7,216 research outputs found

    Focus on the impact of climate change on wetland ecosystem and carbon dynamics

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    The renewed growth in atmospheric methane (CH4)since 2007 after a decade of stabilization has drawn much attention to its causes and future trends. Wetlands are the single largest source of atmospheric CH4. Understanding wetland ecosystems and carbon dynamics is critical to the estimation of global CH4 and carbon budgets. After approximately 7 years of CH4 related research following the renewed growth in atmospheric CH4, Environmental Research Letters launched a special issue of research letters on wetland ecosystems and carbon dynamics in 2014. This special issue highlights recent developments in terrestrial ecosystem models and field measurements of carbon fluxes across different types of wetland ecosystems. The 14 research letters emphasize the importance of wetland ecosystems in the global CO2 and CH4 budget

    Spin current through an ESR quantum dot: A real-time study

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    The spin transport in a strongly interacting spin-pump nano-device is studied using the time-dependent variational-matrix-product-state (VMPS) approach. The precession magnetic field generates a dissipationless spin current through the quantum dot. We compute the real time spin current away from the equilibrium condition. Both transient and stationary states are reached in the simulation. The essentially exact results are compared with those from the Hartree-Fock approximation (HFA). It is found that correlation effect on the physical quantities at quasi-steady state are captured well by the HFA for small interaction strength. However the HFA misses many features in the real time dynamics. Results reported here may shed light on the understanding of the ultra-fast processes as well as the interplay of the non-equilibrium and strongly correlated effect in the transport properties.Comment: 5 pages, 5 figure

    Dimension Engineering of Single-Layer PtN2_2 with the Cairo Tessellation

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    Single-layer PtN2_2 exhibits an intriguing structure consisting of a tessellation pattern called the Cairo tessellation of type 2 pentagons, which belong to one of the existing 15 types of convex pentagons discovered so far that can monohedrally tile a plane. Single-layer PtN2_2 has also been predicted to show semiconducting behavior with direct band gaps. Full exploration of the structure-property relationship awaits the successful exfoliation or synthesis of this novel single-layer material, which depends on the structure of its bulk counterpart with the same stoichiometry to some extent. Bulk PtN2_2 with the pyrite structure is commonly regarded as the most stable structure in the literature. But comparing the energies of single-layer PtN2_2 and bulk PtN2_2 leads to a dilemma that a single-layer material is more stable than its bulk counterpart. To solve this dilemma, we propose stacking single-layer PtN2_2 sheets infinitely to form a new bulk structure of PtN2_2. The resulting tetrahedral layered structure is energetically more stable than the pyrite structure and single-layer PtN2_2. We also find that the predicted bulk structure is metallic, in contrast to the semiconducting pyrite structure. In addition to predicting the 3D structure, we explore the possibility of rolling single-layer PtN2_2 sheets into nanotubes. The required energies are comparable to those needed to form carbon or boron nitride nanotubes from their single-layer sheets, implying the feasibility of obtaining PtN2_2 nanotubes. We finally study the electronic structures of PtN2_2 nanotubes and find that the band gaps of PtN2_2 nanotubes are tunable by changing the number of unit cells NN of single-layer PtN2_2 used to construct the nanotubes. Our work shows that dimension engineering of PtN2_2 not only leads to a more stable 3D structure but also 1D materials with novel properties
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