Anisotropic hysteretic Hall-effect and magnetic control of chiral domains in the chiral spin states of Pr2_2Ir2_2O7_7

We uncover a strong anisotropy in both the anomalous Hall effect (AHE) and the magnetoresistance of the chiral spin states of Pr$_2$Ir$_2$O$_7$. The AHE appearing below 1.5 K at zero magnetic field shows hysteresis which is most pronounced for fields cycled along the [111] direction. This hysteresis is compatible with the field-induced growth of domains composed by the 3-in 1-out spin states which remain coexisting with the 2-in 2-out spin ice manifold once the field is removed. Only for fields applied along the [111] direction, we observe a large positive magnetoresistance and Shubnikov de Haas oscillations above a metamagnetic critical field. These observations suggest the reconstruction of the electronic structure of the conduction electrons by the field-induced spin-texture.Comment: 7 pages and 5 figures (including Supplementary Material), Accepted in Physical Review Letter

Photoemission Spectral Weight Transfer and Mass Renormalization in the Fermi-Liquid System La1−x_{1-x}Srx_xTiO3+y/2_{3+y/2}

We have performed a photoemission study of La$_{1-x}$Sr$_x$TiO$_{3+y/2}$ near the filling-control metal-insulator transition (MIT) as a function of hole doping. Mass renormalization deduced from the spectral weight and the width of the quasi-particle band around the chemical potential $\mu$ is compared with that deduced from the electronic specific heat. The result implies that, near the MIT, band narrowing occurs strongly in the vicinity of $\mu$. Spectral weight transfer occurs from the coherent to the incoherent parts upon antiferromagnetic ordering, which we associate with the partial gap opening at $\mu$.Comment: 4 pages, 3 figure

Investigation of the use of microwave image line integrated circuits for use in radiometers and other microwave devices in X-band and above

Program results are described in which the use of a/high permittivity rectangular dielectric image waveguide has been investigated for use in microwave and millimeter wavelength circuits. Launchers from rectangular metal waveguide to image waveguide are described. Theoretical and experimental evaluations of the radiation from curved image waveguides are given. Measurements of attenuation due to conductor and dielectric losses, adhesives, and gaps between the dielectric waveguide and the image plane are included. Various passive components are described and evaluations given. Investigations of various techniques for fabrication of image waveguide circuits using ceramic waveguides are also presented. Program results support the evaluation of the image line approach as an advantageous method for realizing low loss integrated electronic circuits for X-band and above

The electrokinetic behavior of calcium oxalate monohydrate in macromolecular solutions

Electrophoretic mobilities were measured for calcium oxalate monohydrate (COM) in solutions containing macromolecules. Two mucopolysaccharides (sodium heparin and chrondroitin sulfate) and two proteins (positively charged lysozyme and negatively charged bovine serum albumin) were studied as adsorbates. The effects of pH, calcium oxalate surface charge (varied by calcium or oxalate ion activity), and citrate concentration were investigated. All four macromolecules showed evidence for chemical adsorption. The macromolecule concentrations needed for reversing the surface charge indicated that the mucopopolysacchrides have greater affinity for the COM surface than the proteins. The amount of proteins that can chemically adsorb appears to be limited to approximately one monomolecular layer. When the surface charge is high, an insufficient number of proteins can chemically adsorb to neutralize or reverse the surface charge. The remaining surface charge is balanced by proteins held near the surface by longer range electrostatic forces only. Citrate ions at high concentrations appear to compete effectively with the negative protein for surface sites but show no evidence for competing with the positively charged protein

Simple bonding technique for high-temperature ceramic coatings

Coatings, consisting of zirconia powder bonded with orthophosphoric acid and a small amount of hydrofluoric acid, are hard, strong, and refractory, resist thermal shock, and provide good thermal protection. After the aqueous coating is applied to a metallic surface, only a 600 deg F cure is required before service

Universal Scaling Behavior of Anomalous Hall Effect and Anomalous Nernst Effect in Itinerant Ferromagnets

