FAST CARS: Engineering a Laser Spectroscopic Technique for Rapid Identification of Bacterial Spores

Airborne contaminants, e.g., bacterial spores, are usually analyzed by time consuming microscopic, chemical and biological assays. Current research into real time laser spectroscopic detectors of such contaminants is based on e.g. resonant Raman spectroscopy. The present approach derives from recent experiments in which atoms and molecules are prepared by one (or more) coherent laser(s) and probed by another set of lasers. The connection with previous studies based on "Coherent Anti-Stokes Raman Spectroscopy" (CARS) is to be noted. However generating and utilizing maximally coherent oscillation in macromolecules having an enormous number of degrees of freedom is much more challenging. This extension of the CARS technique is called FAST CARS (Femtosecond Adaptive Spectroscopic Techniques for Coherent Anti-Stokes Raman Spectroscopy), and the present paper proposes and analyses ways in which it could be used to rapidly identify pre-selected molecules in real time.Comment: 43 pages, 21 figures; replacement with references added. Submitted to the Proceedings of National Academy of Science

Grain Boundary Induced Magneto-Far Infrared Resonances in Superconducting YBa2_2Cu3_3O7−δ_{7-\delta } Thin Films

Spectral features induced by 45$^{\circ }$ in-plane misoriented grains have been observed in the far infrared magneto-transmission of YBa$_2$Cu$_3$O$_{7-\delta }$ thin films. Two strong dispersive features are found at 80 and 160 $cm^{-1}$ and a weaker one at 116 $cm^{-1}$. The data can be well represented by Lorentzian oscillator contributions to the conductivity. Several possible interpretations are discussed. We conclude that the resonances are due to vortex core excitations.Comment: Latex file (14 pages) + 4 Postscript figures, uuencode

Coherent phenomena in semiconductors

A review of coherent phenomena in photoexcited semiconductors is presented. In particular, two classes of phenomena are considered: On the one hand the role played by optically-induced phase coherence in the ultrafast spectroscopy of semiconductors; On the other hand the Coulomb-induced effects on the coherent optical response of low-dimensional structures. All the phenomena discussed in the paper are analyzed in terms of a theoretical framework based on the density-matrix formalism. Due to its generality, this quantum-kinetic approach allows a realistic description of coherent as well as incoherent, i.e. phase-breaking, processes, thus providing quantitative information on the coupled ---coherent vs. incoherent--- carrier dynamics in photoexcited semiconductors. The primary goal of the paper is to discuss the concept of quantum-mechanical phase coherence as well as its relevance and implications on semiconductor physics and technology. In particular, we will discuss the dominant role played by optically induced phase coherence on the process of carrier photogeneration and relaxation in bulk systems. We will then review typical field-induced coherent phenomena in semiconductor superlattices such as Bloch oscillations and Wannier-Stark localization. Finally, we will discuss the dominant role played by Coulomb correlation on the linear and non-linear optical spectra of realistic quantum-wire structures.Comment: Topical review in Semiconductor Science and Technology (in press) (Some of the figures are not available in electronic form

Measurement of the Far Infrared Magneto-Conductivity Tensor of Superconducting YBa2_2Cu3_3O7−δ_{7-\delta } Thin Films

We report measurements of the far infrared transmission of superconducting YBa$_2$Cu$_3$O$_{7-\delta }$ thin films from 5 cm$^{-1}$ to 200 cm$^{-1}$ in fields up to 14$T$. A Kramers-Kronig analysis of the magneto-transmission spectrum yields the magneto-conductivity tensor. The result shows that the magneto-conductivity of YBa$_2$Cu$_3$O$_{7-\delta }$ is dominated by three terms: a London term, a low frequency Lorentzian ($\omega _1\approx$ 3 cm$^{-1}$) of width $\Gamma _1=$ 10 cm$^{-1}$ and a finite frequency Lorentzian of width $\Gamma _2=$ 17 cm$^{-1}$ at $\omega _2=$ 24 cm$^{-1}$ in the hole cyclotron resonance active mode of circular polarization.\\Comment: Revised LaTex file (12 pages) + 4 Postscript figures, uuencoded. In response to referees' comments, we refined the paper a lot; we encourage you to download this revised versio

Resonant nonlinear magneto-optical effects in atoms

In this article, we review the history, current status, physical mechanisms, experimental methods, and applications of nonlinear magneto-optical effects in atomic vapors. We begin by describing the pioneering work of Macaluso and Corbino over a century ago on linear magneto-optical effects (in which the properties of the medium do not depend on the light power) in the vicinity of atomic resonances, and contrast these effects with various nonlinear magneto-optical phenomena that have been studied both theoretically and experimentally since the late 1960s. In recent years, the field of nonlinear magneto-optics has experienced a revival of interest that has led to a number of developments, including the observation of ultra-narrow (1-Hz) magneto-optical resonances, applications in sensitive magnetometry, nonlinear magneto-optical tomography, and the possibility of a search for parity- and time-reversal-invariance violation in atoms.Comment: 51 pages, 23 figures, to appear in Rev. Mod. Phys. in Oct. 2002, Figure added, typos corrected, text edited for clarit

Resolving the Drivers of Algal Nutrient Limitation from Boreal to Arctic Lakes and Streams

Nutrient inputs to northern freshwaters are changing, potentially altering aquatic ecosystem functioning through effects on primary producers. Yet, while primary producer growth is sensitive to nutrient supply, it is also constrained by a suite of other factors, including light and temperature, which may play varying roles across stream and lake habitats. Here, we use bioassay results from 89 lakes and streams spanning northern boreal to Arctic Sweden to test for differences in nutrient limitation status of algal biomass along gradients in colored dissolved organic carbon (DOC), water temperature, and nutrient concentrations, and to ask whether there are distinct patterns and drivers between habitats. Single nitrogen (N) limitation or primary N-limitation with secondary phosphorus (P) limitation of algal biomass was the most common condition for streams and lakes. Average response to N-addition was a doubling in biomass; however, the degree of limitation was modulated by the distinct physical and chemical conditions in lakes versus streams and across boreal to Arctic regions. Overall, algal responses to N-addition were strongest at sites with low background concentrations of dissolved inorganic N. Low temperatures constrained biomass responses to added nutrients in lakes but had weaker effects on responses in streams. Further, DOC mediated the response of algal biomass to nutrient addition differently among lakes and streams. Stream responses were dampened at higher DOC, whereas lake responses to nutrient addition increased from low to moderate DOC but were depressed at high DOC. Our results suggest that future changes in nutrient availability, particularly N, will exert strong effects on the trophic state of northern freshwaters. However, we highlight important differences in the physical and chemical factors that shape algal responses to nutrient availability in different parts of aquatic networks, which will ultimately affect the integrated response of northern aquatic systems to ongoing environmental changes

A prism reflector of anti-resonant ring configuration

Two identical prisms are combined to form an anti-resonant ring reflector, giving total reflection without the use of coatings or roof edges. When used as the total reflector in a Q-switched Nd:YAG laser this device has shown a damage threshold twice that of a multilayer reflector