Singlet Ground State and Magnetization Plateaus in Ba3_3Mn2_2O8_8

Magnetic susceptibility and the magnetization process have been measured in \green polycrystal. In this compound, the magnetic manganese ion exists as Mn$^{5+}$ in a tetrahedral environment, and thus the magnetic interaction can be described by an S=1 Heisenberg model. The ground state was found to be a spin singlet with an excitation gap $\Delta/k_{\rm B}=11.2$ K. Magnetization plateaus were observed at zero and at half of the saturation magnetization. These results indicate that the present system can be represented by a coupled antiferromagnetic dimer model.Comment: 4 pages, 4 figures, jpsj styl

Observation of Field-Induced Transverse N\'{e}el Ordering in the Spin Gap System TlCuCl3_3

Neutron elastic scattering experiments have been performed on the spin gap system TlCuCl$_3$ in magnetic fields parallel to the $b$-axis. The magnetic Bragg peaks which indicate the field-induced N\'{e}el ordering were observed for magnetic field higher than the gap field $H_{\rm g}\approx 5.5$ T at $Q=(h, 0, l)$ with odd $l$ in the $a^*-c^*$ plane. The spin structure in the ordered phase was determined. The temperature and field dependence of the Bragg peak intensities and the phase boundary obtained were discussed in connection with a recent theory which describes the field-induced N\'{e}el ordering as a Bose-Einstein condensation of magnons.Comment: 4 pages, 5 eps figures, jpsj styl

Field Induced Multiple Reentrant Quantum Phase Transitions in Randomly Dimerized Antiferromagnetic S=1/2 Heisenberg Chains

The multiple reentrant quantum phase transitions in the $S=1/2$ antiferromagnetic Heisenberg chains with random bond alternation in the magnetic field are investigated by the density matrix renormalization group method combined with the interchain mean field approximation. It is assumed that the odd-th bond is antiferromagnetic with strength $J$ and even-th bond can take the values {\JS} and {\JW} ({\JS} > J > {\JW} > 0) randomly with probability $p$ and $1-p$, respectively. The pure version ($p=0$ and $p=1$) of this model has a spin gap but exhibits a field induced antiferromagnetism in the presence of interchain coupling if Zeeman energy due to the magnetic field exceeds the spin gap. For $0 < p < 1$, the antiferromagnetism is induced by randomness at small field region where the ground state is disordered due to the spin gap in the pure case. At the same time, this model exhibits randomness induced plateaus at several values of magnetization. The antiferromagnetism is destroyed on the plateaus. As a consequence, we find a series of reentrant quantum phase transitions between the transverse antiferromagnetic phases and disordered plateau phases with the increase of the magnetic field for moderate strength of interchain coupling. Above the main plateaus, the magnetization curve consists of a series of small plateaus and the jumps between them, It is also found that the antiferromagnetism is induced by infinitesimal interchain coupling at the jumps between the small plateaus. We conclude that this antiferromagnetism is supported by the mixing of low lying excited states by the staggered interchain mean field even though the spin correlation function is short ranged in the ground state of each chain.Comment: 5 pages, 8 figure

Neutron Diffraction Study of the Pressure-Induced Magnetic Ordering in the Spin Gap System TlCuCl3_3

Neutron elastic scattering measurements have been performed under the hydrostatic pressure in order to investigate the spin structure of the pressure-induced magnetic ordering in the spin gap system TlCuCl$_3$. Below the ordering temperature $T_{\rm N}=16.9$ K for the hydrostatic pressure $P=1.48$ GPa, magnetic Bragg reflections were observed at the reciprocal lattice points {\mib Q}=(h, 0, l) with integer $h$ and odd $l$, which are equivalent to those points with the lowest magnetic excitation energy at ambient pressure. This indicates that the spin gap closes due to the applied pressure. The spin structure of the pressure-induced magnetic ordered state for $P=1.48$ GPa was determined.Comment: 4 pages, 3 figures, 3 eps files, jpsj2.cls styl

Neutron Scattering Study of Magnetic Ordering and Excitations in the Doped Spin Gap System Tl(Cu1−x_{1-x}Mgx_x)Cl3_3