Anomalous Hall effect (AHE) and anomalous Nernst effect (ANE) in a variety of ferromagnetic metals including pure metals, oxides, and chalcogenides, are studied to obtain unified understandings of their origins. We show a universal scaling behavior of anomalous Hall conductivity $\sigma_{xy}$ as a function of longitudinal conductivity $\sigma_{xx}$ over five orders of magnitude, which is well explained by a recent theory of the AHE taking into account both the intrinsic and extrinsic contributions. ANE is closely related with AHE and provides us with further information about the low-temperature electronic state of itinerant ferromagnets. Temperature dependence of transverse Peltier coefficient $\alpha_{xy}$ shows an almost similar behavior among various ferromagnets, and this behavior is in good agreement quantitatively with that expected from the Mott rule.Comment: 4pages, 4figures, 1tabl

Spin Chirality Fluctuation and Anomalous Hall Effect in Itinerant Ferromagnets

The anomalous Hall effect due to the spin chirality order and fluctuation is studied theoretically in a Kondo lattice model without the relativistic spin-orbit interaction. Even without the correlations of the localized spins, $\sigma_{xy}$ can emerge depending on the lattice structure and the spin anisotropy. We reveal the condition for this chirality-fluctuation driven mechanism for $\sigma_{xy}$. Our semiquantitative estimates for a pyrochlore oxide Nd$_2$Mo$_2$O$_7$ give a finite \sigma_{xy} \sim 10 \Ohm^{-1} \cm^{-1} together with a high resistivity \rho_{xx} \sim 10^{-4}-10^{-3} \Ohm \cm, in agreement with experiments.Comment: 5 pages, including 4 figure

(2n×1) Reconstructions of TiO2(011) Revealed by Noncontact Atomic Force Microscopy and Scanning Tunneling Microscopy

We have used noncontact atomic force microscopy (NC-AFM) and scanning tunneling microscopy (STM) to study the rutile TiO2(011) surface. A series of (2n×1) reconstructions were observed, including two types of (4×1) reconstruction. High resolution NC-AFM and STM images indicate that the (4×1)-α phase has the same structural elements as the more widely reported (2×1) reconstruction. An array of analogous higher order (2n×1) reconstructions were also observed where n = 3-5. On the other hand, the (4×1)-β reconstruction seems to be a unique structure without higher order analogues. A model is proposed for this structure that is also based on the (2×1) reconstruction but with additional microfacets of {111} character

Temperature dependent magnetotransport around ν\nu= 1/2 in ZnO heterostructures

The sequence of prominent fractional quantum Hall states up to $\nu$=5/11 around $\nu$=1/2 in a high mobility two-dimensional electron system confined at oxide heterointerface (ZnO) is analyzed in terms of the composite fermion model. The temperature dependence of \Rxx oscillations around $\nu$=1/2 yields an estimation of the composite fermion effective mass, which increases linearly with the magnetic field. This mass is of similar value to an enhanced electron effective mass, which in itself arises from strong electron interaction. The energy gaps of fractional states and the temperature dependence of \Rxx at $\nu$=1/2 point to large residual interactions between composite fermions.Comment: 5 pages, 4 Figure

Magneto-optics induced by the spin chirality in itinerant ferromagnet Nd2_2Mo2_2O7_7

It is demonstrated both theoretically and experimentally that the spin chirality associated with a noncoplanar spin configuration produces a magneto-optical effect. Numerical study of the two-band Hubbard model on a triangle cluster shows that the optical Hall conductivity $\sigma_{xy}(\omega)$ is proportional to the spin chirality. The detailed comparative experiments on pyrochlore-type molybdates $R_2$Mo$_2$O$_7$ with $R=$Nd (Ising-like moments) and $R=$Gd (Heisenberg-like ones) clearly distinguishes the two mechanisms, i.e., spin chirality and spin-orbit interactions. It is concluded that for $R$=Nd, $\sigma_{xy}(\omega)$ is dominated by the spin chirality for the dc ($\omega=0$) and the $d \to d$ incoherent intraband optical transitions between Mo atoms.Comment: 4 pages, 5 figures. submitted to Phys. Rev.