waals scheme. The striped polaron liquid represents the pseudo gap matter or Wigner-like polaron phase at 1/8 doping in cuprate superconductors. The model includes the tendency of pseudo- Jahn-Teller polarons to form anisotropic directional bonds at a preferential volume with the formation of different liquid phases. The model gives the coexistence of a first low density polaron striped liquid and a second high density liquid that appears in cuprate superconductors for doping larger than 1/8. We discuss how the strength of anisotropic bonds controls the variation the phase separation scenarios for complex systems in the presence of a quantum critical point where the phase separation vanishes.Comment: 10 pages, 3 figure

    Multiorbital analysis of the effects of uniaxial and hydrostatic pressure on TcT_c in the single-layered cuprate superconductors

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    The origin of uniaxial and hydrostatic pressure effects on TcT_c in the single-layered cuprate superconductors is theoretically explored. A two-orbital model, derived from first principles and analyzed with the fluctuation exchange approximation gives axial-dependent pressure coefficients, Tc/Pa>0\partial T_c/\partial P_a>0, Tc/Pc<0\partial T_c/\partial P_c<0, with a hydrostatic response Tc/P>0\partial T_c/\partial P>0 for both La214 and Hg1201 cuprates, in qualitative agreement with experiments. Physically, this is shown to come from a unified picture in which higher TcT_c is achieved with an "orbital distillation", namely, the less the dx2y2d_{x^2-y^2} main band is hybridized with the dz2d_{z^2} and 4s4s orbitals higher the TcT_c. Some implications for obtaining higher TcT_c materials are discussed.Comment: 6pages, 4 figure

    Direct observation of nanoscale interface phase in the superconducting chalcogenide Kx_{x}Fe2y_{2-y}Se2_2 with intrinsic phase separation

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    We have used scanning micro x-ray diffraction to characterize different phases in superconducting Kx_{x}Fe2y_{2-y}Se2_2 as a function of temperature, unveiling the thermal evolution across the superconducting transition temperature (Tc_c\sim32 K), phase separation temperature (Tps_{ps}\sim520 K) and iron-vacancy order temperature (Tvo_{vo}\sim580 K). In addition to the iron-vacancy ordered tetragonal magnetic phase and orthorhombic metallic minority filamentary phase, we have found a clear evidence of the interface phase with tetragonal symmetry. The metallic phase is surrounded by this interface phase below \sim300 K, and is embedded in the insulating texture. The spatial distribution of coexisting phases as a function of temperature provides a clear evidence of the formation of protected metallic percolative paths in the majority texture with large magnetic moment, required for the electronic coherence for the superconductivity. Furthermore, a clear reorganization of iron-vacancy order around the Tps_{ps} and Tc_c is found with the interface phase being mostly associated with a different iron-vacancy configuration, that may be important for protecting the percolative superconductivity in Kx_{x}Fe2y_{2-y}Se2_2.Comment: 6 pages, 4 figure

    Two-bands superconductivity with intra- and interband pairing for synthetic superlattices

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    We consider a model for superconductivity in a two-band superconductor, having an anisotropic electronic structure made of two partially overlapping bands with a first hole-like and a second electron-like fermi surface. In this pairing scenario, driven by the interplay between interband Vi,jV_{i,j} and intraband Vi,iV_{i,i} pairing terms, we have solved the two gap equations at the critical temperature T=TcT = T_c and calculate TcT_c and the chemical potential μ\mu as a function of the number of carriers nn for various values of pairing interactions, V1,1V_{1,1}, V2,2V_{2,2}, and V1,2V_{1,2}. The results show the complexity of the physics of condensates with multiple order parameters with the chemical potential near band edges.Comment: 6 pages, 2 figure

    Flux dynamics in NdO1-xFxFeAs bulk sample

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    We present data of multi harmonic magneto-dynamic experiments. In particular, we performed ac magnetic susceptibility experiments on layered pnictide-oxide quaternary compound NdOFeAs doped with fluorine. The experiments allow measure the critical temperature and probe the flux dynamic behavior using the third harmonic component of the ac susceptibility of a NdF0.16FeAsO0.84 bulk sample as a function of temperature and frequency of the applied ac magnetic fields. Measured signals are connected with the non-linear superconducting flux dynamic behavior and are characterized by a flux critical states sustaining a superconducting critical current. In this framework the irreversibility line that describes the stable superconducting state has been extracted from the onset of the third harmonic signal vs. frequency. Finally we present also the analysis of the flux dynamic dimensionality in the investigated sample.Comment: 10 pages, 5 figure

    Effect of defects on reaction of NiO surface with Pb-contained solution

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    In order to understand the role of defects in chemical reactions, we used two types of samples, which are molecular beam epitaxy (MBE) grown NiO(001) film on Mg(001) substrate as the defect free NiO prototype and NiO grown on Ni(110) single crystal as the one with defects. In-situ observations for oxide-liquid interfacial structure and surface morphology were performed for both samples in water and Pb-contained solution using high-resolution X-ray reflectivity and atomic force microscopy. For the MBE grown NiO, no significant changes were detected in the high-resolution X-ray reflectivity data with monotonic increase in roughness. Meanwhile, in the case of native grown NiO on Ni(110), significant changes in both the morphology and atomistic structure at the interface were observed when immersed in water and Pb-contained solution. Our results provide simple and direct experimental evidence of the role of the defects in chemical reaction of oxide surfaces with both water and Pb-contained solution.ope

    Vesicular PtdIns(3,4,5) P 3 and Rab7 are key effectors of sea urchin zygote nuclear membrane fusion

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    Regulation of nuclear envelope (NE) dynamics is an important example of the universal phenomena of membrane fusion. The signalling molecules involved in nuclear membrane fusion may also be conserved in the formation of both pronuclear and zygote NEs in the fertilised egg. Here, we determine that Class I PI3-kinases are needed for in vitro nuclear envelope formation. We show that, in vivo, PtdIns(3,4,5)P3 is transiently located in vesicles around the male pronucleus at the time of nuclear envelope formation and around male and female pronuclei prior to membrane fusion. We illustrate that Class I PI3-kinase activity is also necessary for fusion of the female and male pronuclear membranes. We demonstrate, by coincidence amplified-FRET monitored by fluorescence lifetime imaging microscopy (FLIM), a protein-lipid interaction of Rab7 GTPase and PtdIns(3,4,5)P3 occurring during pronuclear membrane fusion to create the zygote nuclear envelope. We present a working model, which includes several molecular steps in the pathways controlling fusion of NE membranes.</jats:p
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