Magnetic-Field Induced Quantum Critical Point in YbRh2_2Si2_2

We report low-temperature calorimetric, magnetic and resistivity measurements on the antiferromagnetic (AF) heavy-fermion metal YbRh$_2$Si$_2$ (${T_N =}$ 70 mK) as a function of magnetic field $B$. While for fields exceeding the critical value ${B_{c0}}$ at which ${T_N\to0}$ the low temperature resistivity shows an ${AT^2}$ dependence, a ${1/(B-B_{c0})}$ divergence of ${A(B)}$ upon reducing $B$ to ${B_{c0}}$ suggests singular scattering at the whole Fermi surface and a divergence of the heavy quasiparticle mass. The observations are interpreted in terms of a new type of quantum critical point separating a weakly AF ordered from a weakly polarized heavy Landau-Fermi liquid state.Comment: accepted for publication in Phys. Rev. Let

Tuning Heavy Fermion Systems into Quantum Criticality by Magnetic Field

We discuss a series of thermodynamic, magnetic and electrical transport experiments on the two heavy fermion compounds CeNi2Ge2 and YbRh2Si2 in which magnetic fields, B, are used to tune the systems from a Non-Fermi liquid (NFL) into a field-induced FL state. Upon approaching the quantum-critical points from the FL side by reducing B we analyze the heavy quasiparticle (QP) mass and QP-QP scattering cross sections. For CeNi2Ge2 the observed behavior agrees well with the predictions of the spin-density wave (SDW) scenario for three-dimensional (3D) critical spin-fluctuations. By contrast, the observed singularity in YbRh2Si2 cannot be explained by the itinerant SDW theory for neither 3D nor 2D critical spinfluctuations. Furthermore, we investigate the magnetization M(B) at high magnetic fields. For CeNi2Ge2 a metamagnetic transition is observed at 43 T, whereas for YbRh2Si2 a kink-like anomaly occurs at 10 T in M vs B (applied along the easy basal plane) above which the heavy fermion state is completely suppressed.Comment: 15 pages, 8 figures, submitted to Journal of Low Temperature Physics, special Series on "High Magnetic Field Facilities

Field-induced quantum critical route to a Fermi liquid in high-temperature superconductors

In high transition temperature (T_c) superconductivity, charge doping is a natural tuning parameter that takes copper oxides from the antiferromagnet to the superconducting region. In the metallic state above T_c the standard Landau's Fermi-liquid theory of metals as typified by the temperature squared (T^2) dependence of resistivity appears to break down. Whether the origin of the non-Fermi-liquid behavior is related to physics specific to the cuprates is a fundamental question still under debate. We uncover a new transformation from the non-Fermi- to a standard Fermi-liquid state driven not by doping but by magnetic field in the overdoped high-T_c superconductor Tl_2Ba_2CuO_{6+x}. From the c-axis resistivity measured up to 45 T, we show that the Fermi-liquid features appear above a sufficiently high field which decreases linearly with temperature and lands at a quantum critical point near the superconductivity's upper critical field -- with the Fermi-liquid coefficient of the T^2 dependence showing a power-law diverging behavior on the approach to the critical point. This field-induced quantum criticality bears a striking resemblance to that in quasi-two dimensional heavy-Fermion superconductors, suggesting a common underlying spin-related physics in these superconductors with strong electron correlations.Comment: 6 pages, 4 figure

Hall-effect evolution across a heavy-fermion quantum critical point

A quantum critical point (QCP) develops in a material at absolute zero when a new form of order smoothly emerges in its ground state. QCPs are of great current interest because of their singular ability to influence the finite temperature properties of materials. Recently, heavy-fermion metals have played a key role in the study of antiferromagnetic QCPs. To accommodate the heavy electrons, the Fermi surface of the heavy-fermion paramagnet is larger than that of an antiferromagnet. An important unsolved question concerns whether the Fermi surface transformation at the QCP develops gradually, as expected if the magnetism is of spin density wave (SDW) type, or suddenly as expected if the heavy electrons are abruptly localized by magnetism. Here we report measurements of the low-temperature Hall coefficient ($R_H$) - a measure of the Fermi surface volume - in the heavy-fermion metal YbRh2Si2 upon field-tuning it from an antiferromagnetic to a paramagnetic state. $R_H$ undergoes an increasingly rapid change near the QCP as the temperature is lowered, extrapolating to a sudden jump in the zero temperature limit. We interpret these results in terms of a collapse of the large Fermi surface and of the heavy-fermion state itself precisely at the QCP.Comment: 20 pages, 3 figures; to appear in Natur