Neutron elastic and inelastic scattering measurements have been performed in order to investigate the spin structure and the magnetic excitations in the impurity-induced antiferromagnetic ordered phase of the doped spin gap system Tl(Cu$_{1-x}$Mg$_x$)Cl$_3$ with $x=0.03$. The magnetic Bragg reflections indicative of the ordering were observed at ${\pmb Q}=(h, 0, l)$ with integer $h$ and odd $l$ below $T_{\rm N}=3.45$ K. It was found that the spin structure of the impurity-induced antiferromagnetic ordered phase on average in Tl(Cu$_{1-x}$Mg$_x$)Cl$_3$ with $x=0.03$ is the same as that of the field-induced magnetic ordered phase for ${\pmb H} \parallel b$ in the parent compound TlCuCl$_3$. The triplet magnetic excitation was clearly observed in the $a^*$-$c^*$ plane and the dispersion relations of the triplet excitation were determined along four different directions. The lowest triplet excitation corresponding to the spin gap was observed at ${\pmb Q}=(h, 0, l)$ with integer $h$ and odd $l$, as observed in TlCuCl$_3$. It was also found that the spin gap increases steeply below $T_{\rm N}$ upon decreasing temperature. This strongly indicates that the impurity-induced antiferromagnetic ordering coexists with the spin gap state in Tl(Cu$_{1-x}$Mg$_x$)Cl$_3$ with $x=0.03$.Comment: 24 pages, 7 figures, 11 eps files, revtex style, will appear in Phys. Rev.

Field- and pressure-induced magnetic quantum phase transitions in TlCuCl_3

Thallium copper chloride is a quantum spin liquid of S = 1/2 Cu^2+ dimers. Interdimer superexchange interactions give a three-dimensional magnon dispersion and a spin gap significantly smaller than the dimer coupling. This gap is closed by an applied hydrostatic pressure of approximately 2kbar or by a magnetic field of 5.6T, offering a unique opportunity to explore the both types of quantum phase transition and their associated critical phenomena. We use a bond-operator formulation to obtain a continuous description of all disordered and ordered phases, and thus of the transitions separating these. Both pressure- and field-induced transitions may be considered as the Bose-Einstein condensation of triplet magnon excitations, and the respective phases of staggered magnetic order as linear combinations of dimer singlet and triplet modes. We focus on the evolution with applied pressure and field of the magnetic excitations in each phase, and in particular on the gapless (Goldstone) modes in the ordered regimes which correspond to phase fluctuations of the ordered moment. The bond-operator description yields a good account of the magnetization curves and of magnon dispersion relations observed by inelastic neutron scattering under applied fields, and a variety of experimental predictions for pressure-dependent measurements.Comment: 20 pages, 17 figure

Dynamics of an anisotropic Haldane antiferromagnet in strong magnetic field

We report the results of elastic and inelastic neutron scattering experiments on the Haldane gap quantum antiferromagnet Ni(C5D14N2)2N3(PF6) performed at mK temperatures in a wide range of magnetic field applied parallel to the S = 1 spin chains. Even though this geometry is closest to an ideal axially symmetric configuration, the Haldane gap closes at the critical field Hc~4T, but reopens again at higher fields. The field dependence of the two lowest magnon modes is experimentally studied and the results are compared with the predictions of several theoretical models. We conclude that of several existing theories, only the recently proposed model [Zheludev et al., cond-mat/0301424 ] is able to reproduce all the features observed experimentally for different field orientations.Comment: 11 pages 8 figures submitted to Phys. Rev.

Pressure-Induced Magnetic Quantum Phase Transition in Gapped Spin System KCuCl3

Magnetization and neutron elastic scattering measurements under a hydrostatic pressure were performed on KCuCl3, which is a three-dimensionally coupled spin dimer system with a gapped ground state. It was found that an intradimer interaction decreases with increasing pressure, while the sum of interdimer interactions increases. This leads to the shrinkage of spin gap. A quantum phase transition from a gapped state to an antiferromagnetic state occurs at Pc ? 8.2 kbar. For P > P c, magnetic Bragg reflections were observed at reciprocal lattice points equivalent to those for the lowest magnetic excitation at zero pressure. This confirms that the spin gap decreases and closes under applied pressure.Comment: 7 pages, 10 figures, submitted to J. Phys. Soc. Jp

Critical Properties of Condensation of Field-Induced Triplet Quasiparticles

A review on the field-induced magnetic ordering is given, together with some results of a quantum Monte Carlo simulation focused on the critical behevior near the quantum critical point.Comment: Proceedings of SPQS, Sendai, 200

Finite temperature excitations of a trapped Bose-Fermi mixture

We present a detailed study of the low-lying collective excitations of a spherically trapped Bose-Fermi mixture at finite temperature in the collisionless regime. The excitation frequencies of the condensate are calculated self-consistently using the static Hartree-Fock-Bogoliubov theory within the Popov approximation. The frequency shifts and damping rates due to the coupled dynamics of the condensate, noncondensate, and degenerate Fermi gas are also taken into account by means of the random phase approximation and linear response theory. In our treatment, the dipole excitation remains close to the bare trapping frequency for all temperatures considered, and thus is consistent with the generalized Kohn theorem. We discuss in some detail the behavior of monopole and quadrupole excitations as a function of the Bose-Fermi coupling. At nonzero temperatures we find that, as the mixture moves towards spatial separation with increasing Bose-Fermi coupling, the damping rate of the monopole (quadrupole) excitation increases (decreases). This provides us a useful signature to identify the phase transition of spatial separation.Comment: 10 pages, 8 figures embedded; to be published in Phys. Rev.