1,396 research outputs found

    Spin Dynamics in Cuprates: Optical Conductivity of HgBa2CuO4

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    The electron-boson spectral density function I^2ChiOmega responsible for carrier scattering of the high temperature superconductor HgBa2CuO4 (Tc = 90 K) is calculated from new data on the optical scattering rate. A maximum entropy technique is used. Published data on HgBa2Ca2Cu3O8 (Tc = 130 K) are also inverted and these new results are put in the context of other known cases. All spectra (with two notable exceptions) show a peak at an energy (Omega_r) proportional to the superconducting transition temperature Omega_r ~= 6.3 kB.Tc. This charge channel relationship follows closely the magnetic resonance seen by polarized neutron scattering, Omega_r^{neutron} ~= 5.4 kB.Tc. The amplitudes of both peaks decrease strongly with increasing temperature. In some cases, the peak at Omega_r is weak and the spectrum can have additional maxima and a background extending up to several hundred meV

    Angle-resolved photoemission study of the role of nesting and orbital orderings in the antiferromagnetic phase of BaFe2As2

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    We present a detailed comparison of the electronic structure of BaFe2As2 in its paramagnetic and antiferromagnetic (AFM) phases, through angle-resolved photoemission studies. Using different experimental geometries, we resolve the full elliptic shape of the electron pockets, including parts of dxy symmetry along its major axis that are usually missing. This allows us to define precisely how the hole and electron pockets are nested and how the different orbitals evolve at the transition. We conclude that the imperfect nesting between hole and electron pockets explains rather well the formation of gaps and residual metallic droplets in the AFM phase, provided the relative parity of the different bands is taken into account. Beyond this nesting picture, we observe shifts and splittings of numerous bands at the transition. We show that the splittings are surface sensitive and probably not a reliable signature of the magnetic order. On the other hand, the shifts indicate a significant redistribution of the orbital occupations at the transition, especially within the dxz/dyz system, which we discuss

    Highly efficient multilayer organic pure-blue-light emitting diodes with substituted carbazoles compounds in the emitting layer

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    Bright blue organic light-emitting diodes (OLEDs) based on 1,4,5,8,N-pentamethylcarbazole (PMC) and on dimer of N-ethylcarbazole (N,N'-diethyl-3,3'-bicarbazyl) (DEC) as emitting layers or as dopants in a 4,4'-bis(2,2'-diphenylvinyl)-1,1'-biphenyl (DPVBi) matrix are described. Pure blue-light with the C.I.E. coordinates x = 0.153 y = 0.100, electroluminescence efficiency \eta_{EL} of 0.4 cd/A, external quantum efficiency \eta_{ext.} of 0.6% and luminance L of 236 cd/m2 (at 60 mA/cm2) were obtained with PMC as an emitter and the 2,9-dimethyl-4,7-diphenyl-1,10-phenantroline (BCP) as a hole-blocking material in five-layer emitting devices. The highest efficiencies \eta_{EL.} of 4.7 cd/A, and \eta_{ext} = 3.3% were obtained with a four-layer structure and a DPVBi DEC-doped active layer (CIE coordinates x = 0.158, y=0.169, \lambda_{peak} = 456 nm). The \eta_{ext.} value is one the highest reported at this wavelength for blue OLEDs and is related to an internal quantum efficiency up to 20%

    Significant reduction of electronic correlations upon isovalent Ru substitution of BaFe2As2

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    We present a detailed investigation of Ba(Fe0.65Ru0.35)2As2 by transport measurements and Angle Resolved photoemission spectroscopy. We observe that Fe and Ru orbitals hybridize to form a coherent electronic structure and that Ru does not induce doping. The number of holes and electrons, deduced from the area of the Fermi Surface pockets, are both about twice larger than in BaFe2As2. The contribution of both carriers to the transport is evidenced by a change of sign of the Hall coefficient with decreasing temperature. Fermi velocities increase significantly with respect to BaFe2As2, suggesting a significant reduction of correlation effects. This may be a key to understand the appearance of superconductivity at the expense of magnetism in undoped iron pnictides

    Optical signature of sub-gap absorption in the superconducting state of Ba(Fe,Co)2As2

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    The optical conductivity of Ba(Fe0.92_{0.92}Co0.08_{0.08})2_2As2_2 shows a clear signature of the superconducting gap, but a simple ss-wave description fails in accounting for the low frequency response. This task is achieved by introducing an extra Drude peak in the superconducting state representing sub-gap absorption, other than thermally broken pairs. This extra peak and the coexisting ss-wave response respect the total sum rule indicating a common origin for the carriers. We discuss the possible origins for this absorption as (i) quasiparticles due to pair-breaking from interband impurity scattering in a two band s±s_{\pm} gap symmetry model, which includes (ii) the possible existence of impurity levels within an isotropic gap model; or (iii) an indication that one of the bands is highly anisotropic.Comment: 5 pages, 4 figure

    Incommensurate spin density wave in Co-doped BaFe2As2

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    57Fe Mossbauer spectroscopy measurements are presented in the underdoped Ba(Fe{1-x}Cox)2As2 series for x=0.014 (T_c < 1.4K) and x=0.03 and 0.045 (T_c ~ 2 and 12K respectively). The spectral shapes in the so-called spin-density wave (SDW) phase are interpreted in terms of incommensurate modulation of the magnetic structure, and allow the shape of the modulation to be determined. In undoped BaFe2As2, the magnetic structure is commensurate, and we find that incommensurability is present at the lowest doping level (x=0.014). As Co doping increases, the low temperature modulation progressively loses its "squaredness" and tends to a sine-wave. The same trend occurs for a given doping level, as temperature increases. We find that a magnetic hyperfine component persists far above the SDW transition, its intensity being progressively tranferred to a paramagnetic component on heating.Comment: 7 pages, 8 figures, published in EP
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