Luminescent solar concentrators. 2: Experimental and theoretical analysis of their possible efficiencies

Experimental techniques are developed to determine the applicability of a particular luminescing center for use in a luminescent solar concentrator (LSC). The relevant steady-state characteristics of eighteen common organic laser dyes are given. The relative spectral homogeneity of such dyes are shown to depend upon the surrounding material using narrowband laser excitation. We developed three independent techniques for measuring self-absorption rates; these are time-resolved emission, steady-state polarization anisotropy, and spectral convolution. Preliminary dye degradation and prototype efficiency measurements are included. Finally, we give simple relationships relating the efficiency and gain of an LSC to key spectroscopic parameters of its constituents

Luminescent Solar Concentrators

A type of solar concentrator for photovoltaics utilizing light pipe trapping of luminescence is described. Total collector efficiencies of 3. 2% have been measured, and efficiencies of 10% appear theoretically possible. The photodegradation lifetime of the dyes presently used is about one year under optimal conditions

Relativistic Hartree-Bogoliubov description of the deformed ground-state proton emitters

Ground-state properties of deformed proton-rich odd-Z nuclei in the region $59 \leq Z \leq 69$ are described in the framework of Relativistic Hartree Bogoliubov (RHB) theory. One-proton separation energies and ground-state quadrupole deformations that result from fully self-consistent microscopic calculations are compared with available experimental data. The model predicts the location of the proton drip-line, the properties of proton emitters beyond the drip-line, and provides information about the deformed single-particle orbitals occupied by the odd valence proton.Comment: 9 pages, RevTeX, 3 PS figures, submitted Phys. Rev. Letter

Orbital dependent nucleonic pairing in the lightest known isotopes of tin

By studying the 109Xe-->105Te-->101Sn superallowed alpha-decay chain, we observe low-lying states in 101Sn, the one-neutron system outside doubly magic 100Sn. We find that the spins of the ground state (J = 7=2) and first excited state (J = 5=2) in 101Sn are reversed with respect to the traditional level ordering postulated for 103Sn and the heavier tin isotopes. Through simple arguments and state-of-the-art shell model calculations we explain this unexpected switch in terms of a transition from the single-particle regime to the collective mode in which orbital-dependent pairing correlations, dominate.Comment: 5 pages 3 figure

The Single-Particle Structure of Neutron-Rich Nuclei of Astrophysical Interest at the Ornl Hribf

The rapid nuetron-capture process (r process) produces roughly half of the elements heavier than iron. The path and abundances produced are uncertain, however, because of the lack of nuclear strucure information on important neutron-rich nuclei. We are studying nuclei on or near the r-process path via single-nucleon transfer reactions on neutron-rich radioactive beams at ORNL's Holifield Radioactive Ion Beam Facility (HRIBF). Owing to the difficulties in studying these reactions in inverse kinematics, a variety of experimental approaches are being developed. We present the experimental methods and initial results.Comment: Proceedings of the Third International Conference on Fission and Properties of Neutron-Rich Nucle

Beta decay of 71,73Co; probing single particle states approaching doubly magic 78Ni

Low-energy excited states in 71,73Ni populated via the {\beta} decay of 71,73Co were investigated in an experiment performed at the National Superconducting Cyclotron Laboratory (NSCL) at Michigan State University (MSU). Detailed analysis led to the construction of level schemes of 71,73Ni, which are interpreted using systematics and analyzed using shell model calculations. The 5/2- states attributed to the the f5/2 orbital and positive parity 5/2+ and 7/2+ states from the g9/2 orbital have been identified in both 71,73Ni. In 71Ni the location of a 1/2- {\beta}-decaying isomer is proposed and limits are suggested as to the location of the isomer in 73Ni. The location of positive parity cluster states are also identified in 71,73Ni. Beta-delayed neutron branching ratios obtained from this data are given for both 71,73Co.Comment: Accepted for publication in PR

Quasi Harmonic Lattice Dynamics and Molecular Dynamics calculations for the Lennard-Jones solids

We present Molecular Dynamics (MD), Quasi Harmonic Lattice Dynamics (QHLD) and Energy Minimization (EM) calculations for the crystal structure of Ne, Ar, Kr and Xe as a function of pressure and temperature. New Lennard-Jones (LJ) parameters are obtained for Ne, Kr and Xe to reproduce the experimental pressure dependence of the density. We employ a simple method which combines results of QHLD and MD calculations to achieve densities in good agreement with experiment from 0 K to melting. Melting is discussed in connection with intrinsic instability of the solid as given by the QHLD approximation. (See http://www.fci.unibo.it/~valle for related papers)Comment: 7 pages, 5 figures, REVte

Theoretical description of deformed proton emitters: nonadiabatic coupled-channel method

The newly developed nonadiabatic method based on the coupled-channel Schroedinger equation with Gamow states is used to study the phenomenon of proton radioactivity. The new method, adopting the weak coupling regime of the particle-plus-rotor model, allows for the inclusion of excitations in the daughter nucleus. This can lead to rather different predictions for lifetimes and branching ratios as compared to the standard adiabatic approximation corresponding to the strong coupling scheme. Calculations are performed for several experimentally seen, non-spherical nuclei beyond the proton dripline. By comparing theory and experiment, we are able to characterize the angular momentum content of the observed narrow resonance.Comment: 12 pages including 10 figure