5,526 research outputs found

    Competing charge density waves and temperature-dependent nesting in 2H-TaSe2

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    Multiple charge density wave (CDW) phases in 2H-TaSe2 are investigated by high-resolution synchrotron x-ray diffraction. In a narrow temperature range immediately above the commensurate CDW transition, we observe a multi-q superstructure with coexisting commensurate and incommensurate order parameters, clearly distinct from the fully incommensurate state at higher temperatures. This multi-q ordered phase, characterized by a temperature hysteresis, is found both during warming and cooling, in contrast to previous reports. In the normal state, the incommensurate superstructure reflection gives way to a broad diffuse peak that persists nearly up to room temperature. Its position provides a direct and accurate estimate of the Fermi surface nesting vector, which evolves non-monotonically and approaches the commensurate position as the temperature is increased. This behavior agrees with our recent observations of the temperature-dependent Fermi surface in the same compound [Phys. Rev. B 79, 125112 (2009)]

    Ultrafast photodoping and effective Fermi-Dirac distribution of the Dirac particles in Bi2Se3

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    We exploit time- and angle- resolved photoemission spectroscopy to determine the evolution of the out-of-equilibrium electronic structure of the topological insulator Bi2Se. The response of the Fermi-Dirac distribution to ultrashort IR laser pulses has been studied by modelling the dynamics of the hot electrons after optical excitation. We disentangle a large increase of the effective temperature T* from a shift of the chemical potential mu*, which is consequence of the ultrafast photodoping of the conduction band. The relaxation dynamics of T* and mu* are k-independent and these two quantities uniquely define the evolution of the excited charge population. We observe that the energy dependence of the non-equilibrium charge population is solely determined by the analytical form of the effective Fermi-Dirac distribution.Comment: 5 Pages, 3 Figure

    Atomic and Electronic Structure of a Rashba pp-nn Junction at the BiTeI Surface

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    The non-centrosymmetric semiconductor BiTeI exhibits two distinct surface terminations that support spin-split Rashba surface states. Their ambipolarity can be exploited for creating spin-polarized pp-nn junctions at the boundaries between domains with different surface terminations. We use scanning tunneling microscopy/spectroscopy (STM/STS) to locate such junctions and investigate their atomic and electronic properties. The Te- and I-terminated surfaces are identified owing to their distinct chemical reactivity, and an apparent height mismatch of electronic origin. The Rashba surface states are revealed in the STS spectra by the onset of a van Hove singularity at the band edge. Eventually, an electronic depletion is found on interfacial Te atoms, consistent with the formation of a space charge area in typical pp-nn junctions.Comment: 5 pages, 4 figure

    Ultrafast Optical Control of the Electronic Properties of ZrTe5ZrTe_5

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    We report on the temperature dependence of the ZrTe5ZrTe_5 electronic properties, studied at equilibrium and out of equilibrium, by means of time and angle resolved photoelectron spectroscopy. Our results unveil the dependence of the electronic band structure across the Fermi energy on the sample temperature. This finding is regarded as the dominant mechanism responsible for the anomalous resistivity observed at T* \sim 160 K along with the change of the charge carrier character from holelike to electronlike. Having addressed these long-lasting questions, we prove the possibility to control, at the ultrashort time scale, both the binding energy and the quasiparticle lifetime of the valence band. These experimental evidences pave the way for optically controlling the thermoelectric and magnetoelectric transport properties of ZrTe5ZrTe_5

    Establishing the fundamental magnetic interactions in the chiral skyrmionic Mott insulator Cu2OSeO3 by terahertz electron spin resonance

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    The recent discovery of skyrmions in Cu2_2OSeO3_3 has established a new platform to create and manipulate skyrmionic spin textures. We use high-field electron spin resonance (ESR) spectroscopy combining a terahertz free electron laser and pulsed magnetic fields up to 64 T to probe and quantify its microscopic spin-spin interactions. Besides providing direct access to the long-wavelength Goldstone mode, this technique probes also the high-energy part of the excitation spectrum which is inaccessible by standard low-frequency ESR. Fitting the behavior of the observed modes in magnetic field to a theoretical framework establishes experimentally that the fundamental magnetic building blocks of this skyrmionic magnet are rigid, highly entangled and weakly coupled tetrahedra.Comment: 5 pages, 3 Figure

