1,983 research outputs found

    Origin of electron-hole asymmetry in the scanning tunneling spectrum of Bi2Sr2CaCu2O8+δBi_2Sr_2CaCu_2O_{8+\delta}

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    We have developed a material specific theoretical framework for modelling scanning tunneling spectroscopy (STS) of high temperature superconducting materials in the normal as well as the superconducting state. Results for Bi2Sr2CaCu2O8+δBi_2Sr_2CaCu_2O_{8+\delta} (Bi2212) show clearly that the tunneling process strongly modifies the STS spectrum from the local density of states (LDOS) of the dx2y2d_{x^2-y^2} orbital of Cu. The dominant tunneling channel to the surface Bi involves the dx2y2d_{x^2-y^2} orbitals of the four neighbouring Cu atoms. In accord with experimental observations, the computed spectrum displays a remarkable asymmetry between the processes of electron injection and extraction, which arises from contributions of Cu dz2d_{z^2} and other orbitals to the tunneling current.Comment: 5 pages, 4 figures, published in PR

    Single-Dirac-Cone topological surface states in TlBiSe2 class of Topological Insulators

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    We have investigated several strong spin-orbit coupling ternary chalcogenides related to the (Pb,Sn)Te series of compounds. Our first-principles calculations predict the low temperature rhombohedral ordered phase in TlBiTe2, TlBiSe2, and TlSbX2 (X=Te, Se, S) to be topologically Kane-Mele Z2 = -1 nontrivial. We identify the specific surface termination that realizes the single Dirac cone through first-principles surface state computations. This termination minimizes effects of dangling bonds making it favorable for photoemission (ARPES) experiments. Our analysis predicts that thin films of these materials would harbor novel 2D quantum spin Hall states, and support odd-parity topological superconductivity. For a related work also see arXiv:1003.2615v1. Experimental ARPES results will be published elsewhere.Comment: Accepted for publication in Phys. Rev. Lett. (2010). Submitted March 201

    How different Fermi surface maps emerge in photoemission from Bi2212

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    We report angle-resolved photoemission spectra (ARPES) from the Fermi energy (EFE_F) over a large area of the (kx,kyk_x,k_y) plane using 21.2 eV and 32 eV photons in two distinct polarizations from an optimally doped single crystal of Bi2_2Sr2_2CaCu2_2O8+δ_{8+\delta} (Bi2212), together with extensive first-principles simulations of the ARPES intensities. The results display a wide-ranging level of accord between theory and experiment and clarify how myriad Fermi surface (FS) maps emerge in ARPES under various experimental conditions. The energy and polarization dependences of the ARPES matrix element help disentangle primary contributions to the spectrum due to the pristine lattice from those arising from modulations of the underlying tetragonal symmetry and provide a route for separating closely placed FS sheets in low dimensional materials.Comment: submitted to PR

    Induced superconductivity in noncuprate layers of the Bi2_2Sr2_2CaCu2_2O8+δ_{8+\delta} high-temperature superconductor: Modeling of scanning tunneling spectra

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    We analyze how the coherence peaks observed in Scanning Tunneling Spectroscopy (STS) of cuprate high temperature superconductors are transferred from the cuprate layer to the oxide layers adjacent to the STS microscope tip. For this purpose, we have carried out a realistic multiband calculation for the superconducting state of Bi2_2Sr2_2CaCu2_2O8+δ_{8+\delta} (Bi2212) assuming a short range d-wave pairing interaction confined to the nearest-neighbor Cu dx2y2d_{x^2-y^2} orbitals. The resulting anomalous matrix elements of the Green's function allow us to monitor how pairing is then induced not only within the cuprate bilayer but also within and across other layers and sites. The symmetry properties of the various anomalous matrix elements and the related selection rules are delineated.Comment: 9 pages, 2 figures. Accepted for publication in Phys. Rev.

    Structural, magnetic, dielectric and mechanical properties of (Ba,Sr)MnO3_3 ceramics

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    Ceramic samples, produced by conventional sintering method in ambient air, 6H-SrMnO3_3(6H-SMO), 15R-BaMnO3_3(15R-BMO), 4H-Ba0.5_{0.5}Sr0.5_{0.5}MnO3_3(4H-BSMO) were studied. In the XRD measurements for SMO the new anomalies of the lattice parameters at 600-800 K range and the increasing of thermal expansion coefficients with a clear maximum in a vicinity at 670 K were detected. The Neˊ\acute{e}el phase transition for BSMO was observed at TNT_N=250 K in magnetic measurements and its trace was detected in dielectric, FTIR, DSC, and DMA experiments. The enthalpy and entropy changes of the phase transition for BSMO at TNT_N were determined as 17.5 J/mol and 70 mJ/K mol, respectively. The activation energy values and relaxation times characteristic for relaxation processes were determined from the Arrhenius law. Results of ab initio simulations showed that the contribution of the exchange correlation energy to the total energy is about 30%.Comment: 12 pages, 12 figure

    Pinned Balseiro-Falicov Model of Tunneling and Photoemission in the Cuprates

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    The smooth evolution of the tunneling gap of Bi_2Sr_2CaCu_2O_8 with doping from a pseudogap state in the underdoped cuprates to a superconducting state at optimal and overdoping, has been interpreted as evidence that the pseudogap must be due to precursor pairing. We suggest an alternative explanation, that the smoothness reflects a hidden SO(N) symmetry near the (pi,0) points of the Brillouin zone (with N = 3, 4, 5, or 6). Because of this symmetry, the pseudogap could actually be due to any of a number of nesting instabilities, including charge or spin density waves or more exotic phases. We present a detailed analysis of this competition for one particular model: the pinned Balseiro-Falicov model of competing charge density wave and (s-wave) superconductivity. We show that most of the anomalous features of both tunneling and photoemission follow naturally from the model, including the smooth crossover, the general shape of the pseudogap phase diagram, the shrinking Fermi surface of the pseudogap phase, and the asymmetry of the tunneling gap away from optimal doping. Below T_c, the sharp peak at Delta_1 and the dip seen in the tunneling and photoemission near 2Delta_1 cannot be described in detail by this model, but we suggest a simple generalization to account for inhomogeneity, which does provide an adequate description. We show that it should be possible, with a combination of photoemission and tunneling, to demonstrate the extent of pinning of the Fermi level to the Van Hove singularity. A preliminary analysis of the data suggests pinning in the underdoped, but not in the overdoped regime.Comment: 18 pages LaTeX, 26 ps. figure
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