Binding energy and dephasing of biexcitons in In0.18Ga0.82As/GaAs single quantum wells

Biexciton binding energies and biexciton dephasing in In0.18Ga0.82As/GaAs single quantum wells have been measured by time-integrated and spectrally resolved four-wave mixing. The biexciton binding energy increases from 1.5 to 2.6 meV for well widths increasing from 1 to 4 nm. The ratio between exciton and biexciton binding energy changes from 0.23 to 0.3 with increasing inhomogeneous broadening, corresponding to increasing well width. From the temperature dependence of the exciton and biexciton four-wave mixing signal decay, we have deduced the acoustic-phonon scattering of the exciton-biexciton transition. It is found to be comparable to that of the exciton transition, indicating that the deformation potential interactions for the exciton and the exciton-biexciton transitions are comparable

Climatologies of streamer events derived from a transport model and a coupled chemistry-climate model

International audienceStreamers, i.e. finger-like structures, reach from lower into extra-tropical latitudes. They can be detected in N2O or O3 distributions on single lower stratospheric layers in mid-latitudes since they are characterised by high N2O or low O3 values compared to undisturbed mid-latitude values. If irreversible mixing occurs, streamer events significantly contribute to the transfer of tropical air masses to mid-latitudes which is also an exchange of upper tropospheric and stratospheric air. A climatology of streamer events has been established, employing the chemical-transport model KASIMA, which is driven by ECMWF re-analyses (ERA) and operational analyses. For the first time, the seasonal and the geographical distribution of streamer frequencies has been determined on the basis of 9 years of observations. For the current investigation, a meridional gradient criterion has been newly formulated and applied to the N2O distributions calculated with KASIMA. The climatology has been derived by counting all streamer events between 21 and 25 km for the years 1990 to 1998. It has been further used for the validation of a streamer climatology which has been established in the same way employing data of a multi-year simulation with the coupled chemistry-climate model ECHAM4.L39(DLR)/CHEM (E39/C). It turned out that both climatologies are qualitatively in fair agreement, in particular in the northern hemisphere, where much higher streamer frequencies are found in winter than in summer. In the southern hemisphere, KASIMA analyses indicate strongest streamer activity in September. E39/C streamer frequencies clearly offers an offset from June to October, pointing to model deficiencies with respect to tropospheric dynamics. KASIMA and E39/C results fairly agree from November to May. Some of the findings give strong indications that the streamer events found in the altitude region between 21 and 25 km are mainly forced from the troposphere and are not directly related to the dynamics of the stratosphere, in particular not to the dynamics of the polar vortex. Sensitivity simulations with E39/C, which represent recent and possible future atmospheric conditions, have been employed to answer the question how climate change would alter streamer frequencies. It is shown that the seasonal cycle does not change but that significant changes occur in months of minimum and maximum streamer frequencies. This could have an impact on mid-latitude distribution of chemical tracers and compounds. The influence of streamers on the mid-latitude ozone budget has been assessed by applying a special E39/C model configuration. The streamer transport of low ozone is simply inhibited by filling up its ozone content according to the surrounding air masses. It shows that the importance of streamers for the ozone budget strongly decreases with altitude. At 15 km streamers lead to a decrease of ozone by 80%, whereas around 25 km it is only 1 to 5% and at mid-latitude tropopause, ozone decreases by 30% (summer) to 50% (winter)

Physical Adsorption at the Nanoscale: Towards Controllable Scaling of the Substrate-Adsorbate van der Waals Interaction

The Lifshitz-Zaremba-Kohn (LZK) theory is commonly considered as the correct large-distance limit for the van der Waals (vdW) interaction of adsorbates (atoms, molecules, or nanoparticles) with solid substrates. In the standard approximate form, implicitly based on "local" dielectric functions, the LZK approach predicts universal power laws for vdW interactions depending only on the dimensionality of the interacting objects. However, recent experimental findings are challenging the universality of this theoretical approach at finite distances of relevance for nanoscale assembly. Here, we present a combined analytical and numerical many-body study demonstrating that physical adsorption can be significantly enhanced at the nanoscale. Regardless of the band gap or the nature of the adsorbate specie, we find deviations from conventional LZK power laws that extend to separation distances of up to 10--20 nanometers. Comparison with recent experimental observation of ultra long-ranged vdW interactions in the delamination of graphene from a silicon substrate reveals qualitative agreement with the present theory. The sensitivity of vdW interactions to the substrate response and to the adsorbate characteristic excitation frequency also suggests that adsorption strength can be effectively tuned in experiments, paving the way to an improved control of physical adsorption at the nanoscale

