Nonlinear dynamics of polariton scattering in semiconductor microcavity: bistability vs stimulated scattering

We demonstrate experimentally an unusual behavior of the parametric polariton scattering in semiconductor microcavity under a strong cw resonant excitation. The maximum of the scattered signal above the threshold of stimulated parametric scattering does not shift along the microcavity lower polariton branch with the change of pump detuning or angle of incidence but is stuck around the normal direction. We show theoretically that such a behavior can be modelled numerically by a system of Maxwell and nonlinear Schroedinger equations for cavity polaritons and explained via the competition between the bistability of a driven nonlinear MC polariton and the instabilities of parametric polariton-polariton scattering.Comment: 5 pages, 4 Postscript figures; corrected typo

Terahertz emitters based on microcavity dipolaritons

We propose the use of dipolaritons -- quantum well excitons with large dipole moment, coupled to a planar microcavity -- for generating terahertz (THz) radiation. This is achieved by exciting the system with two THz detuned lasers that leads to dipole moment oscillations of the exciton polariton at the detuning frequency, thus generating a THz emission. We have optimized the structural parameters of a system with microcavity embedded AlGaAs double quantum wells and shown that the THz emission intensity is maximized if the laser frequencies both match different dipolariton states. The influence of the electronic tunnel coupling between the wells on the frequency and intensity of the THz radiation is also investigated, demonstrating a trade-off between the polariton dipole moment and the Rabi splitting.Comment: 4 pages, 4 figures. This article has been submitted to Applied Physics Letter

Size-dependence of anisotropic exchange interaction in InAs/GaAs quantum dots

A comprehensive study of the exchange interaction between charge carriers in self-organized InAs/GaAs quantum dots is presented. Single quantum-dot cathodoluminescence spectra of quantum dots of different sizes are analyzed. Special attention is paid to the energetic structure of the charged excited exciton (hot trion). A varying degree of intermixing within the hot trion states leads to varying degrees of polarization of the corresponding emission lines. The emission characteristics change from circularly polarized for small quantum dots to elliptically polarized for large quantum dots. The findings are explained by a change of magnitude of the anisotropic exchange interaction and compared to the related effect of fine-structure splitting in the neutral exciton and biexciton emission.Comment: 4 pages, 3 figures, to be published in phys. stat. sol (b), proceedings of the QD2006, May 1-5 2006, Chamonix-Mont-Blanc, Franc

Spin multistability of cavity polaritons in a magnetic field

Spin transitions are studied theoretically and experimentally in a resonantly excited system of cavity polaritons in a magnetic field. Weak pair interactions in this boson system make possible fast and massive spin flips occurring at critical amplitudes due to the interplay between amplitude dependent shifts of eigenstates and the Zeeman splitting. Dominant spin of a condensate can be toggled forth and back by tuning of the pump intensity only, which opens the way for ultra-fast spin switchings of polariton condensates on a picosecond timescale.Comment: 4 pages, 4 figure

The trion: two electrons plus one hole versus one electron plus one exciton

We first show that, for problems dealing with trions, it is totally hopeless to use the standard many-body description in terms of electrons and holes and its associated Feynman diagrams. We then show how, by using the description of a trion as an electron interacting with an exciton, we can obtain the trion absorption through far simpler diagrams, written with electrons and \emph{excitons}. These diagrams are quite novel because, for excitons being not exact bosons, we cannot use standard procedures designed to deal with interacting true fermions or true bosons. A new many-body formalism is necessary to establish the validity of these electron-exciton diagrams and to derive their specific rules. It relies on the ``commutation technique'' we recently developed to treat interacting close-to-bosons. This technique generates a scattering associated to direct Coulomb processes between electrons and excitons and a dimensionless ``scattering'' associated to electron exchange inside the electron-exciton pairs -- this ``scattering'' being the original part of our many-body theory. It turns out that, although exchange is crucial to differentiate singlet from triplet trions, this ``scattering'' enters the absorption explicitly when the photocreated electron and the initial electron have the same spin -- \emph{i}. \emph{e}., when triplet trions are the only ones created -- \emph{but not} when the two spins are different, although triplet trions are also created in this case. The physical reason for this rather surprising result will be given

