1,370 research outputs found

    Two-proton radioactivity and three-body decay. V. Improved momentum distributions

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    Nowadays quantum-mechanical theory allows one to reliably calculate the processes of 2p radioactivity (true three-body decays) and the corresponding energy and angular correlations up to distances of the order of 1000 fm. However, the precision of modern experiments has now become sufficient to indicate some deficiency of the predicted theoretical distributions. In this paper we discuss the extrapolation along the classical trajectories as a method to improve the convergence of the theoretical energy and angular correlations at very large distances (of the order of atomic distances), where only the long-range Coulomb forces are still operating. The precision of this approach is demonstrated using the "exactly" solvable semianalytical models with simplified three-body Hamiltonians. It is also demonstrated that for heavy 2p emitters, the 2p decay momentum distributions can be sensitive to the effect of the screening by atomic electrons. We compare theoretical results with available experimental data.Comment: 13 pages, 18 figure

    Structure sensitivity of selective acetylene hydrogenation over the catalysts with shape-controlled palladium nanoparticles

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    The structure sensitivity of acetylene hydrogenation on catalysts with controlled shape of palladium nanoparticles was studied. Palladium particles of cubic (Pdcub), cuboctahedral (Pdco) and octahedral (Pdoct) shapes were obtained by a colloidal method. Poly(N-vinyl)pyrrolidone (PVP) was used as the stabilizer of colloidal solutions. In order to eliminate the effect of the polymer on the properties of the catalyst, PVP was removed from the surface of the particles after their transfer to the support by simultaneous treatment with ozone and UV radiation. This allowed complete cleaning of the catalyst surface from the organic stabilizer without any change in the morphology of particles. The effectiveness of this treatment method was confirmed by X-ray photoelectron spectroscopy and scanning electron microscopy. It was found experimentally that the shape of nanoparticles does not influence the catalyst selectivity, but the activity decreases in the order Pdoct > Pdco > Pdcub. Since octahedrons consist of (111) faces, the cubes contain only (100) faces, and the cuboctahedrons are composed of faces of both types, Pd111 is more active than Pd100. Calculations with the use of a statistical method showed that the ∼3-nm Pd octahedrons are nanoparticles with optimum shape and size, giving maximum catalyst activit

    Spectrum of cosmic rays, produced in supernova remnants

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    Nonlinear kinetic theory of cosmic ray (CR) acceleration in supernova remnants is employed to calculate CR spectra. The magnetic field in SNRs is assumed to be significantly amplified by the efficiently accelerating nuclear CR component. It is shown that the calculated CR spectra agree in a satisfactory way with the existing measurements up to the energy 101710^{17} eV. The power law spectrum of protons extends up to the energy 3×10153\times 10^{15} eV with a subsequent exponential cutoff. It gives a natural explanation for the observed knee in the Galactic CR spectrum. The maximum energy of the accelerated nuclei is proportional to their charge number ZZ. Therefore the break in the Galactic CR spectrum is the result of the contribution of progressively heavier species in the overall CR spectrum so that at 101710^{17} eV the CR spectrum is dominated by iron group nuclei. It is shown that this component plus a suitably chosen extragalactic CR component can give a consistent description for the entire Galactic CR spectrum.Comment: 4 pages with emulateapj, 3 figures, accepted for publication in the Astrophysical Journal Letter

    Long-Time Asymptotics of Perturbed Finite-Gap Korteweg-de Vries Solutions

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    We apply the method of nonlinear steepest descent to compute the long-time asymptotics of solutions of the Korteweg--de Vries equation which are decaying perturbations of a quasi-periodic finite-gap background solution. We compute a nonlinear dispersion relation and show that the x/tx/t plane splits into g+1g+1 soliton regions which are interlaced by g+1g+1 oscillatory regions, where g+1g+1 is the number of spectral gaps. In the soliton regions the solution is asymptotically given by a number of solitons travelling on top of finite-gap solutions which are in the same isospectral class as the background solution. In the oscillatory region the solution can be described by a modulated finite-gap solution plus a decaying dispersive tail. The modulation is given by phase transition on the isospectral torus and is, together with the dispersive tail, explicitly characterized in terms of Abelian integrals on the underlying hyperelliptic curve.Comment: 45 pages. arXiv admin note: substantial text overlap with arXiv:0705.034

    Exact quantum master equation for a molecular aggregate coupled to a harmonic bath

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    We consider a molecular aggregate consisting of NN identical monomers. Each monomer comprises two electronic levels and a single harmonic mode. The monomers interact with each other via dipole-dipole forces. The monomer vibrational modes are bilinearly coupled to a bath of harmonic oscillators. This is a prototypical model for the description of coherent exciton transport, from quantum dots to photosynthetic antennae. We derive an exact quantum master equation for such systems. Computationally, the master equation may be useful for the testing of various approximations employed in theories of quantum transport. Physically, it offers a plausible explanation of the origins of long-lived coherent optical responses of molecular aggregates in dissipative environments

    Coulomb Dissociation of 17Ne^{17}Ne

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    On UHECR energy estimation algorithms based on the measurement of electromagnetic component parameters in EAS

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    Model calculations are performed of extensive air shower (EAS) component energies using a variety of hadronic interaction parameters. A conversion factor from electromagnetic component energy to the energy of ultra-high energy cosmic rays (UHECRs) and its model and primary mass dependence is studied. It is shown that model dependence of the factor minimizes under the necessary condition of the same maximum position and muon content of simulated showers.Comment: contracted version is accepted for publication in Doklady Physic

    Asymptotic Expansions for the Conditional Sojourn Time Distribution in the M/M/1M/M/1-PS Queue

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    We consider the M/M/1M/M/1 queue with processor sharing. We study the conditional sojourn time distribution, conditioned on the customer's service requirement, in various asymptotic limits. These include large time and/or large service request, and heavy traffic, where the arrival rate is only slightly less than the service rate. The asymptotic formulas relate to, and extend, some results of Morrison \cite{MO} and Flatto \cite{FL}.Comment: 30 pages, 3 figures and 1 tabl

    Communicative-Pragmatic Assessment Is Sensitive and Time-Effective in Measuring the Outcome of Aphasia Therapy

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    A range of methods in clinical research aim to assess treatment-induced progress in aphasia therapy. Here, we used a crossover randomized controlled design to compare the suitability of utterance-centered and dialogue-sensitive outcome measures in speech-language testing. Fourteen individuals with post- stroke chronic non-fluent aphasia each received two types of intensive training in counterbalanced order: conventional confrontation naming, and communicative-pragmatic speech-language therapy (Intensive Language-Action Therapy, an expanded version of Constraint-Induced Aphasia Therapy). Motivated by linguistic-pragmatic theory and neuroscience data, our dependent variables included a newly created diagnostic instrument, the Action Communication Test (ACT). This diagnostic instrument requires patients to produce target words in two conditions: (i) utterance-centered object naming, and (ii) communicative- pragmatic social interaction based on verbal requests. In addition, we administered a standardized aphasia test battery, the Aachen Aphasia Test (AAT). Composite scores on the ACT and the AAT revealed similar patterns of changes in language performance over time, irrespective of the treatment applied. Changes in language performance were relatively consistent with the AAT results also when considering both ACT subscales separately from each other. However, only the ACT subscale evaluating verbal requests proved to be successful in distinguishing between different types of training in our patient sample. Critically, testing duration was substantially shorter for the entire ACT (10–20 min) than for the AAT (60–90 min). Taken together, the current findings suggest that communicative-pragmatic methods in speech- language testing provide a sensitive and time-effective measure to determine the outcome of aphasia therapy
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