211 research outputs found

    Two-dimensional Jeff{J}_{\rm eff} = 1/2 antiferromagnetic insulator unraveled from interlayer exchange coupling in artificial perovskite iridate superlattices

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    We report an experimental investigation of the two-dimensional Jeff{J}_{\rm eff} = 1/2 antiferromagnetic Mott insulator by varying the interlayer exchange coupling in [(SrIrO3_3)1_1, (SrTiO3_3)m_m] (mm = 1, 2 and 3) superlattices. Although all samples exhibited an insulating ground state with long-range magnetic order, temperature-dependent resistivity measurements showed a stronger insulating behavior in the mm = 2 and mm = 3 samples than the mm = 1 sample which displayed a clear kink at the magnetic transition. This difference indicates that the blocking effect of the excessive SrTiO3_3 layer enhances the effective electron-electron correlation and strengthens the Mott phase. The significant reduction of the Neel temperature from 150 K for mm = 1 to 40 K for mm = 2 demonstrates that the long-range order stability in the former is boosted by a substantial interlayer exchange coupling. Resonant x-ray magnetic scattering revealed that the interlayer exchange coupling has a switchable sign, depending on the SrTiO3_3 layer number mm, for maintaining canting-induced weak ferromagnetism. The nearly unaltered transition temperature between the mm = 2 and the mm = 3 demonstrated that we have realized a two-dimensional antiferromagnet at finite temperatures with diminishing interlayer exchange coupling.Comment: 4 figure

    Magnetic properties of GdT2T_2Zn20_{20} (T = Fe, Co) investigated by X-ray diffraction and spectroscopy

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    We investigate the magnetic and electronic properties of the GdT2T_2Zn20_{20} (TT = Fe and Co) compounds using X-ray resonant magnetic scattering (XRMS), X-ray absorption near-edge structure (XANES) and X-ray magnetic circular dichroism (XMCD) techniques. The XRMS measurements reveal that the GdCo2_2Zn20_{20} compound has a commensurate antiferromagnetic spin structure with a magnetic propagation vector τ\vec{\tau} = (12,12,12)(\frac{1}{2},\frac{1}{2},\frac{1}{2}) below the N\'eel temperature (TNT_N \sim 5.7 K). Only the Gd ions carry a magnetic moment forming an antiferromagnetic structure with magnetic representation Γ6\Gamma_6. For the ferromagnetic GdFe2_2Zn20_{20} compound, an extensive investigation was performed at low temperature and under magnetic field using XANES and XMCD techniques. A strong XMCD signal of about 12.5 %\% and 9.7 %\% is observed below the Curie temperature (TCT_C \sim 85 K) at the Gd-L2L_2 and L3L_3 edges, respectively. In addition, a small magnetic signal of about 0.06 %\% of the jump is recorded at the Zn KK-edge suggesting that the Zn 4pp states are spin polarized by the Gd 5dd extended orbitals

    Pressure-induced collapsed-tetragonal phase in SrCo2As2

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    We present high-energy x-ray diffraction data under applied pressures up to p = 29 GPa, neutron diffraction measurements up to p = 1.1 GPa, and electrical resistance measurements up to p = 5.9 GPa, on SrCo2As2. Our x-ray diffraction data demonstrate that there is a first-order transition between the tetragonal (T) and collapsed-tetragonal (cT) phases, with an onset above approximately 6 GPa at T = 7 K. The pressure for the onset of the cT phase and the range of coexistence between the T and cT phases appears to be nearly temperature independent. The compressibility along the a-axis is the same for the T and cT phases whereas, along the c-axis, the cT phase is significantly stiffer, which may be due to the formation of an As-As bond in the cT phase. Our resistivity measurements found no evidence of superconductivity in SrCo2As2 for p <= 5.9 GPa and T >= 1.8 K. The resistivity data also show signatures consistent with a pressure-induced phase transition for p >= 5.5 GPa. Single-crystal neutron diffraction measurements performed up to 1.1 GPa in the T phase found no evidence of stripe-type or A-type antiferromagnetic ordering down to 10 K. Spin-polarized total-energy calculations demonstrate that the cT phase is the stable phase at high pressure with a c/a ratio of 2.54. Furthermore, these calculations indicate that the cT phase of SrCo2As2 should manifest either A-type antiferromagnetic or ferromagnetic order.Comment: 6 pages, 5 figure

    Pressure and chemical substitution effects in the local atomic structure of BaFe2As2