Polarization bistability and resultant spin rings in semiconductor microcavities

The transmission of a pump laser resonant with the lower polariton branch of a semiconductor microcavity is shown to be highly dependent on the degree of circular polarization of the pump. Spin dependent anisotropy of polariton-polariton interactions allows the internal polarization to be controlled by varying the pump power. The formation of spatial patterns, spin rings with high degree of circular polarization, arising as a result of polarization bistability, is observed. A phenomenological model based on spin dependent Gross-Pitaevskii equations provides a good description of the experimental results. Inclusion of interactions with the incoherent exciton reservoir, which provides spin-independent blueshifts of the polariton modes, is found to be essential.Comment: 5 pages, 3 figure

Controlling circular polarization of light emitted by quantum dots using chiral photonic crystal slab

We study the polarization properties of light emitted by quantum dots that are embedded in chiral photonic crystal structures made of achiral planar GaAs waveguides. A modification of the electromagnetic mode structure due to the chiral grating fabricated by partial etching of the wave\-guide layer has been shown to result in a high circular polarization degree $\rho_c$ of the quantum dot emission in the absence of external magnetic field. The physical nature of the phenomenon can be understood in terms of the reciprocity principle taking into account the structural symmetry. At the resonance wavelength, the magnitude of $|\rho_c|$ is predicted to exceed 98%. The experimentally achieved value of $|\rho_c|=81$% is smaller, which is due to the contribution of unpolarized light scattered by grating defects, thus breaking its periodicity. The achieved polarization degree estimated removing the unpolarized nonresonant background from the emission spectra can be estimated to be as high as 96%, close to the theoretical prediction

Nonlinear emission dynamics of a GaAs microcavity with embedded quantum wells

The emission dynamics of a GaAs microcavity at different angles of observation with respect to the sample normal under conditions of nonresonant picosecond-pulse excitation is measured. At sufficiently high excitation densities, the decay time of the lower-polariton emission increases with the polariton wavevector; at low excitation densities the decay time is independent of the wavevector. The effect of additional nonresonant continuous illumination on the emission originating from the bottom of the lower polariton branch is investigated. The additional illumination leads to a substantial increase in the emission intensity (considerably larger than the intensity of the photoluminescence excited by this illumination alone). This fact is explained in terms of acceleration of the polariton relaxation to the radiative states due to scattering by charge carriers created by the additional illumination. The results obtained show, that at large negative detunings between the photon and exciton modes, polariton-polariton and polariton-free carrier scattering are the main processes responsible for the filling of states near the bottom of the lower polariton branch.Comment: 10 pages, 6 figures. This is an author-created, un-copyedited version of an article accepted for publication in Journal of Physics: Condesed Matter. IOP Publishing Ltd is not responsible for any errors or omissions in this version of the manuscript or any version derived from i

Bistability and nonequilibrium transitions in the optically polarized system of cavity polaritons under nanosecond-long resonant excitation

The polarization dependence of nonequilibrium transitions in a multistable cavity-polariton system is studied under a nanosecond long resonant optical excitation at the normal and magic angle incidences with various polarizations of the pump beam. The temporal correlations between the frequency, intensity, and optical polarization of the intra-cavity field, which all undergo sharp threshold-like changes due to the spin dependent interaction of cavity polaritons, are visualized. The observed dynamics cannot be reproduced within the conventional semi-classical model based on the Gross-Pitaevskii equations. To explain the observed phenomena, it is necessary to take into account the unpolarized exciton reservoir which brings on additional blueshift of bright excitons, equal in the $\sigma^+$ and $\sigma^-$ polarization components. This model explains the effect of polarization instability under both pulsed and continuous wave resonant excitation conditions, consistently with the spin ring pattern formation that has recently been observed under Gaussian shaped excitation.Comment: 13 pages, 13 figure