1,370 research outputs found
Two-proton radioactivity and three-body decay. V. Improved momentum distributions
Nowadays quantum-mechanical theory allows one to reliably calculate the
processes of 2p radioactivity (true three-body decays) and the corresponding
energy and angular correlations up to distances of the order of 1000 fm.
However, the precision of modern experiments has now become sufficient to
indicate some deficiency of the predicted theoretical distributions. In this
paper we discuss the extrapolation along the classical trajectories as a method
to improve the convergence of the theoretical energy and angular correlations
at very large distances (of the order of atomic distances), where only the
long-range Coulomb forces are still operating. The precision of this approach
is demonstrated using the "exactly" solvable semianalytical models with
simplified three-body Hamiltonians. It is also demonstrated that for heavy 2p
emitters, the 2p decay momentum distributions can be sensitive to the effect of
the screening by atomic electrons. We compare theoretical results with
available experimental data.Comment: 13 pages, 18 figure
Structure sensitivity of selective acetylene hydrogenation over the catalysts with shape-controlled palladium nanoparticles
The structure sensitivity of acetylene hydrogenation on catalysts with controlled shape of palladium nanoparticles was studied. Palladium particles of cubic (Pdcub), cuboctahedral (Pdco) and octahedral (Pdoct) shapes were obtained by a colloidal method. Poly(N-vinyl)pyrrolidone (PVP) was used as the stabilizer of colloidal solutions. In order to eliminate the effect of the polymer on the properties of the catalyst, PVP was removed from the surface of the particles after their transfer to the support by simultaneous treatment with ozone and UV radiation. This allowed complete cleaning of the catalyst surface from the organic stabilizer without any change in the morphology of particles. The effectiveness of this treatment method was confirmed by X-ray photoelectron spectroscopy and scanning electron microscopy. It was found experimentally that the shape of nanoparticles does not influence the catalyst selectivity, but the activity decreases in the order Pdoct > Pdco > Pdcub. Since octahedrons consist of (111) faces, the cubes contain only (100) faces, and the cuboctahedrons are composed of faces of both types, Pd111 is more active than Pd100. Calculations with the use of a statistical method showed that the ∼3-nm Pd octahedrons are nanoparticles with optimum shape and size, giving maximum catalyst activit
Spectrum of cosmic rays, produced in supernova remnants
Nonlinear kinetic theory of cosmic ray (CR) acceleration in supernova
remnants is employed to calculate CR spectra. The magnetic field in SNRs is
assumed to be significantly amplified by the efficiently accelerating nuclear
CR component. It is shown that the calculated CR spectra agree in a
satisfactory way with the existing measurements up to the energy eV.
The power law spectrum of protons extends up to the energy eV
with a subsequent exponential cutoff. It gives a natural explanation for the
observed knee in the Galactic CR spectrum. The maximum energy of the
accelerated nuclei is proportional to their charge number . Therefore the
break in the Galactic CR spectrum is the result of the contribution of
progressively heavier species in the overall CR spectrum so that at
eV the CR spectrum is dominated by iron group nuclei. It is shown that this
component plus a suitably chosen extragalactic CR component can give a
consistent description for the entire Galactic CR spectrum.Comment: 4 pages with emulateapj, 3 figures, accepted for publication in the
Astrophysical Journal Letter
Long-Time Asymptotics of Perturbed Finite-Gap Korteweg-de Vries Solutions
We apply the method of nonlinear steepest descent to compute the long-time
asymptotics of solutions of the Korteweg--de Vries equation which are decaying
perturbations of a quasi-periodic finite-gap background solution. We compute a
nonlinear dispersion relation and show that the plane splits into
soliton regions which are interlaced by oscillatory regions, where
is the number of spectral gaps.
In the soliton regions the solution is asymptotically given by a number of
solitons travelling on top of finite-gap solutions which are in the same
isospectral class as the background solution. In the oscillatory region the
solution can be described by a modulated finite-gap solution plus a decaying
dispersive tail. The modulation is given by phase transition on the isospectral
torus and is, together with the dispersive tail, explicitly characterized in
terms of Abelian integrals on the underlying hyperelliptic curve.Comment: 45 pages. arXiv admin note: substantial text overlap with
arXiv:0705.034
Exact quantum master equation for a molecular aggregate coupled to a harmonic bath
We consider a molecular aggregate consisting of identical monomers. Each
monomer comprises two electronic levels and a single harmonic mode. The
monomers interact with each other via dipole-dipole forces. The monomer
vibrational modes are bilinearly coupled to a bath of harmonic oscillators.
This is a prototypical model for the description of coherent exciton transport,
from quantum dots to photosynthetic antennae. We derive an exact quantum master
equation for such systems. Computationally, the master equation may be useful
for the testing of various approximations employed in theories of quantum
transport. Physically, it offers a plausible explanation of the origins of
long-lived coherent optical responses of molecular aggregates in dissipative
environments
On UHECR energy estimation algorithms based on the measurement of electromagnetic component parameters in EAS
Model calculations are performed of extensive air shower (EAS) component
energies using a variety of hadronic interaction parameters. A conversion
factor from electromagnetic component energy to the energy of ultra-high energy
cosmic rays (UHECRs) and its model and primary mass dependence is studied. It
is shown that model dependence of the factor minimizes under the necessary
condition of the same maximum position and muon content of simulated showers.Comment: contracted version is accepted for publication in Doklady Physic
Asymptotic Expansions for the Conditional Sojourn Time Distribution in the -PS Queue
We consider the queue with processor sharing. We study the
conditional sojourn time distribution, conditioned on the customer's service
requirement, in various asymptotic limits. These include large time and/or
large service request, and heavy traffic, where the arrival rate is only
slightly less than the service rate. The asymptotic formulas relate to, and
extend, some results of Morrison \cite{MO} and Flatto \cite{FL}.Comment: 30 pages, 3 figures and 1 tabl
Communicative-Pragmatic Assessment Is Sensitive and Time-Effective in Measuring the Outcome of Aphasia Therapy
A range of methods in clinical research aim to assess treatment-induced
progress in aphasia therapy. Here, we used a crossover randomized controlled
design to compare the suitability of utterance-centered and dialogue-sensitive
outcome measures in speech-language testing. Fourteen individuals with post-
stroke chronic non-fluent aphasia each received two types of intensive
training in counterbalanced order: conventional confrontation naming, and
communicative-pragmatic speech-language therapy (Intensive Language-Action
Therapy, an expanded version of Constraint-Induced Aphasia Therapy). Motivated
by linguistic-pragmatic theory and neuroscience data, our dependent variables
included a newly created diagnostic instrument, the Action Communication Test
(ACT). This diagnostic instrument requires patients to produce target words in
two conditions: (i) utterance-centered object naming, and (ii) communicative-
pragmatic social interaction based on verbal requests. In addition, we
administered a standardized aphasia test battery, the Aachen Aphasia Test
(AAT). Composite scores on the ACT and the AAT revealed similar patterns of
changes in language performance over time, irrespective of the treatment
applied. Changes in language performance were relatively consistent with the
AAT results also when considering both ACT subscales separately from each
other. However, only the ACT subscale evaluating verbal requests proved to be
successful in distinguishing between different types of training in our
patient sample. Critically, testing duration was substantially shorter for the
entire ACT (10–20 min) than for the AAT (60–90 min). Taken together, the
current findings suggest that communicative-pragmatic methods in speech-
language testing provide a sensitive and time-effective measure to determine
the outcome of aphasia therapy
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