    Giant ambipolar Rashba effect in a semiconductor: BiTeI

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    We observe a giant spin-orbit splitting in bulk and surface states of the non-centrosymmetric semiconductor BiTeI. We show that the Fermi level can be placed in the valence or in the conduction band by controlling the surface termination. In both cases it intersects spin-polarized bands, in the corresponding surface depletion and accumulation layers. The momentum splitting of these bands is not affected by adsorbate-induced changes in the surface potential. These findings demonstrate that two properties crucial for enabling semiconductor-based spin electronics -- a large, robust spin splitting and ambipolar conduction -- are present in this material.Comment: 4 pages, 3 figure

    Ballistic versus diffusive magnetoresistance of a magnetic point contact

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    The quasiclassical theory of a nanosize point contacts (PC) between two ferromagnets is developed. The maximum available magnetoresistance values in PC are calculated for ballistic versus diffusive transport through the area of a contact. In the ballistic regime the magnetoresistance in excess of few hundreds percents is obtained for the iron-group ferromagnets. The necessary conditions for realization of so large magnetoresistance in PC, and the experimental results by Garcia et al are discussedComment: 4 pages, TEX, 1 Figur

    The momentum and photon energy dependence of the circular dichroic photoemission in the bulk Rashba semiconductors BiTeX (X = I, Br, Cl)

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    Bulk Rashba systems BiTeX (X = I, Br, Cl) are emerging as important candidates for developing spintronics devices, because of the coexistence of spin-split bulk and surface states, along with the ambipolar character of the surface charge carriers. The need of studying the spin texture of strongly spin-orbit coupled materials has recently promoted circular dichroic Angular Resolved Photoelectron Spectroscopy (cd-ARPES) as an indirect tool to measure the spin and the angular degrees of freedom. Here we report a detailed photon energy dependent study of the cd-ARPES spectra in BiTeX (X = I, Br and Cl). Our work reveals a large variation of the magnitude and sign of the dichroism. Interestingly, we find that the dichroic signal modulates differently for the three compounds and for the different spin-split states. These findings show a momentum and photon energy dependence for the cd-ARPES signals in the bulk Rashba semiconductor BiTeX (X = I, Br, Cl). Finally, the outcome of our experiment indicates the important relation between the modulation of the dichroism and the phase differences between the wave-functions involved in the photoemission process. This phase difference can be due to initial or final state effects. In the former case the phase difference results in possible interference effects among the photo-electrons emitted from different atomic layers and characterized by entangled spin-orbital polarized bands. In the latter case the phase difference results from the relative phases of the expansion of the final state in different outgoing partial waves.Comment: 6 pages, 4 figure

    Momentum resolved spin dynamics of bulk and surface excited states in the topological insulator Bi2Se3\mathrm{Bi_{2}Se_{3}}

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    The prospective of optically inducing a spin polarized current for spintronic devices has generated a vast interest in the out-of-equilibrium electronic and spin structure of topological insulators (TIs). In this Letter we prove that only by measuring the spin intensity signal over several order of magnitude in spin, time and angle resolved photoemission spectroscopy (STAR-PES) experiments is it possible to comprehensively describe the optically excited electronic states in TIs materials. The experiments performed on Bi2Se3\mathrm{Bi_{2}Se_{3}} reveal the existence of a Surface-Resonance-State in the 2nd bulk band gap interpreted on the basis of fully relativistic ab-initio spin resolved photoemission calculations. Remarkably, the spin dependent relaxation of the hot carriers is well reproduced by a spin dynamics model considering two non-interacting electronic systems, derived from the excited surface and bulk states, with different electronic temperatures.Comment: 5 pages and 4 figure

    Hadronic WW production and the Gottfried Sum Rule

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    The difference in production rate between W+W^+ and WW^- at hadron colliders is very sensitive to the the difference between up- and down-quark distributions in the proton. This sensitivity allows for a variety of useful measurements. We consider the difference ds(x,Q2)us(x,Q2)d_s(x,Q^2) - u_s(x,Q^2) in the sea distributions and the difference Δu(x,Q2)Δd(x,Q2)\Delta u(x,Q^2) - \Delta d(x,Q^2) in the polarized parton distribution functions. In both cases we construct an asymmetry to reduce systematic uncertainties. Although we discuss measurements at the Tevatron and future hadron colliders, we find that the Brookhaven Relativistic Heavy Ion Collider (RHIC) is the most appropriate hadron collider for these measurements.Comment: 19 pages (20 figures available from the authors), MAD/PH/74
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