Assessment of the U and Co magnetic moments in UCoGe by X-ray magnetic circular dichroism

The ferromagnetic superconductor UCoGe has been investigated by high field X-ray magnetic circular dichroism (XMCD) at the U-M$_{4,5}$ and Co/Ge-K edges. The analysis of the branching ratio and XMCD at the U-M$_{4,5}$ edges reveals that the U-5$f$ electrons count is close to 3. The orbital ($\sim0.70\,\mu_B$) and spin ($\sim-0.30\,\mu_B$) moments of U at 2.1K and 17T (H//c) have been determined. Their ratio ($\sim-2.3$) suggests a significant delocalization of the 5$f$ electron states. The similar field dependences of the local U/Co and the macroscopic magnetization indicate that the Co moment is induced by the U moment. The XMCD at the Co/Ge-K edges reveal the presence of small Co-4$p$ and Ge-4$p$ orbital moments parallel to the macroscopic magnetization. In addition, the Co-3$d$ moment is estimated to be at most of the order of 0.1$\mu_B$ at 17T. Our results rule out the possibility of an unusual polarisability of the U and Co moments as well as their antiparallel coupling. We conclude that the magnetism which mediates the superconductivity in UCoGe is driven by U.Comment: 4 figures + supplementary materia

Double crystal x-ray diffraction simulations of diffusion in semiconductor microstructures

Diffusion in group IV, III-V and II-VI semiconductors is an interesting problem not only from a fundamental physics viewpoint but also in practical terms, since it could determine the useful lifetime of a device. Any attempt to control the amount of diffusion in a semiconductor device, whether it be a quantum well structure or not, requires an accurate determination of the diffusion coefficient. The present theoretical study shows that this could be achieved via x-ray diffraction studies in quantum well structures. It is demonstrated that the rocking curves of single quantum wells are not sensitive to diffusion. However the intensity of the first order satellite, which is characteristic of superlattice rocking curves, is strongly dependent upon diffusion and it is proposed that this technique could be used to measure the diffusion coefficient D. © 1998 American Institute of Physics

Thermal conductivity through the quantum critical point in YbRh2Si2 at very low temperature

The thermal conductivity of YbRh2Si2 has been measured down to very low temperatures under field in the basal plane. An additional channel for heat transport appears below 30 mK, both in the antiferromagnetic and paramagnetic states, respectively below and above the critical field suppressing the magnetic order. This excludes antiferromagnetic magnons as the origin of this additional contribution to thermal conductivity. Moreover, this low temperature contribution prevails a definite conclusion on the validity or violation of the Wiedemann-Franz law at the field-induced quantum critical point. At high temperature in the paramagnetic state, the thermal conductivity is sensitive to ferromagnetic fluctuations, previously observed by NMR or neutron scattering and required for the occurrence of the sharp electronic spin resonance fracture.Comment: 11 pages + Supplementary Material

Sequential localization of a complex electron fluid

Complex and correlated quantum systems with promise for new functionality often involve entwined electronic degrees of freedom. In such materials, highly unusual properties emerge and could be the result of electron localization. Here, a cubic heavy fermion metal governed by spins and orbitals is chosen as a model system for this physics. Its properties are found to originate from surprisingly simple low-energy behavior, with two distinct localization transitions driven by a single degree of freedom at a time. This result is unexpected, but we are able to understand it by advancing the notion of sequential destruction of an SU(4) spin-orbital-coupled Kondo entanglement. Our results implicate electron localization as a unified framework for strongly correlated materials and suggest ways to exploit multiple degrees of freedom for quantum engineering.Comment: 21 pages, 4 figures (preprint format

Takagi-Taupin Description of X-ray Dynamical Diffraction from Diffractive Optics with Large Numerical Aperture

We present a formalism of x-ray dynamical diffraction from volume diffractive optics with large numerical aperture and high aspect ratio, in an analogy to the Takagi-Taupin equations for strained single crystals. We derive a set of basic equations for dynamical diffraction from volume diffractive optics, which enable us to study the focusing property of these optics with various grating profiles. We study volume diffractive optics that satisfy the Bragg condition to various degrees, namely flat, tilted and wedged geometries, and derive the curved geometries required for ultimate focusing. We show that the curved geometries satisfy the Bragg condition everywhere and phase requirement for point focusing, and effectively focus hard x-rays to a scale close to the wavelength.Comment: 18 pages, 12 figure

A lattice model for the kinetics of rupture of fluid bilayer membranes

We have constructed a model for the kinetics of rupture of membranes under tension, applying physical principles relevant to lipid bilayers held together by hydrophobic interactions. The membrane is characterized by the bulk compressibility (for expansion), the thickness of the hydrophobic part of the bilayer, the hydrophobicity and a parameter characterizing the tail rigidity of the lipids. The model is a lattice model which incorporates strain relaxation, and considers the nucleation of pores at constant area, constant temperature, and constant particle number. The particle number is conserved by allowing multiple occupancy of the sites. An equilibrium ``phase diagram'' is constructed as a function of temperature and strain with the total pore surface and distribution as the order parameters. A first order rupture line is found with increasing tension, and a continuous increase in proto-pore concentration with rising temperature till instability. The model explains current results on saturated and unsaturated PC lipid bilayers and thicker artificial bilayers made of diblock copolymers. Pore size distributions are presented for various values of area expansion and temperature, and the fractal dimension of the pore edge is evaluated.Comment: 15 pages, 8 figure