Scaling approach to itinerant quantum critical points

Based on phase space arguments, we develop a simple approach to metallic quantum critical points, designed to study the problem without integrating the fermions out of the partition function. The method is applied to the spin-fermion model of a T=0 ferromagnetic transition. Stability criteria for the conduction and the spin fluids are derived by scaling at the tree level. We conclude that anomalous exponents may be generated for the fermion self-energy and the spin-spin correlation functions below $d=3$, in spite of the spin fluid being above its upper critical dimension.Comment: 3 pages, 2 figures; discussion of the phase space restriction modified and, for illustrative purposes, restricted to the tree-level analysis of the ferromagnetic transitio

YbRh2Si2: Quantum tricritical behavior in itinerant electron systems

We propose that proximity of the first-order transition manifested by the quantum tricritical point (QTCP) explains non-Fermi-liquid properties of YbRh2Si2. Here, at the QTCP, a continuous phase transition changes into first order at zero temperature. The non-Fermi-liquid behaviors of YbRh2Si2 are puzzling in two aspects; diverging ferromagnetic susceptibility at the antiferromagnetic transition and unconventional power-law dependence in thermodynamic quantities. These puzzles are solved by an unconventional criticality derived from our spin fluctuation theory for the QTCP.Comment: 4 pages, 3 figure

Divergence of the Grueneisen Ratio at Quantum Critical Points in Heavy Fermion Metals

We present low-temperature volume thermal expansion, $\beta$, and specific heat, $C$, measurements on high-quality single crystals of CeNi2Ge2 and YbRh2(Si$_{0.95}$Ge$_{0.05}$)$_2$ which are located very near to quantum critical points. For both systems, $\beta$ shows a more singular temperature dependence than $C$, and thus the Grueneisen ratio ${\Gamma \propto \beta/C}$ diverges as T --> 0. For CeNi2Ge2, our results are in accordance with the spin-density wave (SDW) scenario for three-dimensional critical spin-fluctuations. By contrast, the observed singularity in YbRh2$(Si$_{0.95}$Ge$_{0.05}$)$_2$ cannot be explained by the itinerant SDW theory but is qualitatively consistent with a locally quantum critical picture.Comment: 11 pages, 4 figure

Non Fermi Liquid behavior in the under-screened Kondo model

Using the Schwinger boson spin representation, we reveal a new aspect to the physics of a partially screened magnetic moment in a metal, as described by the spin $S$ Kondo model. We show that the residual ferromagnetic interaction between a partially screened spin and the electron sea destabilizes the Landau Fermi liquid, forming a singular Fermi liquid with a $1/ (T \ln ^{4} (T_{K}/T))$ divergence in the low temperature specific heat coefficient $C_{V}/T$. A magnetic field $B$ tunes this system back into Landau Fermi liquid with a Fermi temperature proportional to $B \ln^2 (T_K/B)$. We discuss a possible link with field-tuned quantum criticality in heavy electron materials.Comment: References corrected. Minor changes to tex

Break up of heavy fermions at an antiferromagnetic instability

We present results of high-resolution, low-temperature measurements of the Hall coefficient, thermopower, and specific heat on stoichiometric YbRh2Si2. They support earlier conclusions of an electronic (Kondo-breakdown) quantum critical point concurring with a field induced antiferromagnetic one. We also discuss the detachment of the two instabilities under chemical pressure. Volume compression/expansion (via substituting Rh by Co/Ir) results in a stabilization/weakening of magnetic order. Moderate Ir substitution leads to a non-Fermi-liquid phase, in which the magnetic moments are neither ordered nor screened by the Kondo effect. The so-derived zero-temperature global phase diagram promises future studies to explore the nature of the Kondo breakdown quantum critical point without any interfering magnetism.Comment: minor changes, accepted for publication in JPS