Zero-bias molecular electronics: Exchange-correlation corrections to Landauer's formula

Standard first principles calculations of transport through single molecules miss exchange-correlation corrections to the Landauer formula. From Kubo response theory, both the Landauer formula and these corrections in the limit of zero bias are derived and calculations are presented.Comment: 4 pages, 3 figures, final version to appear in Phys. Rev. B, Rapid Communication

Yoctosecond photon pulses from quark-gluon plasmas

Present ultra-fast laser optics is at the frontier between atto- and zeptosecond photon pulses, giving rise to unprecedented applications. We show that high-energetic photon pulses down to the yoctosecond timescale can be produced in heavy ion collisions. We focus on photons produced during the initial phase of the expanding quark-gluon plasma. We study how the time evolution and properties of the plasma may influence the duration and shape of the photon pulse. Prospects for achieving double peak structures suitable for pump-probe experiments at the yoctosecond timescale are discussed.Comment: 4 pages, 2 figures; final version as accepted by PR

Control of beam propagation in optically written waveguides beyond the paraxial approximation

Beam propagation beyond the paraxial approximation is studied in an optically written waveguide structure. The waveguide structure that leads to diffractionless light propagation, is imprinted on a medium consisting of a five-level atomic vapor driven by an incoherent pump and two coherent spatially dependent control and plane-wave fields. We first study propagation in a single optically written waveguide, and find that the paraxial approximation does not provide an accurate description of the probe propagation. We then employ coherent control fields such that two parallel and one tilted Gaussian beams produce a branched waveguide structure. The tilted beam allows selective steering of the probe beam into different branches of the waveguide structure. The transmission of the probe beam for a particular branch can be improved by changing the width of the titled Gaussian control beam as well as the intensity of the spatially dependent incoherent pump field.Comment: 10 pages, 9 figure

Dynamic formation of Rydberg aggregates at off-resonant excitation

The dynamics of a cloud of ultra-cold two-level atoms is studied at off-resonant laser driving to a Rydberg state. We find that resonant excitation channels lead to strongly peaked spatial correlations associated with the buildup of asymmetric excitation structures. These aggregates can extend over the entire ensemble volume, but are in general not localized relative to the system boundaries. The characteristic distances between neighboring excitations depend on the laser detuning and on the interaction potential. These properties lead to characteristic features in the spatial excitation density, the Mandel $Q$ parameter, and the total number of excitations. As an application an implementation of the three-atom CSWAP or Fredkin gate with Rydberg atoms is discussed. The gate not only exploits the Rydberg blockade, but also utilizes the special features of an asymmetric geometric arrangement of the three atoms. We show that continuous-wave off-resonant laser driving is sufficient to create the required spatial arrangement of atoms out of a homogeneous cloud.Comment: 8 pages, 7 figure

Nuclear spin dynamics influenced and detected by electron spin polarization in CdTe/CdMgTe quantum wells

Nuclear spin coherence and relaxation dynamics of all constituent isotopes of an n-doped CdTe/(Cd,Mg)Te quantum well structure are studied employing optically detected nuclear magnetic resonance. Using time-resolved pump-probe Faraday ellipticity, we generate and detect the coherent spin dynamics of the resident electrons. The photogenerated electron spin polarization is transferred into the nuclear spin system, which becomes polarized and acts back on the electron spins as the Overhauser field. Under the influence of resonant radio frequency pulses, we trace the coherent spin dynamics of the nuclear isotopes $^{111}$Cd, $^{113}$Cd, and $^{125}$Te. We measure nuclear Rabi oscillations, the inhomogeneous dephasing time $T_2^*$, the spin coherence time $T_2$, and the longitudinal relaxation time $T_1$. Furthermore, we investigate the influence of the laser excitation and the corresponding electron spin polarization on the nuclear spin relaxation time and find a weak extension of this time induced by interaction with the electron spins.Comment: 5 pages, 2 figure

Density of states in graphene with vacancies: midgap power law and frozen multifractality

