6,661 research outputs found

    Doping - dependent superconducting gap anisotropy in the two-dimensional 10-3-8 pnictide Ca10_{10}(Pt3_3As8_8)[(Fe1x_{1-x}Ptx_{x})2_2As2_2]5_5

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    The characteristic features of Ca10_{10}(Pt3_3As8_8)[(Fe1x_{1-x}Ptx_x)2_2As2_2]5_5 ("10-3-8") superconductor are relatively high anisotropy and a clear separation of superconductivity and structural/magnetic transitions, which allows studying the superconducting gap without complications due to the coexisting order parameters. The London penetration depth, measured in underdoped single crystals of 10-3-8 (x=x = 0.028, 0.041, 0.042, and 0.097), shows behavior remarkably similar to other Fe-based superconductors, exhibiting robust power-law, Δλ(T)=ATn\Delta \lambda(T) = A T^n. The exponent nn decreases from 2.36 (x=x = 0.097, close to optimal doping) to 1.7 (x=x = 0.028, a heavily underdoped composition), suggesting that the superconducting gap becomes more anisotropic at the dome edge. A similar trend is found in low-anisotropy superconductors based on BaFe2_2As2_2 ("122"), implying that it is an intrinsic property of superconductivity in iron pnictides, unrelated to the coexistence of magnetic order and superconductivity or the anisotropy of the normal state. Overall this doping dependence is consistent with s±s_{\pm} pairing competing with intra-band repulsion

    Electronic structure of warm dense copper studied by ultrafast x-ray absorption spectroscopy

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    We use time-resolved x-ray absorption spectroscopy to investigate the unoccupied electronic density of states of warm dense copper that is produced isochorically through the absorption of an ultrafast optical pulse. The temperature of the superheated electron-hole plasma, which ranges from 4000 to 10 000 K, was determined by comparing the measured x-ray absorption spectrum with a simulation. The electronic structure of warm dense copper is adequately described with the high temperature electronic density of state calculated by the density functional theory. The dynamics of the electron temperature is consistent with a two-temperature model, while a temperature-dependent electron-phonon coupling parameter is necessary

    Core repulsion effects in alkali trimers

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    The present paper is related to a talk presented during the Symposium on Coherent Control and Ultracold Chemistry held during the Sixth Congress of the International Society for Theoretical Chemical Physics (ISTCP-VI, July 2008). The talk was entitled "Electronic structure properties of alkali dimers and trimers. Prospects for alignment of ultracold molecules". Here we report on the electrostatic repulsion forces of the ionic cores at short separation, involved when the potential energy surfaces of alkali trimers are calculated with a quantum chemistry approach based on effective large-core potentials for ionic core description. We demonstrate that such forces in the triatomic molecule can be obtained as the sum of three pairwise terms. We illustrate our results on the lowest electronic states of Cs3_3, which are computed for the first time within a full configuration interaction based on a large Gaussian basis set. As a preliminary section, we also propose a brief introduction about the importance of alkali trimer systems in the context of cold and ultracold molecules

    Dysregulated protocadherin-pathway activity as an intrinsic defect in induced pluripotent stem cell-derived cortical interneurons from subjects with schizophrenia.

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    We generated cortical interneurons (cINs) from induced pluripotent stem cells derived from 14 healthy controls and 14 subjects with schizophrenia. Both healthy control cINs and schizophrenia cINs were authentic, fired spontaneously, received functional excitatory inputs from host neurons, and induced GABA-mediated inhibition in host neurons in vivo. However, schizophrenia cINs had dysregulated expression of protocadherin genes, which lie within documented schizophrenia loci. Mice lacking protocadherin-α showed defective arborization and synaptic density of prefrontal cortex cINs and behavioral abnormalities. Schizophrenia cINs similarly showed defects in synaptic density and arborization that were reversed by inhibitors of protein kinase C, a downstream kinase in the protocadherin pathway. These findings reveal an intrinsic abnormality in schizophrenia cINs in the absence of any circuit-driven pathology. They also demonstrate the utility of homogenous and functional populations of a relevant neuronal subtype for probing pathogenesis mechanisms during development

    Supramolecular assemblies involving metal organic ring interactions: Heterometallic Cu(II)-Ln(III) two dimensional coordination polymers

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    Three isostructural two-dimensional coordination polymers of the general formula [Ln2(CuL)3(H2O)9]$5.5H2O, where Ln is La (1), Nd (2), and Gd (3), have been synthesized and isolated from aqueous solutions and their single-crystal structures determined by X-ray diffraction. The supramolecular interaction between the non-aromatic metallorings plays an important role in stabilizing the structure of these compounds. The thermal stability, reversible solvent uptake, electronic properties and magnetic studies of these compounds are also reported

    The Ionotropic Receptors IR21a and IR25a mediate cool sensing in Drosophila.

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    Animals rely on highly sensitive thermoreceptors to seek out optimal temperatures, but the molecular mechanisms of thermosensing are not well understood. The Dorsal Organ Cool Cells (DOCCs) of the Drosophila larva are a set of exceptionally thermosensitive neurons critical for larval cool avoidance. Here, we show that DOCC cool-sensing is mediated by Ionotropic Receptors (IRs), a family of sensory receptors widely studied in invertebrate chemical sensing. We find that two IRs, IR21a and IR25a, are required to mediate DOCC responses to cooling and are required for cool avoidance behavior. Furthermore, we find that ectopic expression of IR21a can confer cool-responsiveness in an Ir25a-dependent manner, suggesting an instructive role for IR21a in thermosensing. Together, these data show that IR family receptors can function together to mediate thermosensation of exquisite sensitivity

    Droplet-like Fermi surfaces in the anti-ferromagnetic phase of EuFe2_2As2_2, an Fe-pnictide superconductor parent compound

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    Using angle resolved photoemission it is shown that the low lying electronic states of the iron pnictide parent compound EuFe2_2As2_2 are strongly modified in the magnetically ordered, low temperature, orthorhombic state compared to the tetragonal, paramagnetic case above the spin density wave transition temperature. Back-folded bands, reflected in the orthorhombic/ anti-ferromagnetic Brillouin zone boundary hybridize strongly with the non-folded states, leading to the opening of energy gaps. As a direct consequence, the large Fermi surfaces of the tetragonal phase fragment, the low temperature Fermi surface being comprised of small droplets, built up of electron and hole-like sections. These high resolution ARPES data are therefore in keeping with quantum oscillation and optical data from other undoped pnictide parent compounds.Comment: 4 figures, 6 page

    Even and odd q-deformed charge coherent states and their nonclassical properties

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    Even and odd q-deformed charge coherent states are constructed, their (over)completeness proved and their generation explored. A DD-algebra realization of the SUq_q(1,1) generators is given in terms of them. They are shown to exhibit SUq_q(1,1) squeezing and two-mode qq-antibunching, but neither one-mode, nor two-mode qq-squeezing.Comment: LaTeX, 23 pages, no figure, minor changes, final version to be published in PL
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