Substitution Effects on FeSe Superconductor

We have investigated the effect of atomic substitutions in the FeSe system, which exhibits the simplest crystal structure among the iron-based superconductors. An enhancement of the superconducting transition temperature Tc was observed with the substitution of S or Te for Se; the Tc increased with S substitution by up to 20 %, and also increased with Te substitution up to 75 %. In contrast, Co or Ni substitutions for the Fe site significantly suppressed superconductivity. In this work we present a detailed description of the substitution technique employed to determine Tc in the FeSe system.Comment: 17 pages, 15 figures, 1 tabl

Superconductivity in S-substituted FeTe

We have successfully synthesized a new superconducting phase of FeTe1-xSx with a PbO-type structure. It has the simplest crystal structure in iron-based superconductors. Superconducting transition temperature is about 10 K at x = 0.2. The upper critical field Hc2 was estimated to be ~70 T. The coherent length was calculated to be ~2.2 nm. Because FeTe1-xSx is composed of nontoxic elements, this material is a candidate for applications and will activate more and more research on iron-based superconductor.Comment: 13 pages, 10 figure

Online monitoring system and data management for KamLAND

In January 22, 2002, KamLAND started the data-taking. The KamLAND detector is a complicated system which consists of liquid scintillator, buffer oil, spherical balloon and so on. In order to maintain the detector safety, we constructed monitoring system which collect detector status information such as balloon weight, liquid scintillator oil level and so on. In addition, we constructed continuous Rn monitoring system for the $^7$Be solar neutrino detection. The KamLAND monitoring system consists of various network, LON, 1-Wire, and TCP/IP, and these are indispensable for continuous experimental data acquisition.Comment: Submitted to Nucl.Instrum.Meth.

Electronic charges and electric potential at LaAlO3/SrTiO3 interfaces studied by core-level photoemission spectroscopy

We studied LaAlO3/SrTiO3 interfaces for varying LaAlO3 thickness by core-level photoemission spectroscopy. In Ti 2p spectra for conducting "n-type" interfaces, Ti3+ signals appeared, which were absent for insulating "p-type" interfaces. The Ti3+ signals increased with LaAlO3 thickness, but started well below the critical thickness of 4 unit cells for metallic transport. Core-level shifts with LaAlO3 thickness were much smaller than predicted by the polar catastrophe model. We attribute these observations to surface defects/adsorbates providing charges to the interface even below the critical thickness

Heterogeneity Induced Order in Globally Coupled Chaotic Systems

Collective behavior is studied in globally coupled maps with distributed nonlinearity. It is shown that the heterogeneity enhances regularity in the collective dynamics. Low-dimensional quasiperiodic motion is often found for the mean-field, even if each element shows chaotic dynamics. The mechanism of this order is due to the formation of an internal bifurcation structure, and the self-consistent dynamics between the structures and the mean-field. Keywords: Globally Coupled Map with heterogeneity, Collective behaviorComment: 11 pages (Revtex) + 4 figures (PostScript,tar+gzip

Growth of superconducting single-crystalline (Lu, Ca)Ba2Cu3O7-d whiskers

Single-crystalline (Lu, Ca)Ba2Cu3O7-d (Lu(Ca)123) whiskers have been successfully grown using the Te-doping method. X-ray diffraction patterns of Lu(Ca)123 whiskers showed sharp (0 0 l) peaks corresponding to REBa2Cu3O7-d phase (RE = rare earth elements). Transport measurements showed that the superconducting transition occurred at 83 K in the obtained whiskers.Comment: 3 pages, 3 figures, ISS200

Temperature-Dependence of Magnetically-Active Charge Excitations in Magnetite across the Verwey Transition

We have studied the electronic structure of bulk single crystals and epitaxial films of magnetite Fe$_3$O$_4$. Fe $2p$ core-level spectra show clear differences between hard x-ray (HAX-) and soft x-ray (SX-) photoemission spectroscopy (PES), indicative of surface effects. The bulk-sensitive spectra exhibit temperature ($T$)-dependent charge excitations across the Verwey transition at $T_V$=122 K, which is missing in the surface-sensitive spectra. An extended impurity Anderson model full-multiplet analysis reveals roles of the three distinct Fe-species (A-Fe$^{3+}$, B-Fe$^{2+}$, B-Fe$^{3+}$) below $T_V$ for the Fe $2p$ spectra, and its $T-$dependent evolution. The Fe $2p$ HAXPES spectra show a clear magnetic circular dichroism (MCD) in the metallic phase of magnetized 100-nm-thick films. The model calculations also reproduce the MCD and identify the magnetically distinct sites associated with the charge excitations. Valence band HAXPES shows finite density of states at $E_F$ for the polaronic metal with remnant order above $T_V$, and a clear gap formation below $T_V$. The results indicate that the Verwey transition is driven by changes in the strongly correlated and magnetically active B-Fe$^{2+}$ and B-Fe$^{3+}$ electronic states, consistent with resistivity and bulk-sensitive optical spectra.Comment: 5 pages, 4 figures Accepted in Physical Review Letter

Evolution of superconductivity by oxygen annealing in FeTe0.8S0.2

Oxygen annealing dramatically improved the superconducting properties of solid-state-reacted FeTe0.8S0.2, which showed only a broad onset of superconducting transition just after the synthesis. The zero resistivity appeared and reached 8.5 K by the oxygen annealing at 200\degree C. The superconducting volume fraction was also enhanced from 0 to almost 100%. The lattice constants were compressed by the oxygen annealing, indicating that the evolution of bulk superconductivity in FeTe0.8S0.2 was correlated to the shrinkage of lattice.Comment: 13 pages, 6 figure