The density of states (DoS), $\varrho(E)$, of graphene is investigated numerically and within the self-consistent T-matrix approximation (SCTMA) in the presence of vacancies within the tight binding model. The focus is on compensated disorder, where the concentration of vacancies, $n_\text{A}$ and $n_\text{B}$, in both sub-lattices is the same. Formally, this model belongs to the chiral symmetry class BDI. The prediction of the non-linear sigma-model for this class is a Gade-type singularity $\varrho(E) \sim |E|^{-1}\exp(-|\log(E)|^{-1/x})$. Our numerical data is compatible with this result in a preasymptotic regime that gives way, however, at even lower energies to $\varrho(E)\sim E^{-1}|\log(E)|^{-\mathfrak{x}}$, $1\leq \mathfrak{x} < 2$. We take this finding as an evidence that similar to the case of dirty d-wave superconductors, also generic bipartite random hopping models may exhibit unconventional (strong-coupling) fixed points for certain kinds of randomly placed scatterers if these are strong enough. Our research suggests that graphene with (effective) vacancy disorder is a physical representative of such systems.Comment: References updated onl

C58 on Au(111): a scanning tunneling microscopy study

C58 fullerenes were adsorbed onto room temperature Au(111) surface by low-energy (~6 eV) cluster ion beam deposition under ultrahigh vacuum conditions. The topographic and electronic properties of the deposits were monitored by means of scanning tunnelling microscopy (STM at 4.2 K). Topographic images reveal that at low coverages fullerene cages are pinned by point dislocation defects on the herringbone reconstructed gold terraces (as well as by step edges). At intermediate coverages, pinned monomers, act as nucleation centres for the formation of oligomeric C58 chains and 2D islands. At the largest coverages studied, the surface becomes covered by 3D interlinked C58 cages. STM topographic images of pinned single adsorbates are essentially featureless. The corresponding local densities of states are consistent with strong cage-substrate interactions. Topographic images of [C58]n oligomers show a stripe-like intensity pattern oriented perpendicular to the axis connecting the cage centers. This striped pattern becomes even more pronounced in maps of the local density of states. As supported by density functional theory, DFT calculations, and also by analogous STM images previously obtained for C60 polymers (M. Nakaya et al., J. Nanosci. Nanotechnol. 11, 2829 (2011)), we conclude that these striped orbital patterns are a fingerprint of covalent intercage bonds. For thick C58 films we have derived a band gap of 1.2 eV from scanning tunnelling spectroscopy data, STS, confirming that the outermost C58 layer behaves as a wide band semiconductor

Dimensionality dependence of the wave function statistics at the Anderson transition

The statistics of critical wave functions at the Anderson transition in three and four dimensions are studied numerically. The distribution of the inverse participation ratios (IPR) $P_q$ is shown to acquire a scale-invariant form in the limit of large system size. Multifractality spectra governing the scaling of the ensemble-averaged IPRs are determined. Conjectures concerning the IPR statistics and the multifractality at the Anderson transition in a high spatial dimensionality are formulated.Comment: 4 pages, 4 figure

Quantum Hall Transition in the Classical Limit

We study the quantum Hall transition using the density-density correlation function. We show that in the limit h->0 the electron density moves along the percolating trajectories, undergoing normal diffusion. The localization exponent coincides with its percolation value \nu=4/3. The framework provides a natural way to study the renormalization group flow from percolation to quantum Hall transition. We also confirm numerically that the critical conductivity of a classical limit of quantum Hall transition is \sigma_{xx} = \sqrt{3}/4.Comment: 8 pages, 4 figures; substantial changes include the critical conductivity calculatio

Superconductivity in Pseudo-Binary Silicide SrNixSi2-x with AlB2-Type Structure

We demonstrate the emergence of superconductivity in pseudo-binary silicide SrNixSi2-x. The compound exhibits a structural phase transition from the cubic SrSi2-type structure (P4132) to the hexagonal AlB2-type structure (P6/mmm) upon substituting Ni for Si at approximately x = 0.1. The hexagonal structure is stabilized in the range of 0.1 < x < 0.7. The superconducting phase appears in the vicinity of the structural phase boundary. Ni acts as a nonmagnetic dopant, as confirmed by the Pauli paramagnetic behavior.Comment: 12 pages, 5 figure