1,380 research outputs found
Isospectral Hamiltonians from Moyal products
Recently Scholtz and Geyer proposed a very efficient method to compute metric
operators for non-Hermitian Hamiltonians from Moyal products. We develop these
ideas further and suggest to use a more symmetrical definition for the Moyal
products, because they lead to simpler differential equations. In addition, we
demonstrate how to use this approach to determine the Hermitian counterpart for
a Pseudo-Hermitian Hamiltonian. We illustrate our suggestions with the
explicitly solvable example of the -x^4-potential and the ubiquitous harmonic
oscillator in a complex cubic potential.Comment: 10 pages, to appear special issue Czech. J. Phy
Coulomb-free and Coulomb-distorted recolliding quantum orbits in photoelectron holography
We perform a detailed analysis of the different types of orbits in the
Coulomb Quantum Orbit Strong-field Approximation (CQSFA), ranging from direct
to those undergoing hard collisions. We show that some of them exhibit clear
counterparts in the standard formulations of the strong-field approximation for
direct and rescattered above-threshold ionization, and show that the standard
orbit classification commonly used in Coulomb-corrected models is
over-simplified. We identify several types of rescattered orbits, such as those
responsible for the low-energy structures reported in the literature, and
determine the momentum regions in which they occur. We also find formerly
overlooked interference patterns caused by backscattered, Coulomb-corrected
orbits and assess their effect on photoelectron angular distributions. These
orbits improves the agreement of photoelectron angular distributions computed
with the CQSFA with the outcome of ab-initio methods for high-energy
phtotoelectrons perpendicular to the field-polarization axis.Comment: 19 pages, 9 figure
Multielectron corrections in molecular high-order harmonic generation for different formulations of the strong-field approximation
We make a detailed assessment of which form of the dipole operator to use in
calculating high order harmonic generation within the framework of the strong
field approximation, and look specifically at the role the form plays in the
inclusion of multielectron effects perturbatively with regard to the
contributions of the highest occupied molecular orbital. We focus on how these
corrections affect the high-order harmonic spectra from aligned homonuclear and
heteronuclear molecules, exemplified by and CO, respectively,
which are isoelectronic. We find that the velocity form incorrectly finds zero
static dipole moment in heteronuclear molecules. In contrast, the length form
of the dipole operator leads to the physically expected non-vanishing
expectation value for the dipole operator in this case. Furthermore, the so
called "overlap" integrals, in which the dipole matrix element is computed
using wavefunctions at different centers in the molecule, are prominent in the
first-order multielectron corrections for the velocity form, and should not be
ignored. Finally, inclusion of the multielectron corrections has very little
effect on the spectrum. This suggests that relaxation, excitation and the
dynamic motion of the core are important in order to describe multielectron
effects in molecular high-order high harmonic generation.Comment: Figures 2 and 4 have been simplified in order to fulfil the size
requirements of arXiv; in the new version references have been adde
Excitation, two-center interference and the orbital geometry in laser-induced nonsequential double ionization of diatomic molecules
We address the influence of the molecular orbital geometry and of the
molecular alignment with respect to the laser-field polarization on
laser-induced nonsequential double ionization of diatomic molecules for
different molecular species, namely and . We
focus on the recollision excitation with subsequent tunneling ionization (RESI)
mechanism, in which the first electron, upon return, promotes the second
electron to an excited state, from where it subsequently tunnels. We show that
the electron-momentum distributions exhibit interference maxima and minima due
to the electron emission at spatially separated centers. We provide generalized
analytical expressions for such maxima or minima, which take into account
mixing and the orbital geometry. The patterns caused by the two-center
interference are sharpest for vanishing alignment angle and get washed out as
this parameter increases. Apart from that, there exist features due to the
geometry of the lowest occupied molecular orbital (LUMO), which may be observed
for a wide range of alignment angles. Such features manifest themselves as the
suppression of probability density in specific momentum regions due to the
shape of the LUMO wavefunction, or as an overall decrease in the RESI yield due
to the presence of nodal planes.Comment: 11 pages revtex, 2 figure
Existence criteria for stabilization from the scaling behaviour of ionization probabilities
We provide a systematic derivation of the scaling behaviour of various
quantities and establish in particular the scale invariance of the ionization
probability. We discuss the gauge invariance of the scaling properties and the
manner in which they can be exploited as consistency check in explicit
analytical expressions, in perturbation theory, in the Kramers-Henneberger and
Floquet approximation, in upper and lower bound estimates and fully numerical
solutions of the time dependent Schroedinger equation. The scaling invariance
leads to a differential equation which has to be satisfied by the ionization
probability and which yields an alternative criterium for the existence of
atomic bound state stabilization.Comment: 12 pages of Latex, one figur
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