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    The effects of K and Co substitutions and quasi-hydrostatic applied pressure (P<9 GPa) in the local atomic structure of BaFe2As2, Ba(Fe{0.937}Co{0.063})2As2 and Ba{0.85}K{0.15}Fe2As2 superconductors were investigated by extended x-ray absorption fine structure (EXAFS) measurements in the As K absorption edge. The As-Fe bond length is found to be slightly reduced (<~ 0.01 Angstroms) by both Co and K substitutions, without any observable increment in the corresponding Debye Waller factor. Also, this bond is shown to be compressible (k = 3.3(3)x10^{-3} GPa^{-1}). The observed contractions of As-Fe bond under pressure and chemical substitutions are likely related with a reduction of the local Fe magnetic moments, and should be an important tuning parameter in the phase diagrams of the Fe-based superconductors.Comment: 7 pages, 6 figure

    Optimizing Sales Using Mobile Sales Ticketing Application

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    A pressure-induced collapse of magnetic ordering in βLi2IrO3β−Li_{2}IrO_3 at Pm1.52P_m ∼ 1.5–2 GPa has previously been interpreted as evidence for possible emergence of spin liquid states in this hyperhoneycomb iridate, raising prospects for experimental realizations of the Kitaev model. Based on structural data obtained at room temperature, this magnetic transition is believed to originate in small lattice perturbations that preserve crystal symmetry, and related changes in bond-directional anisotropic exchange interactions. Here we report on the evolution of the crystal structure of βLi2IrO3β−Li_{2}IrO_3 under pressure at low temperatures (T50K)(T≤50 K) and show that the suppression of magnetism coincides with a change in lattice symmetry involving Ir-Ir dimerization. The critical pressure for dimerization shifts from 4.4(2) GPa at room temperature to 1.52∼1.5–2 GPa below 50 K. While a direct FdddC2/cFddd→C2/c transition is observed at room temperature, the low temperature transitions involve new as well as coexisting dimerized phases. Further investigation of the Ir (L3/L2L3/L_2) isotropic branching ratio in x-ray absorption spectra indicates that the previously reported departure of the electronic ground state from a Jeff=1/2J_{eff} = 1/2 state is closely related to the onset of dimerized phases. In essence, our results suggest that the predominant mechanism driving the collapse of magnetism in βLi2IrO3β−Li_{2}IrO_3 is the pressure-induced formation of Ir2Ir_2 dimers in the hyperhoneycomb network. The results further confirm the instability of the Jeff=1/2J_{eff} = 1/2 moments and related noncollinear spiral magnetic ordering against formation of dimers in the low-temperature phase of compressed βLi2IrO3β−Li_{2}IrO_3

    A qualitative exploration of memory cuing by personal items in the home

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    © The Author(s) 2017. We are surrounded by personal items that can trigger memories, such as photos, souvenirs and heirlooms. Also during holidays, we collect items to remind us of the events, but not all bring back memories to the same extent. Therefore, we explored peoples’ responses to personal items related to a holiday, using the home tour interviewing method. In total, 63 accounts of cuing responses from nine home tours were analysed using thematic analysis. This resulted in four types of cuing responses: (a) ‘no-memory’ responses, (b) ‘know’ responses, (c) ‘memory evoked think or feel’ responses and (d) ‘remember’ responses. For each of these cuing response categories, we looked into the types of items and their characteristics. Furthermore, we found that some items can evoke multiple memories. The majority of the memories’ content refers to events close to the moment of acquiring the item

    Exclusive surgical treatment for vestibular schwannoma regrowth or recurrence: A meta-analysis of the literature

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    Vestibular schwannomas can be treated in different ways, but for symptomatic or growing tumors, the gold standard is surgical removal of the lesion. In order to preserve neurovascular structures, partial removal is often performed, leaving a residual that may grow in subsequent years. To date, there is no consensus with regard to surgical treatment of vestibular schwannoma residuals, and so this review focuses on this topic. A structured search was performed on PubMed searching for all articles discussing vestibular schwannoma residuals and recurrences. Only articles discussing surgical treatment were included, focusing on studies which also examined facial nerve outcomes. A total of 51 articles were eligible for review and these included 375 patients. Statistical analysis was performed by correlating the following parameters: patients' gender and age at first surgery, surgical approach adopted at first and subsequent surgeries, tumor and residual size, and extent of resection (gross total, near total, subtotal or others) at first and subsequent surgical procedures. Facial nerve function was also analyzed focusing on its performance when correlated with the different surgical approaches. The data were analyzed by linear regression but there were no correlations between any of the parameters chosen. There was a statistically significant difference between the first approach used (mainly the retrosigmoid route) compared with subsequent approaches (mainly the translabyrinthine route). In total, 8.5 % of patients needed further treatment due to residual regrowth. Facial nerve outcome was independent of the parameters chosen. Exclusive surgical treatment for vestibular schwannoma residuals had a very low failure rate in terms of requiring further treatment. The approach usually chosen for second surgery was the translabyrinthine technique, and this may be explained by the location of the residual, rather than its size. The choice of a particular surgical approach rather than another had no influence on facial nerve function. Complications rates are comparable to Gamma Knife Radiosurgery's as reported in the literature
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