Casimir energy and entropy between dissipative mirrors

We discuss the Casimir effect between two identical, parallel slabs, emphasizing the role of dissipation and temperature. Starting from quite general assumptions, we analyze the behavior of the Casimir entropy in the limit T->0 and link it to the behavior of the slab's reflection coefficients at low frequencies. We also derive a formula in terms of a sum over modes, valid for dissipative slabs that can be interpreted in terms of a damped quantum oscillator.Comment: 8 pages, 1 figur

Retarded Casimir-Polder force on an atom near reflecting microstructures

We derive the fully retarded energy shift of a neutral atom in two different geometries useful for modelling etched microstructures. First we calculate the energy shift due to a reflecting cylindrical wire, and then we work out the energy shift due to a semi-infinite reflecting half-plane. We analyze the results for the wire in various limits of the wire radius and the distance of the atom from the wire, and obtain simple asymptotic expressions useful for estimates. For the half-plane we find an exact representation of the Casimir-Polder interaction in terms of a single, fast converging integral, which is easy to evaluate numerically.Comment: 12 pages, 8 figure

The Casimir Problem of Spherical Dielectrics: Numerical Evaluation for General Permittivities

The Casimir mutual free energy F for a system of two dielectric concentric nonmagnetic spherical bodies is calculated, at arbitrary temperatures. The present paper is a continuation of an earlier investigation [Phys. Rev. E {\bf 63}, 051101 (2001)], in which F was evaluated in full only for the case of ideal metals (refractive index n=infinity). Here, analogous results are presented for dielectrics, for some chosen values of n. Our basic calculational method stems from quantum statistical mechanics. The Debye expansions for the Riccati-Bessel functions when carried out to a high order are found to be very useful in practice (thereby overflow/underflow problems are easily avoided), and also to give accurate results even for the lowest values of l down to l=1. Another virtue of the Debye expansions is that the limiting case of metals becomes quite amenable to an analytical treatment in spherical geometry. We first discuss the zero-frequency TE mode problem from a mathematical viewpoint and then, as a physical input, invoke the actual dispersion relations. The result of our analysis, based upon the adoption of the Drude dispersion relation at low frequencies, is that the zero-frequency TE mode does not contribute for a real metal. Accordingly, F turns out in this case to be only one half of the conventional value at high temperatures. The applicability of the Drude model in this context has however been questioned recently, and we do not aim at a complete discussion of this issue here. Existing experiments are low-temperature experiments, and are so far not accurate enough to distinguish between the different predictions. We also calculate explicitly the contribution from the zero-frequency mode for a dielectric. For a dielectric, this zero-frequency problem is absent.Comment: 23 pages, LaTeX, 7 ps figures; expanded discussion, especially in Sec. 5. To appear in Phys. Rev.

A Tale of Two Fractals: The Hofstadter Butterfly and The Integral Apollonian Gaskets

This paper unveils a mapping between a quantum fractal that describes a physical phenomena, and an abstract geometrical fractal. The quantum fractal is the Hofstadter butterfly discovered in 1976 in an iconic condensed matter problem of electrons moving in a two-dimensional lattice in a transverse magnetic field. The geometric fractal is the integer Apollonian gasket characterized in terms of a 300 BC problem of mutually tangent circles. Both of these fractals are made up of integers. In the Hofstadter butterfly, these integers encode the topological quantum numbers of quantum Hall conductivity. In the Apollonian gaskets an infinite number of mutually tangent circles are nested inside each other, where each circle has integer curvature. The mapping between these two fractals reveals a hidden threefold symmetry embedded in the kaleidoscopic images that describe the asymptotic scaling properties of the butterfly. This paper also serves as a mini review of these fractals, emphasizing their hierarchical aspects in terms of Farey fractions

Casimir Force on Real Materials - the Slab and Cavity Geometry

We analyse the potential of the geometry of a slab in a planar cavity for the purpose of Casimir force experiments. The force and its dependence on temperature, material properties and finite slab thickness are investigated both analytically and numerically for slab and walls made of aluminium and teflon FEP respectively. We conclude that such a setup is ideal for measurements of the temperature dependence of the Casimir force. By numerical calculation it is shown that temperature effects are dramatically larger for dielectrics, suggesting that a dielectric such as teflon FEP whose properties vary little within a moderate temperature range, should be considered for experimental purposes. We finally discuss the subtle but fundamental matter of the various Green's two-point function approaches present in the literature and show how they are different formulations describing the same phenomenon.Comment: 24 pages, 11 figures; expanded discussion, one appendix added, 1 new figure and 10 new references. To appear in J. Phys. A: Math. Theo