Application of Nonlinear Conductivity Spectroscopy to Ion Transport in Solid Electrolytes

The field-dependent ion transport in thin samples of different glasses is characterised by means of nonlinear conductivity spectroscopy. AC electric fields with strengths up to 77 kV/cm are applied to the samples, and the Fourier components of the current spectra are analysed. In the dc conductivity regime and in the transition region to the dispersive conductivity, higher harmonics in the current spectra are detected, which provide information about higher--order conductivity coefficients. Our method ensures that these higher--order conductivity coefficients are exclusively governed by field--dependent ion transport and are not influenced by Joule heating effects. We use the low-field dc conductivity $\sigma_{1,dc}$ and the higher--order dc conductivity coefficient $\sigma_{3,dc}$ to calculate apparent jump distances for the mobile ions, $a_{\rm app}$. Over a temperature range from 283 K to 353 K, we obtain values for $a_{app}$ between 39 \AA $$ and 55 \AA . For all glasses, we find a weak decrease of $a_{\rm app}$ with increasing temperature. Remarkably, the apparent jump distances calculated from our data are considerably larger than typical values published in the literature for various ion conducting glasses. These values were obtained by applying dc electric fields. Our results provide clear evidence that the equation used in the literature to calculate the apparent jump distances does not provide an adequate physical description of field-dependent ion transport.Comment: 6 pages, 5 figure

Spectroscopic Study on the Beryllium Abundances of Red Giant Stars

An extensive spectroscopic study was carried out for the beryllium abundances of 200 red giants (mostly of late G and early K type), which were determined from the near-UV Be II 3131.066 line based on high-dispersion spectra obtained by Subaru/HDS, with an aim of investigating the nature of surface Be contents in these evolved giants; e.g., dependence upon stellar parameters, degree of peculiarity along with its origin and build-up timing. We found that Be is considerably deficient (to widely different degree from star to star) in the photosphere of these evolved giants by ~1-3 dex (or more) compared to the initial abundance. While the resulting Be abundances (A(Be)) appear to weakly depend upon T_eff, log g, [Fe/H], M, age, and v_sin i, this may be attributed to the metallicity dependence of A(Be) coupled with the mutual correlation between these stellar parameters, since such tendencies almost disappear in the metallicity-scaled Be abundance ([Be/Fe]). By comparing the Be abundances (as well as their correlations with Li and C) to the recent theoretical predictions based on sophisticated stellar evolution calculations, we concluded that such a considerable extent/diversity of Be deficit is difficult to explain only by the standard theory of first dredge-up in the envelope of red giants, and that some extra mixing process (such as rotational or thermohaline mixing) must be responsible, which presumably starts to operate already in the main-sequence phase. This view is supported by the fact that appreciable Be depletion is seen in less evolved intermediate-mass B-A type stars near to the main sequence.Comment: 29 pages, 10 figures, 3 tables, accepted for publication in Publ. Astron. Soc. Japa

Explosive lithium production in the classical nova V339 Del (Nova Delphini 2013)

The origin of lithium (Li) and its production process have long been an unsettled question in cosmology and astrophysics. Candidates environments of Li production events or sites suggested by previous studies include big bang nucleosynthesis, interactions of energetic cosmic rays with interstellar matter, evolved low mass stars, novae, and supernova explosions. Chemical evolution models and observed stellar Li abundances suggest that at least half of the present Li abundance may have been produced in red giants, asymptotic giant branch (AGB) stars, and novae. However, no direct evidence for the supply of Li from stellar objects to the Galactic medium has yet been found. Here we report on the detection of highly blue-shifted resonance lines of the singly ionized radioactive isotope of beryllium, $^{7}$Be, in the near ultraviolet (UV) spectra of the classical nova V339 Del (Nova Delphini 2013). Spectra were obtained 38 to 48 days after the explosion. $^{7}$Be decays to form $^{7}$Li within a short time (half-life 53.22 days). The spectroscopic detection of this fragile isotope implies that it has been created during the nova explosion via the reaction ^{3}\mbox{He}(\alpha,\gamma)^{7}\mbox{Be}, and supports the theoretical prediction that a significant amount of $^{7}$Li could be produced in classical nova explosions. This finding opens a new way to explore $^{7}$Li production in classical novae and provides a clue to the mystery of the Galactic evolution of lithium.Comment: 28 pages, 6 figures, published in Natur

Beryllium Abundances of Solar-Analog Stars

An extensive beryllium abundance analysis was conducted for 118 solar analogs (along with 87 FGK standard stars) by applying the spectrum synthesis technique to the near-UV region comprising the Be II line at 3131.066 A, in an attempt to investigate whether Be suffers any depletion such as the case of Li showing a large diversity. We found that, while most of these Sun-like stars are superficially similar in terms of their A(Be) (Be abundances) around the solar value within ~ +/- 0.2dex, 4 out of 118 samples turned out strikingly Be-deficient (by more than ~2 dex) and these 4 stars belong to the group of lowest v_e sin i (projected rotation velocity). Moreover, even for the other majority showing an apparent similarity in Be, we can recognize a tendency that A(Be) gradually increases with an increase in v_e sin i. These observational facts suggest that any solar analog star (including the Sun) generally suffers some kind of Be depletion during their lives, where the rotational velocity (or the angular momentum) plays an important role in the sense that depletion tends to be enhanced by slower rotation. Hence, our findings require that the occasionally stated view "G-type dwarfs with T_eff ~< 6000 K are essentially homogeneous in Be with their original composition retained" should be revised. Also, our analysis indicates that the difference of ~0.2 dex in A(Be) between the solar photosphere and the meteorite really exists, implying that "UV missing opacity" is irrelevant at least for this Be II line.Comment: 18 pages, 12 figures, 3 tables and 3 electronic tables (included as ancillary files), accepted for publication in Publ. Astron. Soc. Japan (2011, Vol. 63, No. 4