Emission Noise and High Frequency Cut-Off of the Kondo Effect in a Quantum Dot

By coupling on chip a carbon nanotube to a quantum noise detector, a superconductor-insulator-superconductor junction, via a resonant circuit, we measure the emission noise of a carbon nanotube quantum dot in the Kondo regime. The signature of the Kondo effect in the current noise is measured for different ratios of the Kondo temperature over the measured frequency and for different asymmetries of the coupling to the contacts, and compared to finite frequency quantum noise calculations. Our results point towards the existence of a high frequency cut-off of the electronic emission noise associated with the Kondo resonance. This cut-off frequency is of the order of a few times the Kondo temperature when the electronic system is close to equilibrium, which is the case for a strongly asymmetric coupling. On the other hand, this cut-off is shifted to lower frequency in a symmetric coupling situation, where the bias voltage drives the Kondo state out-of-equilibrium. We then attribute the low frequency cut-off to voltage induced spin relaxation.Comment: 5 pages, 3 figures and appendi

Measurements of flux dependent screening in Aharonov-Bohm rings

In order to investigate the effect of electronic phase coherence on screening we have measured the flux dependent polarizability of isolated mesoscopic rings at 350 MHz. At low temperature (below 100 mK) both non-dissipative and dissipative parts of the polarizability exhibit flux oscillations with a period of half a flux quantum in a ring. The sign and amplitude of the effect are in good agreement with recent theoretical predictions. The observed positive magneto-polarizability corresponds to an enhancement of screening when time reversal symmetry is broken. The effect of electronic density and temperature are also measured.Comment: 4 pages, revtex, 4 figures, to appear in Phys. Rev. Let

Detection of Quantum Noise from an Electrically-Driven Two-Level System

Quantum mechanics can strongly influence the noise properties of mesoscopic devices. To probe this effect we have measured the current fluctuations at high-frequency (5-90 GHz) using a superconductor-insulator-superconductor tunnel junction as an on-chip spectrum analyser. By coupling this frequency-resolved noise detector to a quantum device we can measure the high-frequency, non-symmetrized noise as demonstrated for a Josephson junction. The same scheme is used to detect the current fluctuations arising from coherent charge oscillations in a two-level system, a superconducting charge qubit. A narrow band peak is observed in the spectral noise density at the frequency of the coherent charge oscillations.Comment: 16 pages, 4 figure

Manipulating the magnetic state of a carbon nanotube Josephson junction using the superconducting phase

The magnetic state of a quantum dot attached to superconducting leads is experimentally shown to be controlled by the superconducting phase difference across the dot. This is done by probing the relation between the Josephson current and the superconducting phase difference of a carbon nanotube junction whose Kondo energy and superconducting gap are of comparable size. It exhibits distinctively anharmonic behavior, revealing a phase mediated singlet to doublet transition. We obtain an excellent quantitative agreement with numerically exact quantum Monte Carlo calculations. This provides strong support that we indeed observed the finite temperature signatures of the phase controlled zero temperature level-crossing transition originating from strong local electronic correlations.Comment: 5 pages, 4 figures + supp. material

0-π\pi quantum transition in a carbon nanotube Josephson junction: universal phase dependence and orbital degeneracy

We investigate experimentally the supercurrent in a clean carbon nanotube quantum dot, close to orbital degeneracy, connected to superconducting leads in a regime of strong competition between local electronic correlations and superconducting proximity effect. For an odd occupancy of the dot and intermediate coupling to the reservoir, the Kondo effect can develop in the normal state and screen the local magnetic moment of the dot. This leads to singlet-doublet transitions that strongly affect the Josephson effect in a single-level quantum dot: the sign of the supercurrent changes from positive to negative (0 to $\pi$-junction). In the regime of strongest competition between the Kondo effect and proximity effect, meaning that the Kondo temperature equals the superconducting gap, the magnetic state of the dot undergoes a first order quantum transition induced by the superconducting phase difference across the junction. This is revealed experimentally by anharmonic current-phase relations. In addition, the very specific electronic configuration of clean carbon nanotubes, with two nearly orbitally degenerated states, leads to different physics depending whether only one or both quasi-degenerate upper levels of the dots participate to transport, which is determined by their occupancy and relative widths. When the transport of Cooper pairs takes place through only one of these levels, we find that the phase diagram of the phase-dependent 0-$\pi$ transition is a universal characteristic of a discontinuous level-crossing quantum transition at zero temperature. In the case were two levels participate to transport, the nanotube Josephson current exhibits a continuous 0-$\pi$ transition, independent of the superconducting phase, revealing a different physical mechanism of the transition.Comment: 14 pages, 12 figure

High Frequency Quantum Admittance and Noise Measurement with an On-chip Resonant Circuit

By coupling a quantum detector, a superconductor-insulator-superconductor junction, to a Josephson junction \textit{via} a resonant circuit we probe the high frequency properties, namely the ac complex admittance and the current fluctuations of the Josephson junction at the resonant frequencies. The admittance components show frequency dependent singularities related to the superconducting density of state while the noise exhibits a strong frequency dependence, consistent with theoretical predictions. The circuit also allows to probe separately the emission and absorption noise in the quantum regime of the superconducting resonant circuit at equilibrium. At low temperature the resonant circuit exhibits only absorption noise related to zero point fluctuations, whereas at higher temperature emission noise is also present.Comment: 15 pages, 15 figure

Tuning the Josephson current in carbon nanotubes with the Kondo effect

We investigate the Josephson current in a single wall carbon nanotube connected to superconducting electrodes. We focus on the parameter regime in which transport is dominated by Kondo physics. A sizeable supercurrent is observed for odd number of electrons on the nanotube when the Kondo temperature Tk is sufficiently large compared to the superconducting gap. On the other hand when, in the center of the Kondo ridge, Tk is slightly smaller than the superconducting gap, the supercurrent is found to be extremely sensitive to the gate voltage Vbg. Whereas it is largely suppressed at the center of the ridge, it shows a sharp increase at a finite value of Vbg. This increase can be attributed to a doublet-singlet transition of the spin state of the nanotube island leading to a pi shift in the current phase relation. This transition is very sensitive to the asymmetry of the contacts and is in good agreement with theoretical predictions.Comment: 5 pages, 4 figure

Magneto-polarisability of mesoscopic systems

In order to understand how screening is modified by electronic interferences in a mesoscopic isolated system, we have computed both analytically and numerically the average thermodynamic and time dependent polarisabilities of two dimensional mesoscopic samples in the presence of an Aharonov-Bohm flux. Two geometries have been considered: rings and squares. Mesoscopic correction to screening are taken into account in a self consistent way, using the response function formalism. The role of the statistical ensemble (canonical and grand canonical), disorder and frequency have been investigated. We have also computed first order corrections to the polarisability due to electron-electron interactions. Our main results concern the diffusive regime. In the canonical ensemble, there is no flux dependence polarisability when the frequency is smaller than the level spacing. On the other hand, in the grand canonical ensemble for frequencies larger than the mean broadening of the energy levels (but still small compared to the level spacing), the polarisability oscillates with flux, with the periodicity $h/2e$. The order of magnitude of the effect is given by $\delta \alpha/\alpha \propto (\lambda_s/Wg)$, where $\lambda$ is the Thomas Fermi screening length, $W$ the width of the rings or the size of the squares and $g$ their average dimensionless conductance. This magnetopolarisability of Aharonov-Bohm rings has been recently measured experimentally \cite{PRL_deblock00} and is in good agreement with our grand canonical result.Comment: 12 pages, 10 figures, revte