742 research outputs found

    Plasmon signatures in high harmonic generation

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    High harmonic generation in polarizable multi-electron systems is investigated in the framework of multi-configuration time-dependent Hartree-Fock. The harmonic spectra exhibit two cut offs. The first cut off is in agreement with the well established, single active electron cut off law. The second cut off presents a signature of multi-electron dynamics. The strong laser field excites non-linear plasmon oscillations. Electrons that are ionized from one of the multi-plasmon states and recombine to the ground state gain additional energy, thereby creating the second plateau.Comment: Major revision, 12 pages, 5 figures, submitted to J. Phys. B (2005), accepte

    Correlated non-perturbative electron dynamics with quantum trajectories

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    An approach to electron correlation effects in atoms that uses quantum trajectories is presented. A comparison with the exact quantum mechanical results for 1D Helium atom shows that the major features of the correlated ground state distribution and of the strong field ionization dynamics are reproduced with quantum trajectories. The intra-atomic resonant transitions are described accurately by a trajectory ensemble. The present approach reduces significantly the computational time and it can be used for both bound and ionizing electrons.Comment: 9 pages, 4 figure

    Phase Space Approach to Laser-driven Electronic Wavepacket Propagation

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    We propose a phase space method to propagate a quantum wavepacket driven by a strong external field. The method employs the so-called biorthogonal von Neumann basis recently introduced for the calculation of the energy eigenstates of time-independent quantum systems [A. Shimshovitz and D.J. Tannor, arXiv:1201.2299v1]. While the individual elements in this basis set are time-independent, a small subset is chosen in a time-dependent manner to adapt to the evolution of the wavepacket in phase space. We demonstrate the accuracy and efficiency of the present propagation method by calculating the electronic wavepacket in a one-dimensional soft-core atom interacting with a superposition of an intense, few-cycle, near-infrared laser pulse and an attosecond extreme-ultraviolet laser pulse.Comment: 4 pages, 4 figures. The following article has been submitted to the Journal of Chemical Physics. After it is published, it will be found at http://jcp.aip.org

    Two Component Heat Diffusion Observed in CMR Manganites

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    We investigate the low-temperature electron, lattice, and spin dynamics of LaMnO_3 (LMO) and La_0.7Ca_0.3MnO_3 (LCMO) by resonant pump-probe reflectance spectroscopy. Probing the high-spin d-d transition as a function of time delay and probe energy, we compare the responses of the Mott insulator and the double-exchange metal to the photoexcitation. Attempts have previously been made to describe the sub-picosecond dynamics of CMR manganites in terms of a phenomenological three temperature model describing the energy transfer between the electron, lattice and spin subsystems followed by a comparatively slow exponential decay back to the ground state. However, conflicting results have been reported. Here we first show clear evidence of an additional component in the long term relaxation due to film-to-substrate heat diffusion and then develop a modified three temperature model that gives a consistent account for this feature. We confirm our interpretation by using it to deduce the bandgap in LMO. In addition we also model the non-thermal sub-picosecond dynamics, giving a full account of all observed transient features both in the insulating LMO and the metallic LCMO.Comment: 6 pages, 5 figures http://link.aps.org/doi/10.1103/PhysRevB.81.064434 v2: Abstract correcte

    Frank's constant in the hexatic phase

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    Using video-microscopy data of a two-dimensional colloidal system the bond-order correlation function G6 is calculated and used to determine the temperature-dependence of both the orientational correlation length xi6 in the isotropic liquid phase and the Frank constant F_A in the hexatic phase. F_A takes the value 72/pi at the hexatic to isotropic liquid phase transition and diverges at the hexatic to crystal transition as predicted by the KTHNY-theory. This is a quantitative test of the mechanism of breaking the orientational symmetry by disclination unbinding
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