Glass-like low frequency ac response of ZrB12_{12} and Nb single crystals in the surface superconducting state

We report experimental studies of the low frequency electrodynamics of ZrB$_{12}$ and Nb single crystals. AC susceptibility at frequencies 3 - 1000 Hz have been measured under a dc magnetic field, $H_0$, applied parallel to the sample surface. In the surface superconducting state, for several $H_0$, the real part of the ac magnetic susceptibility exhibits a logarithmic frequency dependence as for spin-glass systems. Kramers-Kronig analysis of the experimental data, shows large losses at ultra low frequencies ($<3$ Hz). The wave function slope at the surface was found. The linear response of the order parameter to the ac excitation was extracted from the experimental data.Comment: 9 pages, 12 figure

The internal magnetic field in superconducting ferromagnets

We have measured the nonlinear response to the ac magnetic field in the superconducting weak ferromagnet Ru-1222, at different regimes of sample cooling which provides unambiguous evidence of the interplay of the domain structure and the vorticity in the superconducting state. This is {\em direct} proof of coexistence of ferromagnetic and superconductive order parameters in high-$T_c$ ruthenocuprates.Comment: 9 pages, 6 figure

The low-frequency response in the surface superconducting state of ZrB12_{12} single crystal}

The large nonlinear response of a single crystal ZrB$_{12}$ to an ac field (frequency 40 - 2500 Hz) for $H_0>H_{c2}$ has been observed. Direct measurements of the ac wave form and the exact numerical solution of the Ginzburg-Landau equations, as well as phenomenological relaxation equation, permit the study of the surface superconducting states dynamics. It is shown, that the low frequency response is defined by transitions between the metastable superconducting states under the action of an ac field. The relaxation rate which determines such transitions dynamics, is found.Comment: 7 pages, 11 figure

Nonlinear magnetic response in ruthenocuprates

We have performed an investigation of the nonlinear magnetic response in ruthenocuprates. A negative, diverging-like peak at the main magnetic transition T_N in RuSr2RECu2O8 (RE = Gd, Y) indicates a possible canted antiferromagnetic order. Another well defined feature above T_N points to a blocking of superparamagnetic particles through the T^(-3) dependence of the third harmonic at higher temperatures. Below T_N a nondiverging peak appears, which is strongly affected by the addition of 10% of Cu ions in the RuO2 planes. In RuSr2RE(2-x)Ce(x)Cu2O10 the main magnetic transition T_M is accompanied by two characteristic temperatures in the third harmonic of the ac susceptibility, in agreement with recent studies from uSR and Mossbauer spectroscopy. We find that the spin-spin correlation temperature is the same in both families of ruthenocuprates.Comment: accepted for publication in EPJ

Tunable coaxial cavity resonator for linear and nonlinear microwave characterization of superconducting wires

We discuss experimental results obtained using a tunable cylindrical coaxial cavity constituted by an outer Cu cylinder and an inner Pb-BSCCO wire. We have used this device for investigating the microwave response of the superconducting wire, both in the linear and nonlinear regimes. In particular, by tuning the different modes of the cavity to make them resonant at exactly harmonic frequencies, we have detected the power emitted by the superconducting inner wire at the second- and third-harmonic frequency of the driving field. The results obtained in the nonlinear regime, whether for the microwave surface impedance or the harmonic emission, are qualitatively accounted for considering intergrain fluxon dynamics. The use of this kind of device can be of strong interest to investigate and characterise wires of large dimensions to be used for implementing superconducting-based microwave devices.Comment: 14 pages, 6 embedded figures, accepted for publication in Supercond. Sci. Techno

Complex spectral evolution in a BCS superconductor, ZrB12

We investigate the electronic structure of a complex conventional superconductor, ZrB12 employing high resolution photoemission spectroscopy and ab initio band structure calculations. The experimental valence band spectra could be described reasonably well within the local density approximation. Energy bands close to the Fermi level possess t2g symmetry and the Fermi level is found to be in the proximity of quantum fluctuation regime. The spectral lineshape in the high resolution spectra is complex exhibiting signature of a deviation from Fermi liquid behavior. A dip at the Fermi level emerges above the superconducting transition temperature that gradually grows with the decrease in temperature. The spectral simulation of the dip and spectral lineshape based on a phenomenological self energy suggests finite electron pair lifetime and a pseudogap above the superconducting transition temperature

Surface superconducting states in yttrium hexaboride single crystal in a tilted magnetic field

We present the results of an experimental study of the nucleation of superconductivity at the surface of a single crystal YB$_6$ in a tilted dc magnetic field. A recently developed experimental technique allowed us to determine $H_{c3}$ at each side of the sample as a function of the angle between the dc magnetic field and the surface. Experiment shows that the ratio $H_{c3}/ H_{c2}\approx 1.28$ in the direction perpendicular to the surface dc field while according to the theory this ratio should be equal to 1. This sharp distinction cannot be ascribed to the surface roughness.Comment: 6 pages, 8 figure