Frequency response of an atomic resonance driven by weak free-electron-laser fluctuating pulses

Motivated by recent experiments pertaining to the interaction of weak SASE-FEL pulses with atoms and molecules, we investigate the conditions under which such interactions can be described in the framework of a simple phase-diffusion model with decorrelated atom-field dynamics. The nature of the fluctuations that are inevitably present in SASE-FEL pulses is shown to play a pivotal role in the success of the decorrelation. Our analysis is performed in connection with specific recent experimental results from FLASH in the soft X-ray regime.Comment: arXiv admin note: substantial text overlap with arXiv:1209.223

Multiple Ionization under Strong XUV to X-ray Radiation

We review the main aspects of multiple photoionization processes in atoms exposed to intense, short wavelength radiation. The main focus is the theoretical framework for the description of such processes as well as the conditions under which direct multiphoton multiple ionization processes can dominate over the sequential ones. We discuss in detail the mechanisms available in different wavelength ranges from the infrared to the hard X-rays. The effect of field fluctuations, present at this stage in all SASE free-electron-laser (FEL) facilities, as well as the effect of the interaction volume integration, are also discussed