Magnetic and electrical resistance behaviour of the oxides, Ca3−x_{3-x}Yx_xLiRuO6_6 (x= 0.0, 0.5 and 1.0)

We have investigated the magnetic and electrical resistance behaviour of Ca$_{3-x}$Y$_x$LiRuO$_6$. The parent compound exhibits magnetic ordering from Ru sublattice at a rather high temperature, 113 K. Though the paramagnetic Curie temperature ($\theta$$_p$) is negative indicative of antiferromagnetic ordering, the large magnitude (-250 K) of $\theta$$_p$ reveals complex nature of the magnetism in this compound. Ru ions appear to be in the pentavalent state. We note that the N\'eel temperature undergoes only a marginal reduction by Y substitution. All these compositions are found to be insulators and thus the electron doping does not result in metallicity. Thus the overall magnetic and transport behaviour are found to be essentially insensitive to Y substitution for Ca, a finding which may favour the idea of quasi-one-dimensional magnetism in these compounds.Comment: 5 pages of text in RevTex, 6 figures, Solid State Communications (in press

Magnetization Measurement of a Possible High-Temperature Superconducting State in Amorphous Carbon Doped with Sulfur

Magnetization M(T,H) measurements performed on thoroughly characterized commercial amorphous carbon powder doped with sulfur (AC-S), revealed the occurrence of an inhomogeneous superconductivity (SC) below T_c = 38 K. The constructed magnetic field-temperature (H-T) phase diagram resembles that of type-II superconductors. However, AC-S demonstrates a number of anomalies. In particular, we observed (1) a non-monotonic behavior of the lower critical field H_c1(T); (2) a pronounced positive curvature of the "upper critical field boundary" that we associated with the flux lattice melting line Hm(T); (3) a spontaneous ferromagnetic-like magnetization M0 coexisting with SC. Based on the analysis of experimental results we propose a nonstandard SC state in AC-S.Comment: 18 pages including 5 figure

Low temperature magnetic transition in RuSr2EuCeCu2O10 ruthenocuprate

A new magnetic transition in the ruthenocuprate parent compound RuSr2EuCeCu2O10 has been observed below 10 K. It shows up only as a kink in the imaginary part of the ac susceptibility and exhibits a pronounced frequency dependence. At the same time, the real part of the ac susceptibility and the dc magnetization study show very little change in the same temperature window suggesting only a minor fraction of the material to be involved in the transition. Frequency dependence shows excellent agreement with the predictions of the Arrhenius law known to describe well the dynamics of the superparamagnetic particles. The same type of the investigation on the RuSr2Eu1.1Ce0.9Cu2O10 composition showed no evidence of the similar transition, which points to a possible intrinsic behavior.Comment: to be published in Physica