Aharonov-Bohm phase as quantum gate in two-electron charge qubits

We analyze the singlet-triplet splitting on a planar array of quantum dots coupled capacitively to a set of external voltage gates. The system is modelled using an extended Hubbard Hamiltonian keeping two excess electrons on the array. The voltage dependence of the low-energy singlet and triplet states is analyzed using the Feshbach formalism. The formation of a well decoupled two-level system in the ground state is shown to rely on the fact of having two particles in the system. Coherent operation of the array is studied with respect to single quantum bit operations. One quantum gate is implemented via voltage controls, while for the necessary second quantum gate, a uniform external magnetic field is introduced. The Aharonov-Bohm phases on the closed loop tunnel connections in the array are used to effectively suppress the tunneling, despite a constant tunneling amplitude in the structure. This allows one to completely stall the qubit in any arbitrary quantum superposition, providing full control of this interesting quantum system.Comment: 6 pages, 5 figures (submitted to PRB

Potential landscapes and induced charges near metallic islands in three dimensions

We calculate electrostatic potential landscapes for an external probe charge in the presence of a set of metallic islands. Our numerical calculation in three dimensions (3D)uses an efficient grid relaxation technique. The well-known relaxation algorithm for solving the Poisson equation in two dimensions is generalized to 3D. In addition,all charges on the system, free as well as induced charges,are determined accurately and self-consistently to satisfy the desired boundary conditions. This allows the straightforward calculation of the potential on the outer boundary using the free space electrostatic Green's function,as well as the calculation of the entire capacitance matrix of the system. Physically interesting examples of nanoscale systems are presented and analyzed.Comment: 6 pages, 6 figures, submitted to PR

Matrix product state approach for a two-lead, multi-level Anderson impurity model

We exploit the common mathematical structure of the numerical renormalization group and the density matrix renormalization group, namely, matrix product states, to implement an efficient numerical treatment of a two-lead, multi-level Anderson impurity model. By adopting a star-like geometry, where each species (spin and lead) of conduction electrons is described by its own Wilson chain, instead of using a single Wilson chain for all species together, we achieve a very significant reduction in the numerical resources required to obtain reliable results. We illustrate the power of this approach by calculating ground state properties of a four-level quantum dot coupled to two leads. The success of this proof-of-principle calculation suggests that the star geometry constitutes a promising strategy for future calculations the ground state properties of multi-band, multi-level quantum impurity models. Moreover, we show that it is possible to find an "optimal" chain basis, obtained via a unitary transformation (acting only on the index distinguishing different Wilson chains), in which degrees of freedom on different Wilson chains become effectively decoupled from each other further out on the Wilson chains. This basis turns out to also diagonalize the model's chain-to-chain scattering matrix. We demonstrate this for a spinless two-lead model, presenting DMRG-results for the mutual information between two sites located far apart on different Wilson chains, and NRG results with respect to the scattering matrix.Comment: extended version, 11 pages, 12 figure

Non-Fermi liquid behavior in transport through Co doped Au chains

We calculate the conductance as a function of temperature $G(T)$ through Au monoatomic chains containing one Co atom as a magnetic impurity, and connected to two conducting leads with a 4-fold symmetry axis. Using the information derived from {\it ab initio} calculations, we construct an effective model \Heff that hybridizes a 3d$^7$ quadruplet at the Co site with two 3d$^8$ triplets through the hopping of 5d$_{xz}$ and 5d$_{yz}$ electrons of Au. The quadruplet is split by spin anisotropy due to spin-orbit coupling. Solving \Heff with the numerical renormalization group (NRG) % Wb: reverted my own change we find that at low temperatures $G(T)=a-b \sqrt{T}$ and the ground state impurity entropy is $\ln(2)/2$, a behavior similar to the two-channel Kondo model. Stretching the chain leads to a non Kondo phase, with the physics of the underscreened Kondo model at the quantum critical point.Comment: Accepted in Physical Review Letter

Phase lapses in transmission through interacting two-level quantum dots

We investigate the appearance of pi lapses in the transmission phase theta of a two-level quantum dot with Coulomb interaction U. Using the numerical and functional renormalization group methods we study the entire parameter space for spin-polarized as well as spin-degenerate dots, modeled by spinless or spinful electrons, respectively. We investigate the effect of finite temperatures T. For small T and sufficiently small single-particle spacings delta of the dot levels we find pi phase lapses between two transmission peaks in an overwhelming part of the parameter space of the level-lead couplings. For large delta the appearance or not of a phase lapse between resonances depends on the relative sign of the level-lead couplings in analogy to the U=0 case. We show that this generic scenario is the same for spin-polarized and spin-degenerate dots. We emphasize that in contrast to dots with more levels, for a two-level dot with small delta and generic dot-lead couplings (that is up to cases with special symmetry) the "universal" phase lapse behavior is already established at U=0. The most important effect of the Coulomb interaction is to increase the separation of the transmission resonances. The relation of the appearance of phase lapses to the inversion of the population of the dot levels is discussed. For the spin-polarized case and low temperatures we compare our results to recent mean-field studies. For small delta correlations are found to strongly alter the mean-field picture.Comment: submitted to NJ

Matrix product state comparison of the numerical renormalization group and the variational formulation of the density matrix renormalization group

Wilson's numerical renormalization group (NRG) method for solving quantum impurity models yields a set of energy eigenstates that have the form of matrix product states (MPS). White's density matrix renormalization group (DMRG) for treating quantum lattice problems can likewise be reformulated in terms of MPS. Thus, the latter constitute a common algebraic structure for both approaches. We exploit this fact to compare the NRG approach for the single-impurity Anderson model to a variational matrix product state approach (VMPS), equivalent to single-site DMRG. For the latter, we use an ``unfolded'' Wilson chain, which brings about a significant reduction in numerical costs compared to those of NRG. We show that all NRG eigenstates (kept and discarded) can be reproduced using VMPS, and compare the difference in truncation criteria, sharp vs. smooth in energy space, of the two approaches. Finally, we demonstrate that NRG results can be improved upon systematically by performing a variational optimization in the space of variational matrix product states, using the states produced by NRG as input.Comment: 19 pages, 14 figure